Measurement of the argon-gas-induced broadening and line shifting of the barium Rydberg level 6s24d 1 D 2 by two-photon resonant nondegenerate four-wave mixing
Jiang Sun, Zhiqiang Xiong, Juan Sun +2 more
We apply two-photon resonant nondegenerate four-wave mixing with a resonant intermediate state to the observation of the broadening and shifting of the barium Rydberg level 6s24d 1 D 2 by collision with argon. The collision broadening and shifting cross sections are measured. This technique is purely optical, and can investigate the pressure dependence of the transverse relaxation rate Γ 21 between the Rydberg state and an intermediate state, as well as the transverse relaxation rate Γ 20 between the Rydberg state and the ground state.
Chinese Physics B•Jun 1, 2012•1 citation