One of the distinguishing achievements of physics has been the ability to describe the Universe based upon underlying microscopic principles. When there are many participating objects being governed by these microscopic principles, the resultant behavior often harbors emergent collective phenomena that may not be obviously related to the microscopic description. Phase transitions, quantum or classical, are a canonical example of such many-body phenomena that are understood in equilibrium through a framework of thermodynamic constraints, statistical ensembles, and a growth of system-wide correlations at the transition. However, a new class of quantum phase transitions has recently emerged for non-equilibrium systems with behavior that is not captured by this traditional framework. In the case of isolated quantum systems, these transitions occur among excited eigenstates and requires knowledge of the structure of these individual eigenstates in the quantum system. Understanding what drives such a phase transition requires a deeper microscopic knowledge of the role of correlations at the transition. \nThe use of ultracold atoms in optical lattices has paved the way for faithfully realizing quantum phase transitions. In particular, the advent of the quantum gas microscope realized an experimental platform that is highly controllable and provides microscopic access to the many-bodied wave functions. All experiments presented in this thesis use such a quantum gas microscope architecture where a quantum degenerate gas of Rb is used to probe the behavior of non-equilibrium quantum systems in one spatial dimension.\nThis thesis briefly discusses some studies of entanglement in equilibrium quantum phase transitions near the ground state of the system. In the first experiment, we directly measure the second-order R\\'enyi entanglement entropy that develops as a Bose-Hubbard system transitions from a Mott insulator to a superfluid. This is followed by a study of entanglement growth at the transition in the transverse Ising model. \nThese studies progress to the investigation of two particular non-equilibrium quantum phases and their transition into one another: quantum thermalization and many-body localization. We investigate the development of entanglement entropy that mimics thermodynamic entropy for an isolated quantum system which locally thermalizes under its own unitary dynamics. We then investigate the only known robust exception to this thermalizing behavior by studying the onset of many-body localization due to disorder. We observe the breakdown of thermalization in this phase and the logarithmically slow growth of entanglement throughout the system, which identifies the localized system to be an interacting one. Lastly, we investigate the role of correlations in the critical dynamics that emerge at high-orders where the system transitions from thermalizing behavior to many-body localization.
One of the distinguishing achievements of physics has been the ability to describe the Universe based upon underlying microscopic principles. When there are many participating objects being governed by these microscopic principles, the resultant behavior often harbors emergent collective phenomena that may not be obviously related to the microscopic description. Phase transitions, quantum or classical, are a canonical example of such many-body phenomena that are understood in equilibrium through a framework of thermodynamic constraints, statistical ensembles, and a growth of system-wide correlations at the transition. However, a new class of quantum phase transitions has recently emerged for non-equilibrium systems with behavior that is not captured by this traditional framework. In the case of isolated quantum systems, these transitions occur among excited eigenstates and requires knowledge of the structure of these individual eigenstates in the quantum system. Understanding what drives such a phase transition requires a deeper microscopic knowledge of the role of correlations at the transition. \nThe use of ultracold atoms in optical lattices has paved the way for faithfully realizing quantum phase transitions. In particular, the advent of the quantum gas microscope realized an experimental platform that is highly controllable and provides microscopic access to the many-bodied wave functions. All experiments presented in this thesis use such a quantum gas microscope architecture where a quantum degenerate gas of Rb is used to probe the behavior of non-equilibrium quantum systems in one spatial dimension.\nThis thesis briefly discusses some studies of entanglement in equilibrium quantum phase transitions near the ground state of the system. In the first experiment, we directly measure the second-order R\'enyi entanglement entropy that develops as a Bose-Hubbard system transitions from a Mott insulator to a superfluid. This is followed by a study of entanglement growth at the transition in the transverse Ising model. \nThese studies progress to the investigation of two particular non-equilibrium quantum phases and their transition into one another: quantum thermalization and many-body localization. We investigate the development of entanglement entropy that mimics thermodynamic entropy for an isolated quantum system which locally thermalizes under its own unitary dynamics. We then investigate the only known robust exception to this thermalizing behavior by studying the onset of many-body localization due to disorder. We observe the breakdown of thermalization in this phase and the logarithmically slow growth of entanglement throughout the system, which identifies the localized system to be an interacting one. Lastly, we investigate the role of correlations in the critical dynamics that emerge at high-orders where the system transitions from thermalizing behavior to many-body localization.
