Quantum correlations have been an integral if sometimes discomforting aspect of quantum theory for over 85 years. From the early thought-experiments where they were used to argue that quantum mechanics was incomplete, through to their central position as resources in the modern theory of quantum information theory, quantum correlations have proved a hugely rich topic of study. This thesis explores a range of practical and foundational aspects within this ever developing field. Having reviewed fundamental material, we turn to consider the quantum correlations for a task termed anonymous metrology. This is used to demonstrate an operational distinction within the hierarchy of quantum correlations. Building from this we formulate the concept of quantum delocalised interactions, making use of quantum games to study the necessary correlations. With these we establish strong connections to the concurrence monotone and additionally a link with quantum teleportation. We then move to considering entanglement under motion when relativity is accounted for. We demonstrate how the entanglement between internal energy and motional states can be affected by boosts in an analogous way to the known behaviour for spins, and in a more straightforward manner. We then show how this understanding sheds light on the topic of proper time for quantum clocks. Finally we consider a protocol where entanglement can be used to witness non-classicality of gravity. We present improvements which help to bring the scheme closer to experimental feasibility, together with pointing out a potential loophole and how to close it.
Quantum correlations have been an integral if sometimes discomforting aspect of quantum theory for over 85 years. From the early thought-experiments where they were used to argue that quantum mechanics was incomplete, through to their central position as resources in the modern theory of quantum information theory, quantum correlations have proved a hugely rich topic of study. This thesis explores a range of practical and foundational aspects within this ever developing field. Having reviewed fundamental material, we turn to consider the quantum correlations for a task termed anonymous metrology. This is used to demonstrate an operational distinction within the hierarchy of quantum correlations. Building from this we formulate the concept of quantum delocalised interactions, making use of quantum games to study the necessary correlations. With these we establish strong connections to the concurrence monotone and additionally a link with quantum teleportation. We then move to considering entanglement under motion when relativity is accounted for. We demonstrate how the entanglement between internal energy and motional states can be affected by boosts in an analogous way to the known behaviour for spins, and in a more straightforward manner. We then show how this understanding sheds light on the topic of proper time for quantum clocks. Finally we consider a protocol where entanglement can be used to witness non-classicality of gravity. We present improvements which help to bring the scheme closer to experimental feasibility, together with pointing out a potential loophole and how to close it.
Here we provide the contributions' abstracts published in a volume we edited as a special issue in International Journal of Modern Physics B. The volume deals with the recent progress in quantifying quantum correlations beyond the generic notion of 'correlations in a quantum system'. The main goal of the special issue is to provide authoritative reviews on selected topics discussed in the field in the last few years. Nevertheless many articles contain significant original research. The opening section of the issue is dedicated to foundational aspects of quantum mechanics. The second section deals with diverse quantum information insights into the analysis of quantum resources (like entanglement and quantum discord). Many of the concepts presented in the first part of the issue are applied to spin systems in the third section. The last section of the issue is focused on the dynamics of quantum discord in open systems and in quantum communication protocols.
This thesis establishes a number of connections between foundational issues in quantum theory, and some quantum information applications. It starts with a review of quantum contextuality and non-locality, multipartite entanglement characterisation, and of a few quantum information protocols. Quantum non-locality and contextuality are shown to be essential for different implementations of quantum information protocols known as quantum random access codes and quantum communication complexity protocols. I derive sufficient experimental conditions for tests of these quantum properties. I also discuss how the distribution of quantum information through quantum cloning processes can be useful in quantum computing. Regarding entanglement characterisation, some results are obtained relating two problems, that of additivity of the relative entropy of entanglement, and that of identifying different types of tripartite entanglement in the asymptotic regime of manipulations of many copies of a given state. The thesis ends with a description of an information processing task in which a single qubit substitutes for an arbitrarily large amount of classical communication. This result is interpreted in different ways: as a gap between quantum and classical computation space complexity; as a bound on the amount of classical communication necessary to simulate entanglement; and as a basic result on hidden-variable theories for quantum mechanics. I also show that the advantage of quantum over classical communication can be established in a feasible experiment.
