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A high-sensitivity push-pull magnetometer

Breschi, Evelina, Grujić, Zoran D., Knowles, Paul E., Antoine Weis

Published Jun 5, 2014• 20 citations
OpenAlex

Abstract

We describe our approach to atomic magnetometry based on the push-pull optical pumping technique. Cesium vapor is pumped and probed by a resonant laser beam whose circular polarization is modulated synchronously with the spin evolution dynamics induced by a static magnetic field. The magnetometer is operated in a phase-locked loop, and it has an intrinsic sensitivity below 20fT/Hz, using a room temperature paraffin-coated cell. We use the magnetometer to monitor magnetic field fluctuations with a sensitivity of 300fT/Hz.

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We describe our approach to atomic magnetometry based on the push-pull optical pumping technique. Cesium vapor is pumped and probed by a resonant laser beam whose circular polarization is modulated synchronously with the spin evolution dynamics induced by a static magnetic field. The magnetometer is operated in a phase-locked loop, and it has an intrinsic sensitivity below 20fT/Hz, using a room temperature paraffin-coated cell. We use the magnetometer to monitor magnetic field fluctuations with a sensitivity of 300fT/Hz.
We describe our approach to atomic magnetometry based on the push-pull optical pumping technique. Cesium vapor is pumped and probed by a resonant laser beam whose circular polarization is modulated synchronously with the spin evolution dynamics induced by a static magnetic field. The magnetometer is operated in a phase-locked loop, and it has an intrinsic sensitivity below 20fT/Hz, using a room temperature paraffin-coated cell. We use the magnetometer to monitor magnetic field fluctuations with a sensitivity of 300fT/Hz.
Recently, atomic magnetometers have been reported as the most sensitive magnetometers by completely eliminating the spin exchange relaxation. In this paper, we described a design of highly sensitive cesium atomic magnetometer based on circular dichroism, which had the advantage of easily locking the probing laser to the necessary frequency compared with those based on circular birefringence. In order to polarize the cesium atoms uniformly, the pumping laser light was separated into two counter-propagating and counter-circular polarization beams through the atomic vapor cell. We employed a circular analyzer optical configuration to measure the ellipticity of the probing light, which indicated the amplitude of the magnetic field. The external magnetic field was tracked by a digital auto frequency tracking system.
Introduction Shortly after the inception of atomic magnetometry, alkali-vapor magnetometers were being used to measure the Earth's magnetic field to unprecedented precision. During the same era, Bell and Bloom first demonstrated all-optical atomic magnetometry through synchronous optical pumping [1] (see Chapters 1 and 6). In this approach, optical-pumping light is frequency- or amplitude-modulated at harmonics of the Larmor frequency ω L to generate a precessing spin polarization within an alkali vapor at finite magnetic field [2, 3]. Although this technique received considerable attention from the atomic physics community for its applicability to optical pumping experiments, Earth's-field alkali-vapor atomic magnetometers continued to rely on radiofrequency (RF) field excitation for several decades (see Chapter 4). Upon the advent of diode lasers addressing alkali and metastable helium transitions, synchronously pumped magnetometers experienced a revival beginning in the late 1980s. In recent years, such magnetometers have found applications in nuclear magnetic resonance detection [4] (see also Chapter 14), quantum control experiments [5], and chip-scale devices intended for spacecraft use [6] (see also Chapters 7 and 15). All-optical magnetometers possess several advantages over devices that employ RF coils. RF-driven magnetometers can suffer from cross-talk if two sensors are placed in close proximity, since the AC magnetic field driving resonance in one vapor cell can adversely affect the other. All-optical magnetometers are free from such interference. When operated in self-oscillating mode [7], RF-driven magnetometers require an added ±90° electronic phase shift in the feedback loop to counter the intrinsic phase shift between the RF field and the probe-beam modulation.
Spin-exchange relaxation free alkali-metal magnetometers typically operate in the regime of high optical density, presenting challenges for simple and efficient optical pumping and detection. We describe a high-sensitivity Rb magnetometer using a single elliptically polarized off-resonant laser beam. Circular component of the light creates relatively uniform spin polarization while the linear component is used to measure optical rotation generated by the atoms. Modulation of the atomic spin direction with an oscillating magnetic field shifts the detected signal to high frequencies. Using a fiber-coupled distributed feedback laser, we achieve magnetic field sensitivity of 7 fT/Hz7\text{ }\text{fT}/\sqrt{\text{Hz}}7 fT/Hz​ with a miniature $5\ifmmode\times\else\texttimes\fi{}5\ifmmode\times\else\texttimes\fi{}5\text{ }\text{mm}\text{ }\text{Rb}$ vapor cell.
We demonstrated a scalar atomic magnetometer using a microfabricated Cs vapor cell. The atomic spin precession is driven by an amplitude-modulated circularly-polarized pump laser resonant on the D1 transition of Cs atoms and detected by an off-resonant linearly-polarized probe laser using a balanced polarimeter setup. Under a magnetic field with amplitude in the Earth's magnetic field range, the magnetometer in the gradiometer mode can reach sensitivities below 150fT/Hz, which shows that the magnetometer by itself can achieve sub-100fT/Hz sensitivities. In addition to its high sensitivity, the magnetometer has a bandwidth close to 1 kHz due to the broad magnetic resonance inside the small vapor cell. Our experiment suggests the feasibility of a portable low-power and high-performance magnetometer which can be operated in the Earth's magnetic field. Such a device will greatly reduce the restrictions on the operating environment and expand the range of applications for atomic magnetometers, such as detection of nuclear magnetic resonance in low magnetic fields.
We report the design and performance of a nonmagnetic drift stable optically pumped cesium magnetometer with a measured sensitivity of 35 fT at 200 s integration time and stability below 50 fT between 70 and 600 s. The sensor is based on the nonlinear magneto-optical rotation effect: in a Bell–Bloom configuration, a higher order polarization moment (alignment) of Cs atoms is created with a pump laser beam in an anti-relaxation coated Pyrex cell under vacuum, filled with Cs vapor at room temperature. The polarization plane of light passing through the cell is modulated due the precession of the atoms in an external magnetic field of 2.1 μT, used to optically determine the Larmor precession frequency. Operation is based on a sequence of optical pumping and observation of freely precessing spins at a repetition rate of 8 Hz. This free precession decay readout scheme separates optical pumping and probing and, thus, ensures a systematically highly clean measurement. Due to the residual offset of the sensor of <15 pT together with negligible crosstalk of adjacent sensors, this device is uniquely suitable for a variety of experiments in low-energy particle physics with extreme precision, here as a highly stable and systematically clean reference probe in search for time-reversal symmetry violating electric dipole moments.