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Journal of Experimental and Theoretical Physics Letters

Experimental Study of the Optical Qubit on the 435-nm Quadrupole Transition in the 171Yb+ Ion

Ilia V. Zalivako, Ilya A. Semerikov, A. S. Borisenko, Mikhail A. Aksenov, Ksenia Yu. Khabarova, N. Kolachevsky

Published Jul 1, 2021• 20 citations
Publisher

Abstract

Ultracold ions provide one of the most promising platforms for quantum computing and make it possible to reach record coherence times, the fidelity of preparation and readout operations, and single- and two-qubit operations. Encoding quantum information in an optical qubit based on the $$^{2}{{S}_{{1/2}}}(F = 0,{{m}_{F}} = 0)$$ → $$^{2}{{D}_{{3/2}}}(F = 2,{{m}_{F}} = 0)$$ quadrupole transition in the 171Yb+ ion at a wavelength of 435.5 nm, which has potential advantages over similar systems in the scaling of the number of qubits and their sensitivity to fluctuations of the magnetic field, is proposed and experimentally studied. The proposed optical qubit in ytterbium is compared to other most widespread types of ion qubits. Experimental results on the implementation of the Pauli-X single-qubit operation are given. The fidelity of the operation is 96% after correction to the error of preparation and readout and is limited by the temperature of the ion.

