Ultracold quantum gases in optical lattices provide a rich experimental toolbox for simulating the physics of condensed matter systems. With atoms in the lattice playing the role of electrons or Cooper pairs in real materials, it is possible to experimentally realize condensed matter Hamiltonians in a controlled way. To realize the full potential of such quantum simulations, we leverage a quantum gas microscope which can spatially resolve the atoms in the optical lattice at the single site level and project arbitrary potential landscapes onto the atoms by combining the high resolution optics with static holographic masks or a spatial light modulator. The versatility of this system allows for a wide range of studies. In this thesis, we focus on three experiments that highlight the utility of a tunable platform and demonstrate the richness of physics that comes with interactions.\nIn the first, we observe on-site interparticle interactions introduce a non-linearity into the many-body energy spectrum of a harmonic oscillator. The excitation of a single atom into a higher band induces an energy shift in the excitation energy for the second atom, blockading the orbital excitation. We demonstrate a technique for deterministic number filtering based upon orbital excitation blockade. When applied to a high temperature Mott insulator, this number filtering realizes a form of algorithmic cooling, which can be used for initializing a large quantum register or creating low entropy initial states for many-body simulation.\nIn the second, we study the applicability of statistical physics in an isolated system governed by quantum mechanics. While the descriptive power of these two fields has been confirmed through repeated and varied empirical studies, their underlying axioms of entropy maximization and unitary evolution appear mutually exclusive. With our quantum gas microscope, we have the ability to probe local observables such as the on-site number statistics as well as measure the quantum mechanical purity through interference operations. With these capabilities, we are able to observe the local thermalization of a manifestly quantum mechanically pure many-body system.\nIn the last chapter, we report on the first cold atoms studies of an interacting system under an artificial gauge field. We consider the propagation of a pair of atoms in a $2\\times N$ ladder governed by the Harper-Hofstadter model. The eigenstates of this system include both scattering states, which can exhibit chiral propagation, and bound states. A superexchange energy shift in our initial state leads to imbalanced population in the two chiral scattering sectors, leading to chiral propagation dynamics. This effect is the result of both the presence of interactions and the artificial gauge fields. These two components are essential ingredients for fractional quantum Hall physics. Moreover, the dynamic tunable gauge field we develop and the control afforded by a quantum gas microscope make this platform well-suited for future studies in this regime.
Ultracold quantum gases in optical lattices provide a rich experimental toolbox for simulating the physics of condensed matter systems. With atoms in the lattice playing the role of electrons or Cooper pairs in real materials, it is possible to experimentally realize condensed matter Hamiltonians in a controlled way. To realize the full potential of such quantum simulations, we leverage a quantum gas microscope which can spatially resolve the atoms in the optical lattice at the single site level and project arbitrary potential landscapes onto the atoms by combining the high resolution optics with static holographic masks or a spatial light modulator. The versatility of this system allows for a wide range of studies. In this thesis, we focus on three experiments that highlight the utility of a tunable platform and demonstrate the richness of physics that comes with interactions.\nIn the first, we observe on-site interparticle interactions introduce a non-linearity into the many-body energy spectrum of a harmonic oscillator. The excitation of a single atom into a higher band induces an energy shift in the excitation energy for the second atom, blockading the orbital excitation. We demonstrate a technique for deterministic number filtering based upon orbital excitation blockade. When applied to a high temperature Mott insulator, this number filtering realizes a form of algorithmic cooling, which can be used for initializing a large quantum register or creating low entropy initial states for many-body simulation.\nIn the second, we study the applicability of statistical physics in an isolated system governed by quantum mechanics. While the descriptive power of these two fields has been confirmed through repeated and varied empirical studies, their underlying axioms of entropy maximization and unitary evolution appear mutually exclusive. With our quantum gas microscope, we have the ability to probe local observables such as the on-site number statistics as well as measure the quantum mechanical purity through interference operations. With these capabilities, we are able to observe the local thermalization of a manifestly quantum mechanically pure many-body system.\nIn the last chapter, we report on the first cold atoms studies of an interacting system under an artificial gauge field. We consider the propagation of a pair of atoms in a 2timesN ladder governed by the Harper-Hofstadter model. The eigenstates of this system include both scattering states, which can exhibit chiral propagation, and bound states. A superexchange energy shift in our initial state leads to imbalanced population in the two chiral scattering sectors, leading to chiral propagation dynamics. This effect is the result of both the presence of interactions and the artificial gauge fields. These two components are essential ingredients for fractional quantum Hall physics. Moreover, the dynamic tunable gauge field we develop and the control afforded by a quantum gas microscope make this platform well-suited for future studies in this regime.
