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Comparison of 87Rb N-resonances for D1 and D2 transitions

Novikova, I, Phillips, D F, Taichenachev, A V, Walsworth, R L, Yudin, V I, Alexander S. Zibrov

Published Jan 11, 2006• 17 citations
OpenAlex

Abstract

We report an experimental comparison of three-photon-absorption resonances (known as "N-resonances") for the D_1 and D_2 optical transitions of thermal 87Rb vapor. We find that the D_2 N-resonance has better contrast, a broader linewidth, and a more symmetric lineshape than the D_1 N-resonance. Taken together, these factors imply superior performance for frequency standards operating on alkali D_2 N-resonances, in contrast to coherent population trapping (CPT) resonances for which the D_2 transition provides poorer frequency standard performance than the D_1 transition.

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Optics Letters•Apr 17, 2007•37 citations
We report an experimental comparison of three-photon-absorption resonances (known as "N-resonances") for the D_1 and D_2 optical transitions of thermal 87Rb vapor. We find that the D_2 N-resonance has better contrast, a broader linewidth, and a more symmetric lineshape than the D_1 N-resonance. Taken together, these factors imply superior performance for frequency standards operating on alkali D_2 N-resonances, in contrast to coherent population trapping (CPT) resonances for which the D_2 transition provides poorer frequency standard performance than the D_1 transition.
We report an experimental comparison of three-photon-absorption resonances (N-resonances) for the D1 and D2 optical transitions of thermal (87)Rb vapor. We find that the D2 N-resonance has better contrast, a broader linewidth, and a more symmetric line shape than the D1 N-resonance. Taken together, these factors imply superior performance for frequency standards operating on alkali D2 N-resonances, in contrast with coherent population trapping resonances, for which the D2 transition provides poorer frequency standard performance than the D1 transition.
We have compared coherent population trapping (CPT) resonances, both experimentally and theoretically, for excitation of the D(1) and D(2) transitions of thermal (85)Rb vapor. Excitation of the D(1) line results in greater resonance contrast than excitation of the D(2) line and in a reduction in the resonance width, in agreement with theoretical expectations. These results translate into a nearly tenfold improvement in performance for the application of CPT resonances to a frequency standard or a sensitive magnetometer when the D(1) line, rather than the D(2) line, is used.
We report an experimental study of an all-optical three-photon-absorption resonance (known as an "N-resonance") and discuss its potential application as an alternative to atomic clocks based on coherent population trapping (CPT). We present measurements of the N-resonance contrast, width and light shift for /sup 87/Rb under various conditions including both D/sub 1/ and D/sub 2/ optical transitions. Under conditions such that first-order light shifts cancel, we observe promising short-term frequency stability (/spl sim/ 1.5 /spl times/ 10/sup -11/ /spl tau//sub - 1/2 /) for an N-resonance on the Di transition of /sup 87/ Rb vapor.
We have measured the spectral position of the absorption minimum in a coherent population trapping resonance in thermal cesium vapor as a function of light intensity. The dependence of position on intensity is found to be almost linear. We have furthermore studied the dependence of this light shift on neon bufier gas pressure and flnd a strong reduction for higher pressures. So the addition of a bufier gas not only reduces the linewidth of the resonance but also a very important systematic efiect for precision measurements. An atomic three-level system with two low-lying and long-lived levels (a so-called ⁄ system) can exhibit a two-photon resonance when the difierence frequency of two driving flelds matches the splitting of the two lower levels (flg. 1), !2 i !1 = !12 (1). The resonance is called \dark since one-photon absorption and resonance ∞uorescence are strongly reduced because of the trapping of the atomic population in a coherent superposition state of the two lower levels that is no longer coupled to the light flelds (coherent population trapping, CPT) (2). The two-photon resonance can be very narrow (3, 4), with linewidths rivaling those of the microwave-driven magnetic dipole transition between the two lower atomic states. The use of dark resonances for the construction of atomic radio frequency standards (5) or applications for precision measurements, for instance in magnetometry (6), has been suggested, and flrst steps in this direction have been taken (7). It is an essential requirement for such precision applications to understand the in∞uence of experimental conditions on the position and shape of the resonance under investigation. Because of the flnite dephasing rate between the two lower states the position of the absorption minimum at the dark resonance can depend on intensity (8,1), and in experiments a shift of the center of the resonance (light shift, AC Stark shift) is readily observed (9), as was discussed, for instance, for an atomic beam (5) or in connection with a CPT maser (10). In this letter we report measurements of the light shift of the two-photon resonance that couples two hyperflne ground-state levels of the cesium atoms in a thermal vapor both with and without an additional bufier gas.