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Superinductance and fluctuating two-level systems: Loss and noise in disordered and non-disordered superconducting quantum devices

David Niepce

Published Jan 1, 2020• 2 citations
OpenAlex

Abstract

In this thesis, we first demonstrate that a disordered superconductor with high kinetic inductance can realise a microwave low-loss, non-dissipative circuit element with impedance greater than the quantum resistance. This element, known as a superinductor, can suppress the fluctuations of charge in a quantum circuit.For this purpose, we fabricated and characterised 20 nm thick, 40 nm wide niobium-nitride nanowires and determined the impedance to 6.795 kΩ. We demonstrate internal quality factors Qi = 2.5e4 in nanowire resonators at single photon excitation, which is significantly higher than values reported in devices with similar materials and geometries. Moreover, we show that the dominant dissipation in our nanowires is not an intrinsic property of the disordered films, but can instead be fully understood within the framework of two-level systems.To further characterise these losses, we then explore the geometrical scaling, toward nanowire dimensions, of dielectric losses in superconducting microwave resonators fabricated with the same techniques and from the same NbN thin-film as the nanowire superinductors. For this purpose, we perform an experimental and numerical study of dielectric loss at low temperatures. Using 3D finite-element simulation of the Maxwell--London equations, we compute the geometric filling factors of the lossy regions in our resonator structures and fit the experimental data to determine the intrinsic loss tangents of its interfaces and dielectrics. Finally, we study the effect of two-level systems on the performance of various superconducting quantum circuits. For this purpose, we measure coherence-time fluctuations in qubits and frequency fluctuations in resonators. In all devices, through statistical analysis, we identify the signature of individual Lorentzian fluctuators in the noise. We find that fluctuations in qubit relaxation are local to the qubit and are caused by instabilities of near-resonant two-level-systems. Furthermore, when examining the low-frequency noise of three different types of superconducting resonator - one NbN nanowire, one Al coplanar waveguide, and one Al 3D cavity - we observe a similar power-law dependence of the Lorentzian switching time and amplitude on the circulating power in the resonators, suggesting a common noise mechanism in the three different types of devices.

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Geometric scaling of two-level-system loss in superconducting resonators

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Abstract We perform an experimental and numerical study of dielectric loss in superconducting microwave resonators at low temperature. Dielectric loss, due to two-level systems, is a limiting factor in several applications, e.g. superconducting qubits, Josephson parametric amplifiers, microwave kinetic-inductance detectors, and superconducting single-photon detectors. Our devices are made of disordered NbN, which, due to magnetic-field penetration, necessitates 3D finite-element simulation of the Maxwell–London equations at microwave frequencies to accurately model the current density and electric field distribution. From the field distribution, we compute the geometric filling factors of the lossy regions in our resonator structures and fit the experimental data to determine the intrinsic loss tangents of its interfaces and dielectrics. We put emphasis on the loss caused by a spin-on-glass resist such as hydrogen silsesquioxane (HSQ), used for ultrahigh lithographic resolution relevant to the fabrication of nanowires. We find that, when used, HSQ is the dominant source of loss, with a loss tangent of δ HSQ i = 8 × 10 − 3 .

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Wenyuan Zhang

Superinductors are inductors whose microwave characteristic impedances are greater than the resistance quantum, $R_{Q}=h/(2e)^{2}approx6.5kOmega$. They can be implemented using Josephson junction chains and high kinetic inductance nanowires. In this dissertation, we explore applications of superinductors in both implementations in superconducting quantum circuits. The dissertation consists of three parts. In the first part, we discuss the fluxon-parity-protected qubit consisting of a Cooper-pair box (CPB) shunted by a superinductor made of a chain of coupled asymmetric Superconducting Quantum Interference Devices (CASQUIDs). The spectroscopic measurement of a prototype of the fluxon-parity-protected qubit was performed. We observed almost complete suppression of the single fluxon tunneling across the CPB due to the destructive Aharonov-Casher interference when the offset charge on the CPB island was set to $e$ mod(2$e$). A fluxon-parity-protected qubit with a higher superinductance can potentially be used to perform fault-tolerant Clifford gates. In the second part, we studied the microwave losses in high-kinetic-inductance granular Aluminum films using superconducting coplanar-waveguide (CPW) resonators made of the films. We observed that the intrinsic losses in these resonators at low temperatures were limited by resonator coupling to the two-level systems (TLS) in the environment. The demonstrated internal quality factors are comparable with those for CPW resonators made of conventional superconductors. The characterized granular Aluminum films can be used to fabricate superinductors for a wide range of applications in quantum metrology and quantum information processing. In the third part, we discuss the one-dimensional Josephson metamaterial made of a similar structure as the superinductor used in the fluxon-parity-protected qubit. The metamaterial demonstrated strong Kerr nonlinearity with the Kerr constant tunable over a wide range from positive to negative values by the magnetic field. The metamaterial is promising for use as an active medium for quantum-limited Josephson traveling-wave parametric amplifiers.