The rapidly developing interdisciplinary field of quantum information, which merges quantum and information science, studies non-classical aspects of quantum systems. These studies are motivated by the promise that the non-classicality can be used to solve tasks more efficiently than classical methods would allow. In many quantum informational studies, non-classical behaviour is attributed to the notion of entanglement. In this thesis we use photons to experimentally investigate fundamental questions such as: What happens to the entanglement in a system when it is affected by noise? In our study of noisy entanglement we pursue the challenging task of creating bound entanglement. Bound entangled states are created through an irreversible process that requires entanglement. Once in the bound regime, entanglement cannot be distilled out through local operations assisted by classical communication. We show that it is possible to experimentally produce four-photon bound entangled states and that a violation of a Bell inequality can be achieved. Moreover, we demonstrate an entanglement-unlocking protocol by relaxing the condition of local operations. We also explore the non-classical nature of quantum mechanics in several single-photon experiments. In these experiments, we show the violation of various inequalities that were derived under the assumption of non-contextuality. Using qutrits we construct and demonstrate the simplest possible test that offers a discrepancy between classical and quantum theory. Furthermore, we perform an experiment in the spirit of the Kochen-Specker theorem to illustrate the state-independence of this theorem. Here, we investigate whether or not measurement outcomes exhibit fully contextual correlations. That is, no part of the correlations can be attributed to the non-contextual theory. Our results show that only a small part of the experimental generated correlations are amenable to a non-contextual interpretation.
In this thesis we examine a variety of question regarding several quantum information-theoretic concepts as they manifest in the context of relativistic quantum fields. In particular, we study the qualitative and quantitative structure of entanglement (as well as more generalized quantum correlations) in field theory. Primarily we study the nature of vacuum entanglement, but consider spatial correlations in more general field states as well. We also discuss several novel aspects of particle creation phenomena, which generally go hand in hand with the presence of field entanglement. Such investigations are important from two perspectives. First, we gain enlightening new insight into the nature of quantum fields and, therefore, into the fundamental constituents of the matter contained in our universe. Second, we are able to consider the possibility of utilizing the relativistic nature of quantum fields as a resource for quantum technological tasks such as entanglement distribution, information processing, and metrology. \n \nAs a general guiding principle, here we approach such questions from an operational perspective. That is, we focus less on the mathematical facts derivable from a given theory and instead attempt to answer in what concretely physical ways such facts manifest themselves. For example, in what ways can vacuum entanglement actually be experimentally detected and measured, at least in principle? Such an approach allows us to circumvent otherwise problematic interpretational issues. It also lends itself more naturally to the proposal of real world experiments regarding, and utilizations of, the physics being investigated. In this thesis we utilize two models of detection as applied to field theory. \n \nThe first is one that we will develop from scratch and use to great effect in a number of studies; this is the non-perturbative oscillator detector. In this context, a ``detector" is simply some quantum system that is allowed to interact in some way with a quantum field. The response of this system then gives us information about the field properties. Typically such studies are done perturbatively, which presents several severe limitations on what may be investigated. We develop an alternative model, in which the detector is identified as a quantum harmonic oscillator, that allows non-perturbative solutions. We go on to apply this model to a variety of studies. We start by the examining the Unruh effect in a cavity setting. Not only are we able to examine the thermalization behavior of such a detector (which is stronger than what can be achieved perturbatively), we also demonstrate that the Unruh response is largely independent of the cavity boundary conditions, indicating a surprising amount of generality and universality to the phenomenon. We also consider the spacelike extraction of spatial entanglement by a set of such detectors. This includes the harvesting of genuine tripartite entanglement out of the vacuum, as well as the observation that the extractable quantum discord (a generalized measure of quantum correlations) can be greatly amplified by thermal fluctuations in the field, in opposite behavior to entanglement. This calls into question the nature of quantum discord, but also suggests at the possibility of actually using environmental noise as a quantum computational resource. Next, we use the oscillator detector model to great effect by proposing a method of reliably and sustainably generating and distributing entanglement via a cavity field. This protocol is inherently non-perturbative, and we refer to it as entanglement farming. Lastly, we modify the farming scenario to discover a very sensitive resonance effect that generates a large difference in the protocol output due to a minute change in system parameters, including the length of cavity being used. We put this forth as a potential method of quantum seismic metrology. \n \nThe second model that we will consider simply involves performing projective measurements onto a given set of field modes. We will find, however, that such an approach allows us to solve previously intractable problems. In particular, we apply this procedure to the physically sensible choice of localized, positive frequency field modes. Using this model we perform two different studies. In the first, we consider the response of an observer accelerating not through the vacuum state but rather a thermal state. Such a setting has not been (properly) studied previously, due to the computational challenges involved. By applying the localized projective measurement model we are able determine that such an observer sees both an Unruh response from acceleration and a response from the field thermality and that, critically, these responses are distinguishable. We then go on to examine the degradation of quantum correlations between two observers due to the acceleration of one of the observers. This is a prototypical scenario of interest and, by applying realistic measurement assumptions, we obtain results qualitatively different from many previous works on the issue. \n \nIn addition to these models, we question the nature of vacuum entanglement and particle creation by considering an operationally straightforward procedure that greatly demystifies these phenomena and puts them on to solid, physically concrete grounds. This operation is that of very quickly introducing a boundary condition onto one's field, for example by creating a mirror. The real particles generated in this process will then be quantum entangled with each other, even if they are created at spatially separate locations, and this entanglement derives exactly from the previously present vacuum entanglement. Not only does this realization provide an operationally satisfying interpretation of vacuum entanglement, it also suggests a straightforward procedure for its experimental verification. \n \nIn all of this, the computational framework that we will rely upon is that of Gaussian quantum mechanics. This is a restriction of continuous variable quantum mechanics that, while limited in its applicability, provides extremely powerful computational tools in the cases that it may be used. The scenarios of interest in this thesis fall within this category and lend themselves naturally to a Gaussian approach. With this we are able to perform, near trivially, many otherwise intractable studies.
