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arXiv:2412.05482 · Applied Physics Letters

Loss tangent fluctuations due to two-level systems in superconducting microwave resonators

André Vallières, Megan E. Russell, Xinyuan You, David A. Garcia Wetten, Dominic P. Goronzy, Mitchell J. Walker, Michael J. Bedzyk, Mark C. Hersam, Alexander Romanenko, Yao Lu, Anna Grassellino, Jens Koch, Corey Rae McRae

Published Mar 1, 2025• 8 citations
arXivHTMLPDF

Abstract

Superconducting microwave resonators are critical to quantum computing and sensing technologies. Additionally, they are common proxies for superconducting qubits when determining the effects of performance-limiting loss mechanisms such as from two-level systems (TLSs). The extraction of these loss mechanisms is often performed by measuring the internal quality factor Qi as a function of power or temperature. In this work, we investigate large temporal fluctuations of Qi at low powers over periods of 12–16 h (relative standard deviation σQi/Qi=13%). These fluctuations are ubiquitous across multiple resonators, chips, and cooldowns. We are able to attribute these fluctuations to variations in the TLS loss tangent due to two main indicators. First, measured fluctuations decrease as power and temperature increase. Second, for interleaved measurements, we observe correlations between low- and medium-power Qi fluctuations and an absence of correlations with high-power fluctuations. Agreement with the TLS loss tangent mean is obtained by performing measurements over a time span of a few hours. We hypothesize that, in addition to decoherence, due to coupling to individual near-resonant TLS, superconducting qubits are affected by these observed TLS loss tangent fluctuations.