DOI
10.1134/s0021364021140113

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Ultracold ions provide one of the most promising platforms for quantum computing and make it possible to reach record coherence times, the fidelity of preparation and readout operations, and single- and two-qubit operations. Encoding quantum information in an optical qubit based on the 2S1/2(F=0,mF=0)^{2}{{S}_{{1/2}}}(F = 0,{{m}_{F}} = 0)2S1/2​(F=0,mF​=0) → 2D3/2(F=2,mF=0)^{2}{{D}_{{3/2}}}(F = 2,{{m}_{F}} = 0)2D3/2​(F=2,mF​=0) quadrupole transition in the 171Yb+ ion at a wavelength of 435.5 nm, which has potential advantages over similar systems in the scaling of the number of qubits and their sensitivity to fluctuations of the magnetic field, is proposed and experimentally studied. The proposed optical qubit in ytterbium is compared to other most widespread types of ion qubits. Experimental results on the implementation of the Pauli-X single-qubit operation are given. The fidelity of the operation is 96% after correction to the error of preparation and readout and is limited by the temperature of the ion.
Abstract We report the results of studying a compact laser system designed for manipulating a quantum state of the optical qubit based on the 2S1/2 → 2D3/2 quadrupole transition in the 171Yb+ ion at a wavelength of 435.5 nm. An emission power of the laser system reaches 500 μW at λ = 435.5 nm and the relative frequency instability of at most 3 × 10−15 is achieved at averaging intervals from 0.5 to 50 s with a subtracted linear frequency drift. The compactness of the developed system makes it possible to employ it in transportable systems including optical clocks.
For quantum-information processing (QIP) with trapped ions, the isotope 43Ca+{^{43}\text{C}\text{a}}^{+}43Ca+ offers the combined advantages of a quantum memory with long coherence time, a high-fidelity readout, and the possibility of performing two-qubit gates on a quadrupole transition with a narrow-band laser. Compared to other ions used for quantum computing, 43Ca+{^{43}\text{C}\text{a}}^{+}43Ca+ has a relatively complicated level structure. We discuss how to meet the basic requirements for QIP and demonstrate ground-state cooling, robust state initialization, and efficient readout for the hyperfine qubit with a single 43Ca+{^{43}\text{C}\text{a}}^{+}43Ca+ ion. A microwave field and a Raman light field are used to drive qubit transitions, and the coherence times for both fields are compared. Phase errors due to interferometric instabilities in the Raman field generation do not limit the experiments on a time scale of 100 ms. We find a quantum-information storage time of many seconds for the hyperfine qubit.
Trapped ions offer a controlled and versatile platform for the simulation of spin and spin-boson quantum systems. The Coulomb interaction between ions trapped in a harmonic potential can be used to mediate interactions between effective spins in the ion chain. Generally, coherent operations on ions are performed on ground-state qubits encoded in magnetically insensitive hyperfine sublevels. In this thesis, we extend this toolbox with the aim of simultaneously manipulating both ground-state and optical qubits, with the latter encoded in metastable optically excited states. The optical qubit provides another set of coherent and dissipative operations that can be performed on the ions, opening new avenues for quantum computing and simulation. In our experiment, we use 171Yb+ and 172Yb+ ions to encode ground-state and optical qubits. We discuss the laser setup needed to address the narrow quadrupole transition from 2S1/2 →2 D3/2 of 3.02 Hz linewidth, and we describe spectroscopy techniques to study this transition in both the isotopes. We describe how the low linewidth allows resolved sideband cooling on the shared motional modes in an ion chain, enabling sympathetic cooling with one ion, 172Yb+ , while simultaneously performing coherent operations on the 171Yb+ ion. Finally, we discuss the prospects of using this tool for light-shift entangling gates, showing the flexibility of this trapped-ion system for simulating coherent as well as dissipative quantum systems.
We experimentally demonstrate laser spectroscopy of the electric-quadrupole transition 6s2S1/2−−5d2D3/26s{}^{2}{S}_{1/2}--5d{}^{2}{D}_{3/2}6s2S1/2​−−5d2D3/2​ of a single trapped 171Yb{}^{171}\mathrm{Yb}171Yb ion. The probed transition has a natural linewidth of 3.1 Hz, and is at a wavelength of 435.5 nm. A 171Yb{}^{171}\mathrm{Yb}171Yb ion is laser cooled to the range of the Doppler limit in a radio-frequency Paul trap. The $F=0--{F}^{\ensuremath{'}}=2,$ ${m}_{{F}^{\ensuremath{'}}}=0$ hyperfine component of the 2S1/2−−2D3/2{}^{2}{S}_{1/2}{--}^{2}{D}_{3/2}2S1/2​−−2D3/2​ transition is excited by a laser source whose frequency is controlled by an optical reference cavity of high intrinsic stability. The recoilless carrier component of the vibrational sideband spectrum is resolved with a minimum linewidth of approximately 80 Hz, corresponding to a fractional frequency resolution of $1.2\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}13}.$ This resolution limit is attributed to laser frequency instability. The effective decoherence rates of the residual ion motion are inferred from the observation that the axial and two radial low-frequency first-order secular-vibration sidebands show minimum linewidths in the range of 0.2--1 kHz. Prospects for an optical frequency standard based on the investigated atomic system are discussed.
Trapped ions are currently one of the most promising architectures for realising the quantum information processor. The long lived internal states are ideal for representing qubit states and, through controlled interactions with electromagnetic radiation, ions can be manipulated to execute coherent logic operations. In this thesis an experiment capable of trapping Yb+ ions, including 171Yb+, is presented. Since ion energy can limit the coherence of qubit manipulations, characterisation of an ion trap heating rate is vital. Using a trapped 174Yb+ ion a heating rate consistent with previous measurements of other ion species in similar ion traps is obtained. This result shows abnormal heating of Yb+ does not occur, further solidifying the suitability of this species for quantum information processing. Efficient creation, and cooling of trapped ions requires exact wavelengths for the ionising, cooling and repump transitions. A simple technique to measure the 1S0 ? 1P1 transition wavelengths, required for isotope selective photoionisation of neutral Yb, is developed. Using the technique new wavelengths, accurate to 60 MHz, are obtained and differ from previously published results by 660 MHz. Through a simple modification the technique can also predict Doppler shifted transition frequencies, which may be required in non-perpendicular atom-laser interactions. Using trapped ions, the 2S1=2 ? 2P1/2 Doppler cooling and 2D3/2 ? 2D[3/2]1/2 repump transitions are also measured to a greater accuracy than previously reported. Many experiments require wavelengths which can only be obtained using complex expensive laser systems. To remedy this a simple cost effective laser is developed to enable laser diodes to be operated at sub zero temperatures, extending the range of obtainable wavelengths. Additional diode modulation capabilities allow for the manipulation of atoms and ions with hyperfine structures. The laser is shown to be suitable for manipulating Yb+ ions by cooling a diode from 372 nm to 369 nm and simultaneously generating 2.1 GHz frequency sidebands. Coherent manipulation such as arbitrary qubit rotations, motional coupling and ground state cooling, are required for trapped ion quantum computing. Two photon stimulated Raman transitions are identified as a suitable technique to implement all of these requirements and an investigation into implementing this technique with 171Yb+ is conducted. The possibility of exciting a Raman transition via either a dipole or quadrupole transitions in 171Yb+ is analysed, with dipole transitions preferred because quadrupole transitions are found to be too demanding experimentally. An inexpensive setup, utilising a dipole transition, is designed and tested. Although currently limited the setup shows potential to be an inexpensive, high fidelity method of exciting a Raman transition.
The use of multilevel quantum information carriers, also known as qudits, has attracted significant interest as a way of further scaling quantum computing devices. However, such multilevel systems usually express shorter coherence time than their two-level counterparts, which limits their computational potential. We thus propose and experimentally demonstrate two approaches for realizing the continuous dynamical decoupling of magnetic-sensitive states with mF = ±1 for qudits encoded in optical transition of trapped 171Yb+ ions. We improve the coherence time of qudit levels by an order of magnitude (more than 9 ms) without any magnetic shielding, revealing the potential advantage of the symmetry of the 171Yb+ ion energy structure for counteracting magnetic field noise. Our results are a step toward realizing qudit-based algorithms using trapped ions.