The rapidly developing interdisciplinary field of quantum information, which merges quantum and information science, studies non-classical aspects of quantum systems. These studies are motivated by the promise that the non-classicality can be used to solve tasks more efficiently than classical methods would allow. In many quantum informational studies, non-classical behaviour is attributed to the notion of entanglement. In this thesis we use photons to experimentally investigate fundamental questions such as: What happens to the entanglement in a system when it is affected by noise? In our study of noisy entanglement we pursue the challenging task of creating bound entanglement. Bound entangled states are created through an irreversible process that requires entanglement. Once in the bound regime, entanglement cannot be distilled out through local operations assisted by classical communication. We show that it is possible to experimentally produce four-photon bound entangled states and that a violation of a Bell inequality can be achieved. Moreover, we demonstrate an entanglement-unlocking protocol by relaxing the condition of local operations. We also explore the non-classical nature of quantum mechanics in several single-photon experiments. In these experiments, we show the violation of various inequalities that were derived under the assumption of non-contextuality. Using qutrits we construct and demonstrate the simplest possible test that offers a discrepancy between classical and quantum theory. Furthermore, we perform an experiment in the spirit of the Kochen-Specker theorem to illustrate the state-independence of this theorem. Here, we investigate whether or not measurement outcomes exhibit fully contextual correlations. That is, no part of the correlations can be attributed to the non-contextual theory. Our results show that only a small part of the experimental generated correlations are amenable to a non-contextual interpretation.
The rapidly developing interdisciplinary field of quantum information, which merges quantum and information science, studies non-classical aspects of quantum systems. These studies are motivated by the promise that the non-classicality can be used to solve tasks more efficiently than classical methods would allow. In many quantum informational studies, non-classical behaviour is attributed to the notion of entanglement. In this thesis we use photons to experimentally investigate fundamental questions such as: What happens to the entanglement in a system when it is affected by noise? In our study of noisy entanglement we pursue the challenging task of creating bound entanglement. Bound entangled states are created through an irreversible process that requires entanglement. Once in the bound regime, entanglement cannot be distilled out through local operations assisted by classical communication. We show that it is possible to experimentally produce four-photon bound entangled states and that a violation of a Bell inequality can be achieved. Moreover, we demonstrate an entanglement-unlocking protocol by relaxing the condition of local operations. We also explore the non-classical nature of quantum mechanics in several single-photon experiments. In these experiments, we show the violation of various inequalities that were derived under the assumption of non-contextuality. Using qutrits we construct and demonstrate the simplest possible test that offers a discrepancy between classical and quantum theory. Furthermore, we perform an experiment in the spirit of the Kochen-Specker theorem to illustrate the state-independence of this theorem. Here, we investigate whether or not measurement outcomes exhibit fully contextual correlations. That is, no part of the correlations can be attributed to the non-contextual theory. Our results show that only a small part of the experimental generated correlations are amenable to a non-contextual interpretation.
There are two powerful arguments against the possibility of extending quantum mechanics, the violation of Bell inequalities and the Kochen-Specker theorem, but the connection between the two remains confused. Following the distinctive strategy proposed by Cabello [Phys. Rev. Lett. 127, 070401 (2021)], Bell inequalities can be violated by state-independent contextuality sets. However, the experimental realization of such ideas is challenging as it requires high-dimensional entanglement. Orbital angular momentum provides an unlimited state space and the number of effective dimensions can be readily tailored as required. We performed an experimental test of non-locality based on Bell inequalities from contextuality, using orbital angular momentum entanglement in a bipartite photonic system. Our experiment not only shows a new way to produce non-locality but also connects contextuality and non-locality, two fundamental quantum resources that are critical for quantum computation and secure communication tasks.
Quantum mechanics is nonlocal, meaning it cannot be described by any classical local hidden variable model. In this thesis we study two aspects of quantum nonlocality. Part I addresses the question of what classical resources are required to simulate nonlocal quantum correlations. We start by constructing new local models for noisy entangled quantum states. These constructions exploit the connection between nonlocality and Grothendieck's inequality, first noticed by Tsirelson. Next, we consider local models augmented by a limited amount of classical communication. After generalizing Bell inequalities to this setting, we show that (i) one bit of communication is sufficient to simulate the correlations of projective measurements on a maximally entangled state of two qubits, and (ii) five bits of communication are sufficient to simulate the joint correlation of two-outcome measurements on any bipartite quantum state. The latter result can be interpreted as a stronger (constrained) version of Grothendieck's inequality. In part II, we investigate the monogamy of nonlocal correlations. In a setting where three parties, A, B, and C, share an entangled quantum state of arbitrary dimension, we: (i) bound the trade-off between AB's and AC's violation of the CHSH inequality, obtaining an intriguing generalization of Tsirelson's bound, and (ii) demonstrate that forcing B and C to be classically correlated prevents A and B from violating certain Bell inequalities. We study not only correlations that arise within quantum theory, but also arbitrary correlations that do not allow signaling between separate groups of parties. These results are based on new techniques for obtaining Tsirelson bounds, or bounds on the quantum value of a Bell inequality, and have applications to interactive proof systems and cryptography.