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Frequency instability of superconducting resonators and qubits leads to dephasing and time-varying energy loss and hinders quantum processor tune-up. Its main source is dielectric noise originating in surface oxides. Thorough noise studies are needed to develop a comprehensive understanding and mitigation strategy of these fluctuations. We use a frequency-locked loop to track the resonant frequency jitter of three different resonator types—one niobium nitride superinductor, one aluminum coplanar waveguide, and one aluminum cavity—and we observe notably similar random telegraph signal fluctuations. At low microwave drive power, the resonators exhibit multiple, unstable frequency positions, which, for increasing power, coalesce into one frequency due to motional narrowing caused by sympathetic driving of two-level system defects by the resonator. In all three devices, we identify a dominant fluctuator whose switching amplitude (separation between states) saturates with increasing drive power, but whose characteristic switching rate follows the power law dependence of quasi-classical Landau-Zener transitions.

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ISTA Thesis

Andrea Trioni

Quantum mechanics reveals a world that defies classical determinism, where uncertainty, superposition, and fluctuations are fundamental aspects. Engineering devices that harness these quantum features requires not only precision, but also a deep understanding of how they interact with their surrounding environment. Superconducting circuits, which exploit macroscopic quantum coherence in low-loss superconducting materials, provide a scalable platform for implementing such systems. Among the critical elements in these circuits, superinductors—high-impedance, dissipation-free inductive components—play a central role by suppressing charge fluctuations. They allow quantum states to be delocalized in phase space, protect qubits from environmental noise, and facilitate access to phenomena such as dual Josephson physics and ultra-strong coupling regimes. This thesis explores two complementary implementations of high-impedance circuits: geometric superinductors, demonstrating that high impedance can be achieved beyond kinetic inductance, and Josephson junction chains, used to investigate both microwave mode properties and DC transport across the superconductor-to-insulator transition. Part I addresses geometric superinductors. Contrary to the common belief that high-impedance superconducting circuits require kinetic inductance, we demonstrate that purely geometric designs can achieve characteristic impedance exceeding the resistance quantum. By exploiting mutual coupling between adjacent turns, coil-based inductors achieve enhanced self-inductance, creating a reliable platform for qubits and resonators. Modeling, simulation, fabrication, and characterization confirm that these elements behave as superinductor. With low loss, high linearity, and minimal stray capacitance, these elements are reproducible, free of uncontrolled tunneling events, and capable of strong magnetic coupling. This establishes geometric superinductors as robust, single-wave-function superconducting devices suitable for hardware protected qubits and hybrid systems. Part II presents classical numerical simulations of a Quantum Phase Slip circuit to study dual Shapiro steps. The circuit consists of an ideal Quantum Phase Slip element embedded in a resistive-inductive environment with a parasitic capacitance. Part III extends the investigation of high characteristic-impedance circuit elements to one-dimensional Josephson junction chains, which act as a quantum simulator for many-body physics and the superconductor–insulator transition. Different devices are realized on both sides of the DC phase transition, showing either a supercurrent branch or Coulomb blockade at zero bias. The effect of the crossover on microwave modes, however, remains insufficiently investigated. Studying these modes provides insight into the interplay between disorder and phase-slip events. Small differences in circuit component sizes determine which side of the transition a device falls on, making these results relevant not only for fundamental understanding but also for the design of quantum devices, emphasizing the crucial role of the electromagnetic environment in stabilizing and controlling fragile quantum states. Together, these results illustrate how carefully engineered high characteristic-impedance elements provide a link between macroscopic circuits and the inherently uncertain quantum world, enabling experiments that probe, control, and ultimately exploit quantum fluctuations for applications in quantum information, metrology, solid state physics and beyond.