Imagine a new generation of computers that dramatically surpasses the most powerful supercomputers, being able to tackle the most challenging of computational problems. These problems arise, for example, in quantum physics where the computational power required to model a many-particle system increases exponentially with the number of its constituents, and as a consequence the calculations become prohibitively time-consuming. Nobel laureate Richard Feynman proposed this new type of computer in the early 1980s: ‘Let the computer itself be built of quantum mechanical elements which obey quantum mechanical laws.’ Such a quantum simulator would allow researchers to tackle challenging problems in condensed-matter physics. In particular many-body fermionic quantum systems are very difficult to compute due to the antisymmetric nature of the wave function, and the resulting sign problem for quantum Monte Carlo methods. This is why a quantum simulator will be an excellent test bed to investigate phenomena and properties of strongly correlated fermionic quantum systems. A powerful experimental platform to realize a quantum simulator is laser-cooled atoms [1] held in an artificial crystal of light, generated by superimposing laser beams. The atoms are kept in this optical lattice similar to marbles in the hollows of an egg carton, and they can mimic the behaviour of electrons in a real crystal. These systems interface atomic physics with condensed matter physics in a new way, as the tools of atomic physics allow for exquisite control of many experimental parameters, which are often inaccessible in solid state experiments. In-situ imaging techniques [2] using ‘quantum-gas microscopes’ constitute a new approach to the study of many-body quantum systems in an optical lattice with unprecedented resolution at the single-particle and single-site level [3,4]. This new method is complementary to earlier optical lattice experiments measuring distributions in momentum space after a time-of-flight expansion. A quantum-gas microscope uses an optical imaging system (Fig. 1a) for collecting the fluorescence light of ultracold atoms in an optical lattice with high spatial resolution comparable to the lattice spacing of ≈ 500 nm. (a) Atoms in optical lattice atoms are imaged with a high-resolution microscope objective [4]. (b) Single-site addressing is achieved by focussing a laser beam through the microscope onto selected atoms, bringing them into resonance with microwave radiation which produces spin flips [12]. (c) and (d) Single-atom-resolved fluorescence images of bosonic Mottinsulators [4,9]. (e) Deterministically prepared atom distribution using single-site addressing [12]. (f) Direct observation of single-atom quantum walks [15]. Fluorescence imaging of atoms in a quantum-gas microscope has made it possible to directly observe bosonic Mott insulators with single-atom resolution [4–6], giving access to in-situ measurements of temperature and entropy distributions. Subsequently, ground-breaking experiments in many-body quantum dynamics have been performed, such as the first direct observation of correlation spreading after quenches of the system to lower lattice depths [7]. Other experiments include the quantum simulation of an antiferromagnetic spin-1/2 chain [8], the realization of algorithmic cooling [9], the direct measurement of correlations across the superfluid-to-Mott-insulator transition [10], or the observation of the ‘Higgs’ amplitude mode [11]. The high-resolution imaging system is also capable of optically addressing individual atoms with sub-diffraction-limited resolution. For this purpose, a laser beam is focussed though the microscope objective onto selected lattice sites, bringing the atoms into resonance with microwave radiation which produces spin flips [12,13]. The preparation of arbitrary atom distributions in the lattice not only opens perspectives for neutral-atom quantum information processing, but also allows the deterministic creation of specific out-of-equilibrium situations, and their ensuing system dynamics can be studied with single-atom resolution. Examples include the creation of spin impurities and the study of their dynamics in a many-body system [14], the observation of quantum walks [15] and magnon-bound states [16], and the measurement of entanglement entropy [17]. The technique used for single-site-resolved detection of individual atoms in the optical lattice is fluorescence imaging. It requires laser cooling of the atoms to sub-Doppler temperatures while detecting the fluorescence photons emitted during this process. A challenge is to achieve a low particle loss rate and to prevent the atoms from hopping between lattice sites. In the case of the first quantum-gas microscopes, this has been implemented with bosonic rubidium-87 atoms, and also recently for ytterbium-174. However, it has proven more challenging for fermionic