Quantum information science explores the foundational aspects of quantum mechanics and its ombination with information science for new information technologies. The underlying key resource is non-classical correlations. These counter-intuitive correlations between quantum systems can be used for encoding, transmitting and measuring information in quantum information tasks. Although quantum properties can be used in a variety of systems, here we explore photons. These information carriers are fast, easy to generate and manipulate and only interact weakly with the environment. These properties make them to excellent candidates to be employed in experiments. Developing quantum technology, such as single photon sources and single photon detectors, allows us to investigate the foundational aspects of quantum mechanics in quantum information tasks. These tasks use non-classical correlations, which form a hierarchy, from Bell nonlocality to Einstein-Podolsky-Rosen (EPR) steering to quantum nonseparability. Two systems are nonlocally correlated, when measuring one system affects the measurement results on the other system, hence the name `steering. In test for non-classical correlations, we share a quantum state between two observers which are trusted or untrusted. While observers are both untrusted or trusted in entanglement witness tests and Bell inequality violations, respectively, EPR-steering is distinct from these two classes by its fundamental asymmetry: one party is trusted while the other is untrusted.
Abstract Contextuality is a phenomenon at the heart of quantum mechanics different from classical behavior and has been recently identified as a resource in quantum information processing. Experimental demonstration of contextuality is thus an important goal. We experimentally demonstrate a test of state-independent contextuality in a four-dimensional Hilbert space with single photons and violate the inequality by at least 387 standard deviations. Despite imperfections and possible measurement disturbance, our results cannot be explained in non-contextual models. We also provide a theoretical analysis of a test of contextuality with a coherent light field and show how the definitions affect the emergence of non-classical correlations. Our result sheds new light on the conflict between quantum and classical physics.
The photon is a quantum system that is by nature robust against noise, and fast travelling, providing an ideal information carrier for quantum information science. The field of quantum information science has generated a great deal of interest for both researchers and the public due to the advantages it can have over classical technologies in areas including communication, computing and cryptography. In this thesis, I explore several different ways that photons can be used to realize quantum information advantages and enable quantum technologies, information tasks and fundamental studies of physics. A strong emphasis is placed on their practical implementation in optical experiments, where the challenges of noise, loss and device imperfections must be considered and combated. I utilize spontaneous parametric downconversion-based sources of high-quality single photons, and their polarization, path, and temporal degrees of freedom for encoding quantum information. In my first experimental project, I demonstrate the first violation of noncontextuality with time-polarization intraparticle entangled states encoded in a single photon by implementing a powerful interference-based measurement technique for photonic states. I perform a test of noncontextuality, acquiring a parameter |SCHSH| = 2.744 ± 0.006, which violates the classical bound of 2 by over 110 standard deviations, rigorously certifying both entanglement and contextuality of the system. We propose a new approach for preparing and measuring high-dimensional time-bin states, that overcomes many of the limitations of previous techniques, and demonstrate it for time-bin qubits and qutrits. In the next experimental project, I investigate the topic of universal cloning in quantum steering-with cloning and steering being two fundamental aspects of quantum physics deeply involved in the security of quantum protocols. I report the first experimental demonstration of cloned quantum steering, showing a simultaneous violation in a steering test by two clones made from one part of an entangled pair of photons. This provides a conclusive result on the question of whether the cloning of quantum steering is possible. We also present theoretical results that clarify our understanding of cloned steering for qubits: we find a no-go theorem where quantum steering can only be copied by a qubit universal cloning machine for 2 and 3 clones, and a monogamy relation where for N clones, steering is only possible if a minimum of N + 1 measurements are performed on each clone. I discuss the field of random number generation, and study how quantum physics allows for certifiably unpredictable random sequences, without needing complete trust in all of the physical devices, offering high levels of security over classical approaches. I report the first discrete-variable detection-loophole-free implementation of one-sided device-independent randomness expansion of certified random bits, based on the quantum steering task. These results illustrate an approach to secure randomness with greater tolerance to noise and loss compared to Bell test-based protocols. The final experimental project looks at quantum autoencoders, which are a quantum machine learning tool that we investigate for the purpose of denoising quantum states. I model and simulate a denoising quantum autoencoder which compresses ququarts into a qubit space and reconstructs noise-reduced ququart states. I construct an experimental apparatus that implements this device, and demonstrate quantum state tomography of ququart states, and the training of the autoencoder.