•Jan 1, 2025•0 citations
In this thesis, we first demonstrate that a disordered superconductor with high kinetic inductance can realise a microwave low-loss, non-dissipative circuit element with impedance greater than the quantum resistance. This element, known as a superinductor, can suppress the fluctuations of charge in a quantum circuit.For this purpose, we fabricated and characterised 20 nm thick, 40 nm wide niobium-nitride nanowires and determined the impedance to 6.795 kΩ. We demonstrate internal quality factors Qi = 2.5e4 in nanowire resonators at single photon excitation, which is significantly higher than values reported in devices with similar materials and geometries. Moreover, we show that the dominant dissipation in our nanowires is not an intrinsic property of the disordered films, but can instead be fully understood within the framework of two-level systems.To further characterise these losses, we then explore the geometrical scaling, toward nanowire dimensions, of dielectric losses in superconducting microwave resonators fabricated with the same techniques and from the same NbN thin-film as the nanowire superinductors. For this purpose, we perform an experimental and numerical study of dielectric loss at low temperatures. Using 3D finite-element simulation of the Maxwell--London equations, we compute the geometric filling factors of the lossy regions in our resonator structures and fit the experimental data to determine the intrinsic loss tangents of its interfaces and dielectrics. Finally, we study the effect of two-level systems on the performance of various superconducting quantum circuits. For this purpose, we measure coherence-time fluctuations in qubits and frequency fluctuations in resonators. In all devices, through statistical analysis, we identify the signature of individual Lorentzian fluctuators in the noise. We find that fluctuations in qubit relaxation are local to the qubit and are caused by instabilities of near-resonant two-level-systems. Furthermore, when examining the low-frequency noise of three different types of superconducting resonator - one NbN nanowire, one Al coplanar waveguide, and one Al 3D cavity - we observe a similar power-law dependence of the Lorentzian switching time and amplitude on the circulating power in the resonators, suggesting a common noise mechanism in the three different types of devices.
Abstract We perform an experimental and numerical study of dielectric loss in superconducting microwave resonators at low temperature. Dielectric loss, due to two-level systems, is a limiting factor in several applications, e.g. superconducting qubits, Josephson parametric amplifiers, microwave kinetic-inductance detectors, and superconducting single-photon detectors. Our devices are made of disordered NbN, which, due to magnetic-field penetration, necessitates 3D finite-element simulation of the Maxwell–London equations at microwave frequencies to accurately model the current density and electric field distribution. From the field distribution, we compute the geometric filling factors of the lossy regions in our resonator structures and fit the experimental data to determine the intrinsic loss tangents of its interfaces and dielectrics. We put emphasis on the loss caused by a spin-on-glass resist such as hydrogen silsesquioxane (HSQ), used for ultrahigh lithographic resolution relevant to the fabrication of nanowires. We find that, when used, HSQ is the dominant source of loss, with a loss tangent of δ HSQ i = 8 × 10 − 3 .
Superinductors are inductors whose microwave characteristic impedances are greater than the resistance quantum, RQ=h/(2e)2approx6.5kOmegaR_{Q}=h/(2e)^{2}approx6.5kOmegaRQ​=h/(2e)2approx6.5kOmega. They can be implemented using Josephson junction chains and high kinetic inductance nanowires. In this dissertation, we explore applications of superinductors in both implementations in superconducting quantum circuits. The dissertation consists of three parts. In the first part, we discuss the fluxon-parity-protected qubit consisting of a Cooper-pair box (CPB) shunted by a superinductor made of a chain of coupled asymmetric Superconducting Quantum Interference Devices (CASQUIDs). The spectroscopic measurement of a prototype of the fluxon-parity-protected qubit was performed. We observed almost complete suppression of the single fluxon tunneling across the CPB due to the destructive Aharonov-Casher interference when the offset charge on the CPB island was set to eee mod(2eee). A fluxon-parity-protected qubit with a higher superinductance can potentially be used to perform fault-tolerant Clifford gates. In the second part, we studied the microwave losses in high-kinetic-inductance granular Aluminum films using superconducting coplanar-waveguide (CPW) resonators made of the films. We observed that the intrinsic losses in these resonators at low temperatures were limited by resonator coupling to the two-level systems (TLS) in the environment. The demonstrated internal quality factors are comparable with those for CPW resonators made of conventional superconductors. The characterized granular Aluminum films can be used to fabricate superinductors for a wide range of applications in quantum metrology and quantum information processing. In the third part, we discuss the one-dimensional Josephson metamaterial made of a similar structure as the superinductor used in the fluxon-parity-protected qubit. The metamaterial demonstrated strong Kerr nonlinearity with the Kerr constant tunable over a wide range from positive to negative values by the magnetic field. The metamaterial is promising for use as an active medium for quantum-limited Josephson traveling-wave parametric amplifiers.