Quantum mechanics has achieved unparalleled success as an operational theory, describing a wide range of experiments to remarkable accuracy. However, the physical foundations on which it rests remain as puzzling as they were a century ago, and a concise statement of the physical principles that underlie quantum mechanics is still outstanding. One promising approach holds that these principles should be formulated in terms of information, since many of the counter-intuitive effects in quantum theory concern questions such as what one can know about a quantum system and how the information encoded therein can be processed and distributed between parties. Another challenging feature of quantum theory is its incompatibility with the other cornerstone of modern physics, general relativity. In order to reconcile the two, one must identify and retain only the essential concepts and principles of each theory, and in the case of general relativity, causality has been identified as such a concept. This raises the question of how our classical understanding of causality must change when quantum theory is taken into account. In order to address these questions about information, knowledge and causality, I turn to the framework of causal models. In classical statistics, causal models explain the relations among a set of variables in terms of causal influences, which makes them a powerful tool for structuring our knowledge about complex systems and developing strategies for interacting with them. More importantly, the framework provides the conceptual underpinnings and mathematical methods for addressing questions about causation, information and knowledge in a rigorous manner. In this thesis, I develop a version of the classical causal models framework that is compatible with quantum theory and explore its physical implications. \n \n \nA first step is to define quantum versions of fundamental elements such as variables, conditionals and belief propagation rules. This allows one to consider the question of what one can come to know about a quantum variable from the point of view of causal modelling. The conditionals relating quantum variables are found to have a richer structure than their classical counterparts, which can be exploited for the task of discerning causal relations given limited data -- a central problem in classical causal modelling. The mathematical properties of quantum conditionals also establish a correspondence between various classes of two-party correlations, such as bound and distillable entanglement, and the types of causal structures that can give rise to them, which may become a useful tool for entanglement theory and quantum information processing. In the context of open quantum systems dynamics, quantum causal models provide a clear physical explanation of not completely positive maps and, more broadly, of non-Markovian quantum dynamics. Finally, I consider the possibility of non-classical effects in the way that different causal mechanisms are combined -- that is, non-classical causal structures. For the simple case of two causally ordered variables, I propose indicators that witness different classes of combinations of causal mechanisms, including a non-classical mixture, and describe an experiment realizing examples of the different classes. \n \n \nAs these results illustrate, the framework of quantum causal models provides both greater conceptual clarity and a comprehensive mathematical formalism for studying a diverse set of problems, ranging from foundational questions to applications in open systems dynamics and the exploration of non-classical causal structures, which are likely to feature in a future theory of quantum gravity. The material presented in this thesis is intended as a foundation and inspiration for further applications of quantum causal models.
100±Δt Years of Quantum Uncertainty: From Origins to Modern Insights
Heisenberg's uncertainty principle is a cornerstone of quantum mechanics, marking a decisive departure from classical physics. Conceived almost a century ago through a thought experiment showing that measuring an electron's position inevitably disturbs its momentum, it began as a deceptively simple idea that sparked countless studies and grew into the rich research field it is today. This review traces its development into a spectrum of mathematical formulations -- known as uncertainty relations -- and explores their interconnections and wide-ranging applications. We highlight its central role in quantum metrology, where it underpins strategies for extracting information from quantum systems with ever-increasing precision, and its links to multiparameter estimation and squeezed states. This review, dedicated to the centenary of the uncertainty principle, reflects on how it has deepened our understanding of quantum theory and driven practical advances, and looks ahead to a century poised for further surprising and transformative discoveries.