A system of ultracold atoms in an optical lattice provides a powerful platform for quantum simulation. In our laboratory, we use a quantum gas microscope to tune lattice parameters not only in a global scale but also at the level of individual sites. This allows us to control and detect the quantum state of interacting many-body systems as well as to engineer a broad class of Hamiltonians with high fidelity. Leveraging this versatility, we can realize several types of strongly correlated bosonic systems, which present intriguing behaviors and implement novel phases of matter. Analyzing snapshots of the atomic distribution with single-site resolution, we measure correlations and entanglement within these systems to reveal their main features, including non-equilibrium dynamics and quantum phase transitions. In this thesis, I present the works performed by our team for four different types of systems. First of all, I briefly introduce the behavior of a 1D disordered system in the critical regime between the thermal and the many-body-localized phases. In particular, we discuss what happens when a disordered and a non-disordered region are coupled via a single site. We find evidence for accelerated transport of thermal inclusion into the localized region, which shows the existence of a quantum avalanche, i.e. thermalization via accelerated transport throughout the localized system. In the second part, we realize a fractional quantum Hall state using an artificial gauge field, by implementing an adiabatic preparation protocol. We identify a topological phase transition in our system and characterize several key physical features expected for a Laughlin state by measuring density correlations and Hall conductivity. The next topic of this thesis relates to quantum magnetism. Mapping nearest hopping in a tilted optical lattice to spin flips, we realize a finite one-dimensional chain of 1/2-spins with closed boundary conditions. We perform an in-depth investigation on behaviors shown across the quantum phase transition between paramagnetic and antiferromagnetic ground states, including the evolution of the magnetization and Néel order parameter. Also, we find evidence for quantum superposition at the many-body level as a result of geometric frustration. In the last chapter, I report the experimental realization of a novel dipolar Bose-Hubbard Hamiltonian, based on a strongly tilted lattice system. When the tilt becomes the dominant energy scale, the Hamiltonian is fragmented, and the system behaves in a way that conserves dipole moment. Starting from a 1D chain of unity filled sites, we generate individual dipolar and anti-dipolar excitations at desired pinpoints. We observe quantum walks of these dipolar quasi-particles as well as their scattering dynamics, which allows us to study this new type of Hamiltonian using a bottom-up approach.
The experimental control and observation of quantum many-body systems has become a reality with the advent of ultracold quantum matter. The high level of isolation of these experiments, together with the development of novel measurement techniques, has revived a fundamental debate concerning the thermal equilibration of isolated quantum systems, commonly named "quantum thermalization". In this thesis we make use of a quantum-gas microscope to explore the thermalizing dynamics of highly isolated systems of ultracold bosonic atoms in optical lattices. The ability to prepare and control quantum systems made up of hundreds of atoms makes it possible to explore regimes that represent a challenge for classical numeric simulations. A major part of this dissertation deals with Bose-Hubbard systems in the presence of quenched disorder. We begin by studying the microscopic properties of its phases near equilibrium, where by tuning the strength of the disorder, observe features consistent with the emergence of a so-called Bose-glass phase. We then continue by preparing states far from equilibrium and exploring their quantum many-body dynamics. In particular, we observe signatures of the phenomenon of "many-body localization", which implies a breakdown of quantum thermalization. In addition, we study whether localized systems can be thermalized via the coupling to a bath of few degrees of freedom, i.e. a quantum bath. We do so by preparing a mixture of two interacting atomic species, where one acts as the bath and the other as the localized system. We do observe delocalizing dynamics for large enough baths, though in regimes of weak coupling localization can survive for extremely long times. The second main topic of this thesis is the thermalization of periodically driven many-body systems, so-called Floquet thermalization. In these systems, the absence of energy conservation eventually brings any initial state into a featureless infinite-temperature one. However, for sufficiently high frequencies this thermalization process can take arbitrarily long times, which can enable the engineering of exotic long-lived prethermal states. We use the high isolation of our system, together with the high sensitivity of quantum-gas microscopy, to measure the heating rates for a range of driving frequencies and interaction regimes. Our results show a dramatic suppression of the heating as the frequency of the drive is increased, which is consistent with theoretical expectations.
This thesis reports on first experiments on the observation of ergodicity breaking in a two-component, interacting fermionic gas of Potassium-40 subject to quasi-periodic optical lattices in one and two dimensions, demonstrating the breakdown of thermalization in highly excited states of isolated quantum systems. Our observations can be explained by the phenomenon of many-body localization, a non-ergodic phase of matter, whose properties can be detected with non-equilibrium probes. To probe such a phase, we first design a far-from-equilibrium initial state and then monitor how much the system remembers of this design during time evolution. This allows us to identify regimes and timescales where disorder can protect local quantum information and distinguish such cases from regimes where interactions amalgamate local information into highly nonlocal quantum correlations. We then describe how this treatment systematically breaks down in all real-world systems as the system is (necessarily) coupled to some bath-like structure. Following very recent developments, we are further able to show that order can exist even in driven quantum systems, which were earlier thought to exhibit no interesting features, corresponding to an infinite temperature state. We also extend the experimental realm to explore two dimensions and show that the dynamics emerge as a distinct interplay of interactions, disorder, and dimensions. Upon probing a putative MBL transition, we further show signatures of a new kind of slow relaxation, potentially arising due to randomness in the initial state. We close with some theoretical results on probing quantum dynamics ensuing in the absence of transport and a discussion of exciting areas for future experiments.