Disordered superconducting materials with high kinetic inductance are an important resource for generating nonlinearity in quantum circuits and creating high-impedance environments. In thin films fabricated from these materials, the combination of disorder and low effective dimensionality leads to increased order parameter fluctuations and enhanced kinetic inductance values. Among the challenges of harnessing these compounds in coherent devices are their proximity to the superconductor-insulator phase transition and the two-level systems located in the disordered structure. Here, we fabricate tungsten silicide wires from quasi-two-dimensional films and embed them into microwave resonators and fluxonium qubits, where the kinetic inductance provides the inductive part of the circuits. In this work, we study the dependence of loss on the frequency, disorder, and geometry of the devices, and find that the loss increases with the level of disorder and is dominated by the localized quasiparticles trapped in the spatial variations of the superconducting gap. High kinetic inductance materials are widely used in superconducting circuits, yet their loss mechanisms are not fully understood. Here the authors study quantum circuits incorporating nanowires made of quasi-2D disordered superconductor WSi and identify localized quasiparticles as the dominant source of loss.
Frequency instability of superconducting resonators and qubits leads to dephasing and time-varying energy loss and hinders quantum processor tune-up. Its main source is dielectric noise originating in surface oxides. Thorough noise studies are needed to develop a comprehensive understanding and mitigation strategy of these fluctuations. We use a frequency-locked loop to track the resonant frequency jitter of three different resonator types—one niobium nitride superinductor, one aluminum coplanar waveguide, and one aluminum cavity—and we observe notably similar random telegraph signal fluctuations. At low microwave drive power, the resonators exhibit multiple, unstable frequency positions, which, for increasing power, coalesce into one frequency due to motional narrowing caused by sympathetic driving of two-level system defects by the resonator. In all three devices, we identify a dominant fluctuator whose switching amplitude (separation between states) saturates with increasing drive power, but whose characteristic switching rate follows the power law dependence of quasi-classical Landau-Zener transitions.
Quantum decoherence due to charge fluctuations is still a problem in many device architectures for quantum computing or metrology, but it can be suppressed by shunting the circuit with a high microwave impedance, known as a $s\phantom{\rule{0}{0ex}}u\phantom{\rule{0}{0ex}}p\phantom{\rule{0}{0ex}}e\phantom{\rule{0}{0ex}}r\phantom{\rule{0}{0ex}}i\phantom{\rule{0}{0ex}}n\phantom{\rule{0}{0ex}}d\phantom{\rule{0}{0ex}}u\phantom{\rule{0}{0ex}}c\phantom{\rule{0}{0ex}}t\phantom{\rule{0}{0ex}}a\phantom{\rule{0}{0ex}}n\phantom{\rule{0}{0ex}}c\phantom{\rule{0}{0ex}}e$. This study uses the kinetic inductance of a nanowire of disordered superconductor to demonstrate a low-loss, small-capacitance superinductor, in a simpler approach than the traditionally used Josephson-junction arrays. Such nanowire superinductors should have an impact on engineering long-lived superconducting qubits, and quantum-coherent experiments with mesoscopic systems.
Quantum mechanics reveals a world that defies classical determinism, where uncertainty, superposition, and fluctuations are fundamental aspects. Engineering devices that harness these quantum features requires not only precision, but also a deep understanding of how they interact with their surrounding environment. Superconducting circuits, which exploit macroscopic quantum coherence in low-loss superconducting materials, provide a scalable platform for implementing such systems. Among the critical elements in these circuits, superinductors—high-impedance, dissipation-free inductive components—play a central role by suppressing charge fluctuations. They allow quantum states to be delocalized in phase space, protect qubits from environmental noise, and facilitate access to phenomena such as dual Josephson physics and ultra-strong coupling regimes. This thesis explores two complementary implementations of high-impedance circuits: geometric superinductors, demonstrating that high impedance can be achieved beyond kinetic inductance, and Josephson junction chains, used to investigate both microwave mode properties and DC transport across the superconductor-to-insulator transition. Part I addresses geometric superinductors. Contrary to the common belief that high-impedance superconducting circuits require kinetic inductance, we demonstrate that purely geometric designs can achieve characteristic impedance exceeding the resistance quantum. By exploiting mutual coupling between adjacent turns, coil-based inductors achieve enhanced self-inductance, creating a reliable platform for qubits and resonators. Modeling, simulation, fabrication, and characterization confirm that these elements behave as superinductor. With low loss, high linearity, and minimal stray capacitance, these elements are reproducible, free of uncontrolled tunneling events, and capable of strong magnetic coupling. This establishes geometric superinductors as robust, single-wave-function superconducting devices suitable for hardware protected qubits and hybrid systems. Part II presents classical numerical simulations of a Quantum Phase Slip circuit to study dual Shapiro steps. The circuit consists of an ideal Quantum Phase Slip element embedded in a resistive-inductive environment with a parasitic capacitance. Part III extends the investigation of high characteristic-impedance circuit elements to one-dimensional Josephson junction chains, which act as a quantum simulator for many-body physics and the superconductor–insulator transition. Different devices are realized on both sides of the DC phase transition, showing either a supercurrent branch or Coulomb blockade at zero bias. The effect of the crossover on microwave modes, however, remains insufficiently investigated. Studying these modes provides insight into the interplay between disorder and phase-slip events. Small differences in circuit component sizes determine which side of the transition a device falls on, making these results relevant not only for fundamental understanding but also for the design of quantum devices, emphasizing the crucial role of the electromagnetic environment in stabilizing and controlling fragile quantum states. Together, these results illustrate how carefully engineered high characteristic-impedance elements provide a link between macroscopic circuits and the inherently uncertain quantum world, enabling experiments that probe, control, and ultimately exploit quantum fluctuations for applications in quantum information, metrology, solid state physics and beyond.