alkaline species such as potassium-40 and lithium-6, as their low mass and small excited state hyperfine splitting-prevented standard sub-Doppler cooling from working. As a result, it took several years to extend the quantum-gas microscope technique to fermionic species, and in 2015 several groups have demonstrated single-atom-resolved imaging of fermions [18]. In these setups, the direct observation of band insulators [19], fermionic Mott insulators [20,21] and even antiferromagnetic correlations [22] has been reported most recently. These developments provide fascinating opportunities to study many-body fermionic quantum systems with single-particle access. The fermionic nature of the electron is vital to understanding a range of phenomena within solid-state physics, such as electron pairing in superconductivity, and quantum magnetism. In this context, the quantum simulator will allow, e.g. for direct measurement of ordered quantum phases and out-of-equilibrium dynamics, with access to quantities such as spin--spin correlation functions and the growth of many-body entanglement. The high-resolution imaging systems could also be used to project tailored time-varying light fields onto the atoms, allowing the removal of high-entropy regions by locally modifying the confining potential to attain very low-entropy states. Attaining these low-entropy many-particle states is one of the key challenges in our field. In summary, quantum-gas microscopes offer unprecedented access to many-body quantum systems, and they will allow us to gain an even deeper insight into the intriguing world of quantum physics that governs the properties of strongly correlated materials. Using a well-controlled quantum system to simulate other quantum systems could help resolve some of the most challenging problems scientists face in condensed matter physics and materials science, but it will also provide new insights in quantum chemistry, high-energy physics and biology. SK acknowledges funding from the EU (ERC FERMILATT, SIQS, QuProCs) and SUPA.
A system of ultracold atoms in an optical lattice provides a powerful platform for quantum simulation. In our laboratory, we use a quantum gas microscope to tune lattice parameters not only in a global scale but also at the level of individual sites. This allows us to control and detect the quantum state of interacting many-body systems as well as to engineer a broad class of Hamiltonians with high fidelity. Leveraging this versatility, we can realize several types of strongly correlated bosonic systems, which present intriguing behaviors and implement novel phases of matter. Analyzing snapshots of the atomic distribution with single-site resolution, we measure correlations and entanglement within these systems to reveal their main features, including non-equilibrium dynamics and quantum phase transitions. In this thesis, I present the works performed by our team for four different types of systems. First of all, I briefly introduce the behavior of a 1D disordered system in the critical regime between the thermal and the many-body-localized phases. In particular, we discuss what happens when a disordered and a non-disordered region are coupled via a single site. We find evidence for accelerated transport of thermal inclusion into the localized region, which shows the existence of a quantum avalanche, i.e. thermalization via accelerated transport throughout the localized system. In the second part, we realize a fractional quantum Hall state using an artificial gauge field, by implementing an adiabatic preparation protocol. We identify a topological phase transition in our system and characterize several key physical features expected for a Laughlin state by measuring density correlations and Hall conductivity. The next topic of this thesis relates to quantum magnetism. Mapping nearest hopping in a tilted optical lattice to spin flips, we realize a finite one-dimensional chain of 1/2-spins with closed boundary conditions. We perform an in-depth investigation on behaviors shown across the quantum phase transition between paramagnetic and antiferromagnetic ground states, including the evolution of the magnetization and Néel order parameter. Also, we find evidence for quantum superposition at the many-body level as a result of geometric frustration. In the last chapter, I report the experimental realization of a novel dipolar Bose-Hubbard Hamiltonian, based on a strongly tilted lattice system. When the tilt becomes the dominant energy scale, the Hamiltonian is fragmented, and the system behaves in a way that conserves dipole moment. Starting from a 1D chain of unity filled sites, we generate individual dipolar and anti-dipolar excitations at desired pinpoints. We observe quantum walks of these dipolar quasi-particles as well as their scattering dynamics, which allows us to study this new type of Hamiltonian using a bottom-up approach.
