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On the quasi-static evolution of nonequilibrium steady states

Walid K. Abou Salem

Published Jan 1, 2007• 19 citations
Publisher

Abstract

The quasi-static evolution of steady states far from equilibrium is investigated from the point of view of quantum statistical mechanics. As a concrete example of a thermodynamic system, a two-level quantum dot coupled to several reservoirs of free fermions at different temperatures is considered. A novel adiabatic theorem for unbounded and nonnormal generators of evolution is proven and applied to study the quasi-static evolution of the nonequilibrium steady state (NESS) of the coupled system. © Birkhäuser Verlag Basel/Switzerland 2007.

DOI
10.3929/ethz-b-000067125

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The quasi-static evolution of steady states far from equilibrium is investigated from the point of view of quantum statistical mechanics. As a concrete example of a thermodynamic system, a two-level quantum dot coupled to several reservoirs of free fermions at different temperatures is considered. A novel adiabatic theorem for unbounded and nonnormal generators of evolution is proven and applied to study the quasi-static evolution of the nonequilibrium steady state (NESS) of the coupled system. © Birkhäuser Verlag Basel/Switzerland 2007.
The fluctuations of macroscopic observables in quantum systems which are in a nonequilibrium steady state are studied rigorously in the thermodynamic limit. In particular, the nonequilibrium steady state (NESS) of a quantum spin system that is composed of two infinite reservoirs at different temperatures coupled in a bounded region is considered. Under suitable assumptions on the interaction and the asymptotics of the fluctuations, a nonequilibrium central limit theorem for the fluctuations of the NESS expectation value of the empirical average of observables is proven by showing the analyticity of the corresponding moment generating function in a neighbourhood of the origin using the cluster expansion method. Furthermore, the large deviation principle is proven for a class of observables by establishing the existence and differentiability of the corresponding moment generating function.
Based on a recent progress in nonequilibrium statistical mechanics of infinitely extended quantum systems, a nonequlibrium steady state (NESS) is constructed for a single-level quantum dot interacting with two free reservoirs under less general but more practically useful conditions than the previous works. As an example, a model of an Ahoronov-Bohm ring with a quantum dot is studied in detail. Then, NESS is shown to be regarded as a MacLennan-Zubarev ensemble. A formal relation between response and correlation at NESS is derived as well.
The purpose of this work is to discuss recent progress in deriving the fundamental laws of thermodynamics (0 th, 1 st and 2 nd-law) from nonequilibrium quantum statistical mechanics. Basic thermodynamic notions are clarified and different reversible and irreversible thermodynamic processes are studied from the point of view of quantum statistical mechanics. Special emphasis is put on new adiabatic theorems for steady states close to and far from equilibrium, and on investigating cyclic thermodynamic processes using an extension of Floquet theory. This work is based on the author’s doctoral thesis, ETH-Diss 16187.
The purpose of this work is to discuss recent progress in deriving the fundamental laws of thermodynamics (0th, 1st and 2nd-law) from nonequilibrium quantum statistical mechanics. Basic thermodynamic notions are clarified and different reversible and irreversible thermodynamic processes are studied from the point of view of quantum statistical mechanics. Special emphasis is put on new adiabatic theorems for steady states close to and far from equilibrium, and on investigating cyclic thermodynamic processes using an extension of Floquet theory.
Systems whose boundaries are in contact with heat baths at different temperatures allow for the realization of nonequilibrium steady states (NESS) characterized by distribution functions that are still time independent, yet different from the equilibrium distributions. Such states have interesting properties even in classical statistical mechanics, but recently their quantum analogs have received attention, for both fundamental and applied reasons. This review provides an account of recent progress in this field. It introduces various models to describe the rich NESS phenomenology and covers analytic and numerical methods for analyzing them.
We develop a method of calculating the nonequilibrium steady state (NESS) of an open quantum system that is weakly coupled to reservoirs in different equilibrium states. We describe the system using a Redfield-type quantum master equation (QME). We decompose the Redfield QME into a Lindblad-type QME and the remaining part R\mathcal{R}R. Regarding the steady state of the Lindblad QME as the unperturbed solution, we perform a perturbative calculation with respect to R\mathcal{R}R to obtain the NESS of the Redfield QME. The NESS thus determined is exact up to the first order in the system-reservoir coupling strength (pump/loss rate), which is the same as the order of validity of the QME. An advantage of the proposed method in numerical computation is its applicability to systems larger than those in methods of directly solving the original Redfield QME. We apply the method to a noninteracting fermion system to obtain an analytical expression of the NESS density matrix. We also numerically demonstrate the method in a nonequilibrium quantum spin chain.