DOI
10.1063/5.0253375

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Superconducting microwave resonators are critical to quantum computing and sensing technologies. Additionally, they are common proxies for superconducting qubits when determining the effects of performance-limiting loss mechanisms such as from two-level systems (TLSs). The extraction of these loss mechanisms is often performed by measuring the internal quality factor Qi as a function of power or temperature. In this work, we investigate large temporal fluctuations of Qi at low powers over periods of 12–16 h (relative standard deviation σQi/Qi=13%). These fluctuations are ubiquitous across multiple resonators, chips, and cooldowns. We are able to attribute these fluctuations to variations in the TLS loss tangent due to two main indicators. First, measured fluctuations decrease as power and temperature increase. Second, for interleaved measurements, we observe correlations between low- and medium-power Qi fluctuations and an absence of correlations with high-power fluctuations. Agreement with the TLS loss tangent mean is obtained by performing measurements over a time span of a few hours. We hypothesize that, in addition to decoherence, due to coupling to individual near-resonant TLS, superconducting qubits are affected by these observed TLS loss tangent fluctuations.
High quality factor, i.e. low loss, microwave resonators are important for quantum information storage and addressing. In this work we study the resonance frequency and loss in superconducting coplanar waveguide resonators as a function of power and temperature. We find that there is increased loss at low power and low temperature. The increased loss is attributed to the existence of two-level systems (TLS) at the surfaces, interfaces, and in the bulk of insulators deposited on the structures. We show that both the temperature dependence of the resonant frequency and the power dependence of the loss can be used to find the TLS contribution to the loss. The TLS intrinsic loss tangent derived from the frequency shift data at high power is shown to agree well with the direct loss measurement at low power. The former allows for a relatively fast measurement of the TLS loss. As an example, we measure the properties of amorphous AlOXdeposited on the resonators and find a TLS loss tangent of 1 × 10-3.
Superconducting quantum computing is experiencing a tremendous growth. Although major milestones have already been achieved, useful quantum-computing applications are hindered by a variety of decoherence phenomena. Decoherence due to two-level systems (TLSs) hosted by amorphous dielectric materials is ubiquitous in planar superconducting devices. We use high-quality quasilumped-element resonators as quantum sensors to investigate TLS-induced loss and noise. We perform two-tone experiments with a probe and pump electric fields; the pump is applied at different power levels and detunings. We measure and analyze time series of the quality factor and resonance frequency for very long time periods, up to 1000 h. We additionally carry out simulations based on the TLS interacting model in the presence of a pump field. We find that loss and noise are reduced at medium and high power, matching the simulations, but not at low power.
Superconducting resonators are widely used in many applications such as qubit readout for quantum computing applications, and kinetic inductance detectors. These resonators are susceptible to numerous loss and noise mechanisms under microwave excitation, especially the dissipation due to non-equilibrium quasi-particles and two-level systems (TLS), which can result in a decrease of the superconducting intrinsic quality factor (QiQ_iQi​) in high quality superconducting resonators. Particularly in the few-photon and low temperature (T) regime, TLS losses can become a dominant loss mechanism. In this study, novel aluminum half-wavelength resonators are investigated, focusing on the loss properties at extra-low power and low temperature. An unusual increase of Qi(T)Q_i(T)Qi​(T) with deceasing temperature is observed. This behavior is attributed to the increase of TLS coherence time (T2T_2T2​) at ultra-low temperatures and powers. This T2T_2T2​ increase is consistent with other work on resonant frequency noise in resonators and measurements of individual TLS, and likely arises from interacting TLS in the aluminum half-wavelength resonators.
Superconducting qubits are a leading system for realizing large-scale quantum processors, but overall gate fidelities suffer from coherence times limited by microwave dielectric loss.Recently discovered tantalum-based qubits exhibit record lifetimes exceeding 0.3 ms.Here, we perform systematic, detailed measurements of superconducting tantalum resonators in order to disentangle sources of loss that limit state-of-the-art tantalum devices.By studying the dependence of loss on temperature, microwave photon number, and device geometry, we quantify materials-related losses and observe that the losses are dominated by several types of saturable two-level systems (TLSs), with evidence that both surface and bulk related TLSs contribute to loss.Moreover, we show that surface TLSs can be altered with chemical processing.With four different surface conditions, we quantitatively extract the linear absorption associated with different surface TLS sources.Finally, we quantify the impact of the chemical processing at singlephoton powers, the relevant conditions for qubit device performance.In this regime, we measure resonators with internal quality factors ranging from 5 to 15 × 10 6 , comparable to the best qubits reported.In these devices, the surface and bulk TLS contributions to loss are comparable, showing that systematic improvements in materials on both fronts are necessary to improve qubit coherence further.
In this thesis, we first demonstrate that a disordered superconductor with high kinetic inductance can realise a microwave low-loss, non-dissipative circuit element with impedance greater than the quantum resistance. This element, known as a superinductor, can suppress the fluctuations of charge in a quantum circuit.For this purpose, we fabricated and characterised 20 nm thick, 40 nm wide niobium-nitride nanowires and determined the impedance to 6.795 kΩ. We demonstrate internal quality factors Qi = 2.5e4 in nanowire resonators at single photon excitation, which is significantly higher than values reported in devices with similar materials and geometries. Moreover, we show that the dominant dissipation in our nanowires is not an intrinsic property of the disordered films, but can instead be fully understood within the framework of two-level systems.To further characterise these losses, we then explore the geometrical scaling, toward nanowire dimensions, of dielectric losses in superconducting microwave resonators fabricated with the same techniques and from the same NbN thin-film as the nanowire superinductors. For this purpose, we perform an experimental and numerical study of dielectric loss at low temperatures. Using 3D finite-element simulation of the Maxwell--London equations, we compute the geometric filling factors of the lossy regions in our resonator structures and fit the experimental data to determine the intrinsic loss tangents of its interfaces and dielectrics. Finally, we study the effect of two-level systems on the performance of various superconducting quantum circuits. For this purpose, we measure coherence-time fluctuations in qubits and frequency fluctuations in resonators. In all devices, through statistical analysis, we identify the signature of individual Lorentzian fluctuators in the noise. We find that fluctuations in qubit relaxation are local to the qubit and are caused by instabilities of near-resonant two-level-systems. Furthermore, when examining the low-frequency noise of three different types of superconducting resonator - one NbN nanowire, one Al coplanar waveguide, and one Al 3D cavity - we observe a similar power-law dependence of the Lorentzian switching time and amplitude on the circulating power in the resonators, suggesting a common noise mechanism in the three different types of devices.
The performance of superconducting circuits for quantum computing is limited by materials losses. In particular, coherence times are typically bounded by two-level system (TLS) losses at single photon powers and millikelvin temperatures. The identification of low loss fabrication techniques, materials, and thin film dielectrics is critical to achieving scalable architectures for superconducting quantum computing. Superconducting microwave resonators provide a convenient qubit proxy for assessing performance and studying TLS loss and other mechanisms relevant to superconducting circuits such as non-equilibrium quasiparticles and magnetic flux vortices. In this review article, we provide an overview of considerations for designing accurate resonator experiments to characterize loss, including applicable types of losses, cryogenic setup, device design, and methods for extracting material and interface losses, summarizing techniques that have been evolving for over two decades. Results from measurements of a wide variety of materials and processes are also summarized. Finally, we present recommendations for the reporting of loss data from superconducting microwave resonators to facilitate materials comparisons across the field.