Ultracold atoms in optical lattices provide an extremely clean and controllable setting to explore quantum many-body phases of matter. Here we give a brief review of the strong-correlation physics that has been realized using such ultracold atoms in optical lattices ranging from the realization of Hubbard models to studies of quantum magnetism and the detection of single atoms with lattice site resolution. All this has opened up fundamentally new opportunities for the investigation of quantum many-body systems. Introduction Over the past years, ultracold atoms in optical lattices have emerged as versatile new systems to explore the physics of quantum many-body systems. On the one hand, they can be helpful in gaining a better understanding of known phases of matter and their dynamical behavior; on the other hand, they allow one to realize completely novel quantum systems that have not been studied before in nature [1, 2, 3]. Commonly, the approach of exploring quantum many-body systems in such a way is referred to as “quantum simulations.” Examples of some of the first strongly interacting many-body phases that have been realized both in lattices and in the continuum include the quantum phase transition from a superfluid to a Mott insulator [4, 5, 6], fermionic Mott insulators [7, 8], the achievement of a Tonks- Girardeau gas [9, 10], and the realization of the Bose-Einsten condensate (BEC)– Bardeen-Cooper-Schrieffer (BCS) crossover (see also Chapter 12) in Fermi gas mixture [11] using Feshbach resonances [12]. In almost all of these experiments, detection was limited to time-of-flight imaging or more refined derived techniques that mainly characterized the momentum distribution of the quantum gas [2]. For several years, researchers in the field have therefore aspired to employ in situ single-particle detection methods for the analysis of ultracold quantum gases. Only recently has it become possible to implement such imaging techniques, marking a milestone for the characterization and manipulation of ultracold quantum gases [13, 14, 15, 16, 17]. In our discussion, we will focus on one of the most successful of these techniques based on high-resolution fluorescence imaging. Despite being a rather new technique, such quantum gas microscopy has already proven to be an enabling technology for probing and manipulating quantum many-body systems. For the first time, controllable and strongly interacting many-body systems, as realized with ultracold atoms, could be observed on a local scale [17, 16].
"The many weird properties of quantum mechanics at the very small scale have led to surprising and useful discoveries that manifest at the macroscopic level, like the quantum Hall effect and high temperature superconductivity. Yet trying to understand the origin of correlated behavior from interacting quantum systems via classical simulation requires an infeasible level of computing power. Instead, we can use an easily tunable, clean quantum system as a quantum simulation of a more unwieldy system, building the same model to study the same physics, but in a more controlled environment. Our field of cold neutral atoms in optical lattices has seen success over many years as a platform for quantum simulation of various lattice models from condensed matter physics. The recent (2015) implementation of lattices not in position, but in a synthetic dimension by coupling individual quantum states with lasers has led to a more bottom-up approach to engineering lattice models. In this thesis, we present our ""momentum-space lattice"" technique in which we use individual laser frequencies to couple the momentum states of a rubidium-87 Bose-Einstein condensate, in order to create lattices with site-by-site and link-by-link precision. This technique is simple to implement experimentally, requiring just two additional common optical components (acousto-optic modulators) compared to a real-space lattice, yet is incredibly versatile. Using momentum-space lattices, we have studied the physics of artificial magnetic fields, disorder and pseudodisorder-induced localization, and atomic interactions across eight works described in this thesis. More interesting are the not-so-well-known effects that arise in the interplay among these three components of topology, disorder, and interactions, and we have made headway towards studying physics in this regime. To be more specific, in our studies we have generated an artificial magnetic field for neutral atoms, and directly observed the resulting chiral currents in both a square ladder and zigzag lattice geometry. We have further monitored the quantum walk behavior of atoms under disordered and pseudodisordered lattices, observing a transition to localization under a quasiperiodic potential. We have been able to introduce a tunable energy dependence to this localization transition (single-particle mobility edge) in two ways: with the addition of more tunneling pathways, and by modifying the form of the potential. Finally, we have studied the effects of nonlinear inter-atomic interactions in the momentum-space lattice, observing self-trapping in a double well system as well as on a full lattice, showing a skewed current-phase relationship in an analog to Josephson junction arrays, and investigating an interaction-induced shift in localization behavior under pseudodisorder. In constructing the momentum-space lattice apparatus, Eric, Bryce, and I have created a promising new platform for Hamiltonian engineering. The studies described here not only show off the capabilities of the technique, but also realize new models, reveal new physics, and provide a new perspective complementary to both real-space lattice techniques and real materials. We have observed topological edge states more directly than previous works and engineered precise lattice parameter variations unavailable to other techniques, and yet the best is still to come. With our ongoing experimental upgrades comes access to the regime of strong inter-particle interactions, which promises more challenging yet more rewarding experiments."
