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Optics Express

High-precision cavity spectroscopy using high-frequency squeezed light

J. Junker, D. M. Wilken, Elanor H. Huntington, M. Heurs

Published Jan 15, 2021• 12 citations
Publisher

Abstract

In this article, we present a novel spectroscopy technique that improves the signal-to-shot-noise ratio without the need to increase the laser power. Detrimental effects by technical noise sources are avoided by frequency-modulation techniques (frequency up-shifting). Superimposing the signal on non-classical states of light leads to a reduced quantum noise floor. Our method reveals in a proof-of-concept experiment small signals at Hz to kHz frequencies even below the shot noise limit. Our theoretical calculations fully support our experimental findings. The proposed technique is interesting for applications such as high-precision cavity spectroscopy, e.g., for explosive trace gas detection where the specific gas might set an upper limit for the laser power employed.

DOI
10.1364/oe.416713

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•Sep 25, 2020•1 citation
In this article, we present a novel spectroscopy technique that improves the signal-to-shot-noise ratio without the need to increase the laser power. Detrimental effects by technical noise sources are avoided by frequency-modulation techniques (frequency up-shifting). Superimposing the signal on non-classical states of light leads to a reduced quantum noise floor. Our method reveals in a proof-of-concept experiment small signals at Hz to kHz frequencies even below the shot noise limit. Our theoretical calculations fully support our experimental findings. The proposed technique is interesting for applications such as high-precision cavity spectroscopy, e.g., for explosive trace gas detection where the specific gas might set an upper limit for the laser power employed.
High levels of laser power stability are necessary for high precision metrology applications. The classical limit for the achievable power stability is determined by the shot noise of the light used to generate a power control signal. Increasing the power of the detected light reduces the relative shot noise level and allows higher stabilities. However, sufficiently high power is not always available and the detection of high laser powers is challenging. Here, we demonstrate a nonclassical way to improve the achievable power stability without increasing the detected power. By the injection of a squeezed vacuum field of light we improve the classical laser power stability beyond its shot noise limit by 9.4_{-0.6}^{+0.6} dB at Fourier frequencies between 5 and 80 kHz. For only 90.6 μA of detected photocurrent we achieve a relative laser power noise of 2.0_{-0.1}^{+0.1}×10^{-8}/sqrt[Hz]. This is the first demonstration of a squeezed light-enhanced laser power stabilization and its performance is equivalent to an almost tenfold increase of detected laser power in a classical scheme. The analysis reveals that the technique presented here has the potential to achieve stability levels of 4.2×10^{-10}/sqrt[Hz] with 58 mA photocurrent measured on a single photodetector.
Low-power-noise lasers are essential for many high-precision experiments. Shot noise imposes a fundamental limit on the power stability achievable with classical light sources. In this Letter, we report the generation of bright squeezed light in the audio band, which can improve the sensitivity of otherwise shot-noise-limited measurements. The bright squeezed light source is experimentally realized via the use of squeezed vacuum in a power stabilization scheme. We demonstrate a laser beam at a power of 9.9 mW with a broadband power noise suppression below the classical stabilization limit by up to 8 . 7 − 0.4 + 0.3 dB in the audio band, resulting in a bright squeezed beam with a power noise of 5 . 7 − 0.4 + 0.3 dB below shot noise for frequencies from 6 kHz to 20 kHz. We further conceptually outline a method to surpass this result in the future.
The optical shot-noise limit of a laser beam represents the classical limit in precision and signal to noise ratio achievable in optical sensors and imaging systems. It is known that quantum states of light, such as squeezed light and quantum correlated twin beams can be used to enhance precision and signal to noise ratio to beyond this limit. This promises optical sensors with fundamentally superior performance to the state of the art. While quantum-enhanced signal to noise ratio has been demonstrated with macroscopic powers of squeezed probe beam, demonstrations of quantum enhanced precision have remained at extremely low powers of light (femto-Watts). Here we will give examples where increasing SNR with quantum light is not sufficient to increase precision and we will review proof of principle experiments that have demonstrated sub shot noise precision, including for absorption spectroscopy and imaging. We will also report our efforts to achieve this sub-shot-noise precision performance for transmission measurement with ~0.1mW of average probe power, equating to ~10W peak power in a pulsed experiment. Time permitting, we will discuss how integrated optics and integrated electronics enables 10s GHz bandwidth in the detection of squeezed light, for integrated quantum sensor technology.
Absorption spectroscopy is a widely used technique that permits the detection and characterization of gas species at low concentrations. We propose a sensing strategy combining the advantages of frequency modulation spectroscopy with the reduced noise properties accessible by squeezing the probe state. A homodyne detection scheme allows the simultaneous measurement of the absorption at multiple frequencies and is robust against dispersion across the absorption profile. We predict a significant enhancement of the signal-to-noise ratio that scales exponentially with the squeezing factor. An order of magnitude improvement beyond the standard quantum limit is possible with state-of-the-art squeezing levels facilitating high precision gas sensing.
A phase-sensitive (PS) heterodyne detector is intrinsically resistant to classical noises and useful in measurement of low-frequency signals below the shot noise. Despite the existence of image band vacuum, we show that the quantum-noise power level of this heterodyne detector sensing a coherent signal is exactly one light quantum per measurement time, i.e., twice the vacuum fluctuation power, which can be further reduced by use of squeezed light. We then report on an experiment on a PS heterodyne detector with a 10 Hz 1.0×10−18 W optical signal (1064 nm wavelength) at its input. The noise floor of the unmodulated coherent light is 2.2(±0.1)×10−19 W/Hz from 2 Hz to 20 Hz, and the signal-to-noise ratio is about 6.6 dB for the measured signal when the resolution bandwidth is 1 Hz. The quantum noise floor is reduced by 1.6(±0.3)dB when squeezed light is used, and the sub-shot-noise power spectral density is 1.6(±0.1)×10−19 W/Hz between 2 Hz and 20 Hz. This work should be an important advance towards squeezing-improved precision measurements of low-frequency signals with heterodyne detectors, including audio-band gravitational-wave detection.
Squeezed light has lower quantum noise in amplitude or phase than the quantum noise limit (QNL) of classical light. This enables enhancing sensitivity -- quantified by the signal-to-noise ratio (SNR) -- to beyond the QNL in optical techniques such as spectroscopy, gravitational wave detection, magnetometry and imaging. Precision -- the variance of repeated estimates -- has also been enhanced beyond the QNL using squeezed vacuum to estimate optical phase and transmission. However, demonstrations have been limited to femtowatts of probe power. Here we demonstrate simultaneous precision and sensitivity beyond the QNL for estimating modulated transmission using a squeezed amplitude probe of 0.2 mW average (25 W peak) power. This corresponds to 8 orders of magnitude above the power limitations of previous sub-QNL precision measurements. Our theory and experiment show precision enhancement scales with the amount of squeezing and increases with the resolution bandwidth of detection. We conclude that quantum enhanced precision in estimating a modulated transmission increases when observing dynamics at ∼\sim∼ kHz and above. This opens the way to performing measurements that compete with the optical powers of current classical techniques, but have superior precision and sensitivity beyond the classical limit.