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Annals of Physics

Generation of multimode quantum correlation with energy-level cascaded four-wave mixing processes

Jiawei Li, Wei Li, Mengqi Niu, Yixing Lin, Changbiao Li, Yin Cai, Yanpeng Zhang

Published Oct 15, 2020• 13 citations
Publisher
DOI
10.1016/j.aop.2020.168316

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The nonlinear parametric process is of great significance for achieving high-quality coherent optical signals and quantum correlated photons. With the development of classical and quantum information processing, the study of the properties of parametric processes is evolving in complex scenarios of multimode, which is limited in conventional nonlinear media due to strict phase matching, e.g. nonlinear crystals. Here we study the dressing-energy-level-cascaded four-wave mixing process to generate multimode optical parametric signals. Via cascading double-Λ type configuration of 85 Rb D 1 line, the non-degenerate energy-level-cascaded FWM is constructed to generate multimode self-parametric amplification. Moreover, with the dressing effects based on atomic coherence, the spatial and frequency multimode characteristics of energy-level-cascaded FWM parametric amplification, i.e., the modes number and pattern, are actively modulated by the pump fields detuning. Also, the spatial modes from the coupling of two coexisting spontaneous parametric FWMs can be controlled to reach tremendous scalability via the atomic coherence and Kerr non-linearity. The atomic coherence effects and unique phase-matching symmetry nature allow flexible modulation of the multimode property of the generated parametric signals within a nonlinear device, which paves a way for multimode classical and quantum information processing.
Quantum Squeezing is one of the most important quantum resources in quantum optics and quantum information. In particular, multimode quantum squeezing, with ultra-low quantum fluctuations and quantum correlations amongst many optical modes, is essential for realizing multipartite entanglement and quantum precision measurements. In this paper, we propose an all-optically controlled scheme to generate three-mode bright quantum correlated beams from energy-level cascaded four-wave mixing (ELC-FWM). By using a linear modes transform approach, the input-output relation and the covariance matrix of the produced states are obtained. Moreover, single-, double- and triple-seeding conditions are investigated to measure the quantum squeezing properties. We find that various permutations of two- and three-mode quadrature squeezing can be generated and optimized to reach the corresponding limit, via only modulating the ratio of the multiple seeds, without need of any post-operating linear optics, e.g., beam splitters. Such weak seeding light controlled scheme suggests the modulation and the optimization of multimode quantum states might be operated at photons-level, providing a reconfigurable and integrated strategy for complex quantum information processing and quantum metrology.
Multimode quantum states, such as multipartite quantum entanglement or quantum correlations, are important for both fundamental science and the future development of quantum technologies. Here we theoretically propose and experimentally realize a scheme that can fully exploit the multi-spatial-mode nature of the four-wave-mixing (FWM) process, i.e., spatial multiplexing, and thus integrates multiple FWM processes into a single cell at each stage of the cascaded process. The number of generated quantum-correlated beams 2n{2}^{n}2n is exponentially dependent on the number of vapor cells nnn. In addition, the quantum correlations between the multiple beams also increase as the number of vapor cell increases. For the case of n=2n=2n=2, we experimentally show that the degree of intensity-difference squeezing between the four quantum-correlated beams in our scheme is enhanced to $\ensuremath{-}8.2\ifmmode\pm\else\textpm\fi{}0.2$ dB from $\ensuremath{-}5.6\ifmmode\pm\else\textpm\fi{}0.3$ and $\ensuremath{-}6.5\ifmmode\pm\else\textpm\fi{}0.2$ dB of squeezing obtained with a single FWM process. Our system may find applications in quantum information and precision measurement.