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High Power Laser Science and Engineering

A perspective on high photon flux nonclassical light and applications in nonlinear optics

Theocharis Lamprou, Ioannis Liontos, Nikolaos C. Papadakis, P. Tzallas

Published Jan 1, 2020• 13 citations
Publisher

Abstract

Abstract Nonclassical light sources have a vital role in quantum optics as they offer a unique resource for studies in quantum technology. However, their applicability is restricted by their low intensity, while the development of new schemes producing intense nonclassical light is a challenging task. In this perspective article, we discuss potential schemes that could be used towards the development of high photon flux nonclassical light sources and their future prospects in nonlinear optics.

DOI
10.1017/hpl.2020.44

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Abstract Nonclassical light sources have a vital role in quantum optics as they offer a unique resource for studies in quantum technology. However, their applicability is restricted by their low intensity, while the development of new schemes producing intense nonclassical light is a challenging task. In this perspective article, we discuss potential schemes that could be used towards the development of high photon flux nonclassical light sources and their future prospects in nonlinear optics.
Integrated optical devices will play a central role in the future development of nonlinear quantum photonics. Here we consider the generation of nonclassical states of light within them with a focus on Gaussian states beyond the low-gain, single photon pair regime accurately described by perturbation theory. Starting from the solid foundation provided by Maxwell’s equations, we then move to applications by presenting a unified formulation that allows for a comparison of stimulated and spontaneous experiments in ring resonators and nanophotonic waveguides and leads directly to the calculation of the quantum states of light generated in high-gain nonlinear quantum photonic experiments.
Sources of highly nonclassical light are important building blocks of many proposed implementations of optical quantum technologies [1]. The most common realisations of nonclassical light sources are either based on two-level quantum emitters or on nonlinear sources of photon pairs and squeezed light [2] and are generally limited in the properties of the quantum states of light they can efficiently generate: single-photon states for two-level systems and squeezed states (with a Gaussian Wigner function) for nonlinear sources.
Quantum non-Gaussianity (QNG) corresponds to an essential resource in many prospective applications of quantum technologies. QNG states of light have been demonstrated in a broad range of experimental platforms with various complementary advantages [1]. However, in order to allow for their direct and efficient utilization for interaction with the target quantum system, their degrees of freedom have to be well-defined and controllable. This imposes a requirement on the generation of QNG light in a single optical mode. While the intrinsic single-photon sources including trapped ions, atoms, or molecules, naturally offer a close-to a single mode emission, their technologically more accessible counterparts including majority of the solid-state emitters and sources based on heralded generation of nonclassical states in various parametric nonlinear processes typically provide a multi-mode output. Although several demonstrations of a single-mode operation of nonclassical light sources based on these platforms have been recently demonstrated, an unambiguous observation of a single-mode QNG light has never been presented.
Ultrashort light pulses play an important role in the generation, manipulation and characterization of nonclassical light. Nonclassical light is often generated from a classical pump beam using a nonlinear optical process. One might expect that the high peak intensity of ultrashort pulses would provide the necessary driver for such processes, and this is indeed the case. Ultrashort pulses have been used to generate squeezed states, and quadrature entangled states via three and four wave mixing, photon number states, polarization and frequency or directional entangled photon pairs states via three wave mixing.
Recent progress in meta-optics, particularly the development of metasurfaces, has enabled compact, tunable, and integrable control over the amplitude, phase, polarization, and wavefront of light, thereby allowing a paradigm shift in traditional optical science and engineering. In parallel, the ability to generate and precisely manipulate nonclassical light is central to quantum optics, enabling key functionalities in secure quantum communication, precision measurement, and scalable quantum computation. This review aims to bridge these two rapidly advancing fields by presenting recent progress in the application of structured materials to the manipulation of quantum states of light. We begin by introducing the concept of singular optics, followed by a discussion of various families of spatially and temporally structured beams that form the foundation for many of the phenomena explored in quantum photonics. Next, we revisit the theoretical framework of quantum optics, including the formalism of photon quantization and the principles governing quantum frequency conversion. We then examine how metasurfaces can be engineered to enable highly efficient nonlinear quantum processes, including both up-conversion and down-conversion, thereby offering new approaches for generating and controlling complex quantum states. Furthermore, we discuss the crucial role of structured materials in shaping the properties of quantum light and in applications such as quantum ghost imaging. The review concludes by identifying emerging directions for integrating meta-optical platforms with quantum systems, highlighting their potential for scalable manipulation of nonclassical light at the nanoscale.
Nonclassical photon sources are key components in quantum information science and technology. Here, the basic principles and progresses for single photon generation and their further manipulation based on second- or third-order nonlinear processes in various degrees of freedom are briefly reviewed and discussed. Based on spontaneous parametric down-conversion and spontaneous four-wave mixing, various nonlinear materials such as quasi-phase-matching crystals, dispersion-shifted fibers, and silicon-on-insulator waveguides are used for single photon generation. The kinds of entanglement generated include polarization, time-energy, time-bin, and orbital angular momentum. The key ingredient for photon pair generation in nonlinear processes is described and discussed. Besides, we also introduce quantum frequency conversion for converting a single photon from one wavelength to another wavelength, while keeping its quantum properties unchanged. Finally, we give a comprehensive conclusion and discussion about future perspectives for single photon generation and manipulation in nonlinear processes. This chapter will provide an overview about the status, current challenge, and future perspectives about single photon generation and processing in nonlinear processes.