Experiments with ultracold atoms in optical lattices provide outstanding opportunities to realize exotic quantum states due to a high degree of tunability and control. In this thesis, I present experiments that extend this control from global parameters to the level of individual particles. \n\nUsing a quantum gas microscope for 87Rb, we have developed a single-site addressing scheme based on digital amplitude holograms. The system self-corrects for aberrations in the imaging setup and creates arbitrary beam profiles. We are thus able to shape optical potentials on the scale of single lattice sites and control the dynamics of individual atoms. \n\nWe study the role of quantum statistics and interactions in the Bose-Hubbard model on the fundamental level of two particles. Bosonic quantum statistics are apparent in the Hong-Ou-Mandel interference of massive particles, which we observe in tailored double-well potentials. These underlying statistics, in combination with tunable repulsive interactions, dominate the dynamics in single- and two-particle quantum walks. We observe highly coherent position-space Bloch oscillations, bosonic bunching in Hanbury Brown-Twiss interference and the fermionization of strongly interacting bosons.\n\nMany-body states of indistinguishable quantum particles are characterized by large-scale spatial entanglement, which is difficult to detect in itinerant systems. Here, we extend the concept of Hong-Ou-Mandel interference from individual particles to many-body states to directly quantify entanglement entropy. We perform collective measurements on two copies of a quantum state and detect entanglement entropy through many-body interference. We measure the second order Rényi entropy in small Bose-Hubbard systems and detect the buildup of spatial entanglement across the superfluid-insulator transition.\n\nOur experiments open new opportunities for the single-particle-resolved preparation and characterization of many-body quantum states.
One of the distinguishing achievements of physics has been the ability to describe the Universe based upon underlying microscopic principles. When there are many participating objects being governed by these microscopic principles, the resultant behavior often harbors emergent collective phenomena that may not be obviously related to the microscopic description. Phase transitions, quantum or classical, are a canonical example of such many-body phenomena that are understood in equilibrium through a framework of thermodynamic constraints, statistical ensembles, and a growth of system-wide correlations at the transition. However, a new class of quantum phase transitions has recently emerged for non-equilibrium systems with behavior that is not captured by this traditional framework. In the case of isolated quantum systems, these transitions occur among excited eigenstates and requires knowledge of the structure of these individual eigenstates in the quantum system. Understanding what drives such a phase transition requires a deeper microscopic knowledge of the role of correlations at the transition. \nThe use of ultracold atoms in optical lattices has paved the way for faithfully realizing quantum phase transitions. In particular, the advent of the quantum gas microscope realized an experimental platform that is highly controllable and provides microscopic access to the many-bodied wave functions. All experiments presented in this thesis use such a quantum gas microscope architecture where a quantum degenerate gas of Rb is used to probe the behavior of non-equilibrium quantum systems in one spatial dimension.\nThis thesis briefly discusses some studies of entanglement in equilibrium quantum phase transitions near the ground state of the system. In the first experiment, we directly measure the second-order R\\'enyi entanglement entropy that develops as a Bose-Hubbard system transitions from a Mott insulator to a superfluid. This is followed by a study of entanglement growth at the transition in the transverse Ising model. \nThese studies progress to the investigation of two particular non-equilibrium quantum phases and their transition into one another: quantum thermalization and many-body localization. We investigate the development of entanglement entropy that mimics thermodynamic entropy for an isolated quantum system which locally thermalizes under its own unitary dynamics. We then investigate the only known robust exception to this thermalizing behavior by studying the onset of many-body localization due to disorder. We observe the breakdown of thermalization in this phase and the logarithmically slow growth of entanglement throughout the system, which identifies the localized system to be an interacting one. Lastly, we investigate the role of correlations in the critical dynamics that emerge at high-orders where the system transitions from thermalizing behavior to many-body localization.