Ultracold quantum gases in optical lattices provide a rich experimental toolbox for simulating the physics of condensed matter systems. With atoms in the lattice playing the role of electrons or Cooper pairs in real materials, it is possible to experimentally realize condensed matter Hamiltonians in a controlled way. To realize the full potential of such quantum simulations, we leverage a quantum gas microscope which can spatially resolve the atoms in the optical lattice at the single site level and project arbitrary potential landscapes onto the atoms by combining the high resolution optics with static holographic masks or a spatial light modulator. The versatility of this system allows for a wide range of studies. In this thesis, we focus on three experiments that highlight the utility of a tunable platform and demonstrate the richness of physics that comes with interactions.\nIn the first, we observe on-site interparticle interactions introduce a non-linearity into the many-body energy spectrum of a harmonic oscillator. The excitation of a single atom into a higher band induces an energy shift in the excitation energy for the second atom, blockading the orbital excitation. We demonstrate a technique for deterministic number filtering based upon orbital excitation blockade. When applied to a high temperature Mott insulator, this number filtering realizes a form of algorithmic cooling, which can be used for initializing a large quantum register or creating low entropy initial states for many-body simulation.\nIn the second, we study the applicability of statistical physics in an isolated system governed by quantum mechanics. While the descriptive power of these two fields has been confirmed through repeated and varied empirical studies, their underlying axioms of entropy maximization and unitary evolution appear mutually exclusive. With our quantum gas microscope, we have the ability to probe local observables such as the on-site number statistics as well as measure the quantum mechanical purity through interference operations. With these capabilities, we are able to observe the local thermalization of a manifestly quantum mechanically pure many-body system.\nIn the last chapter, we report on the first cold atoms studies of an interacting system under an artificial gauge field. We consider the propagation of a pair of atoms in a 2timesN ladder governed by the Harper-Hofstadter model. The eigenstates of this system include both scattering states, which can exhibit chiral propagation, and bound states. A superexchange energy shift in our initial state leads to imbalanced population in the two chiral scattering sectors, leading to chiral propagation dynamics. This effect is the result of both the presence of interactions and the artificial gauge fields. These two components are essential ingredients for fractional quantum Hall physics. Moreover, the dynamic tunable gauge field we develop and the control afforded by a quantum gas microscope make this platform well-suited for future studies in this regime.
Classical statistical mechanics relies on the ergodic hypothesis, which states that a system explores the entire allowed phase space during its time evolution. Pure quantum states are at odds with this concept as they remain in a single quantum state even if the system's parameters are suddenly altered. However, in a generic many-body system, coherent dynamics drive local thermalization of its subsystems. In this case, any local observable appears thermal and can be described by a statistical ensemble even though the full state remains pure. The key to understanding the phenomenon of quantum thermalization lies in the entanglement properties of the system: The presence of entanglement creates local entropy that validates the use of statistical physics.\nIn this thesis, we experimentally study the emergence of statistical mechanics in a quantum state and observe the fundamental role of quantum entanglement in facilitating this emergence. We perform microscopy on an evolving quantum system, and we see thermalization occur on a local scale while we measure that the full quantum state remains pure.\nThe only known robust exception from the paradigm of quantum thermalization is provided by disordered systems. In this case, the particle transport ceases through the system, preventing the formation of a sufficient amount of entanglement required for thermalization. However, if the many-body system is interacting, the state develops non-local quantum correlations that are inaccessible to any local observable. These correlations spread exponentially slowly in time throughout the entire system and are considered a hallmark feature of many-body-localized states.\nIn order to study the interplay between thermalization and localization in our system, we develop novel methods for high fidelity state preparation and readout. We achieved an exquisite isolation of our system from the environment, which allows us to monitor coherent many-body dynamics over multiple decades of time evolution.\nWe experimentally realize such a many-body localized system and observe the formation of non-local quantum correlations, while the particle transport is frozen in the system. Our work experimentally establishes many-body localization as a qualitatively distinct phenomenon from localization in non-interacting, disordered systems.
The study of non-equilibrium behaviors of quantum matter is one of the research directions at the frontiers of condensed matter physics and, in general, of theoretical and experimental physics. Understanding the mechanisms which prevent many quantum particles from reaching thermal equilibrium can ultimately shed light on the foundations of statistical physics and provide insight into the anomalous long-time collective behaviors observed in experiments. In this thesis, we present new theoretical developments in this direction. In the first part of the thesis we discuss the non-equilibrium dynamics of the two-dimensional quantum Ising model, the prototypical model of magnetism. In particular, we investigate the dynamics of interfaces separating different spin domains. In some regimes, we can provide an exact description of their unitary time evolution, but we also discuss the robustness of our predictions away from the exactly-solvable limit. Moreover, we address the same problem in the presence of disorder and provide a hydrodynamic interpretation of our findings. In the second part of the thesis, we investigate the localization properties of disordered quantum systems. In particular, we develop a renormalization-group picture of the Anderson localization transition in generic geometries. This provides a new framework to understand the phase diagram of such systems and their critical behavior beyond the usual finite-size scaling analysis. We also provide further insights on this topic both by studying resonances and their connection with observables and by employing unsupervised non-parametric learning techniques to probe disordered systems in an experimentally accessible form. The results presented in this thesis constitute a step forward in understanding the non-equilibrium phases and regimes of quantum matter and they pave the way to interesting future developments.