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Probing quantum thermalization and localization in Bose-Hubbard systems

Antonio Rubio-Abadal

Published Jan 1, 2020• 0 citations
Publisher

Abstract

The experimental control and observation of quantum many-body systems has become a reality with the advent of ultracold quantum matter. The high level of isolation of these experiments, together with the development of novel measurement techniques, has revived a fundamental debate concerning the thermal equilibration of isolated quantum systems, commonly named "quantum thermalization". In this thesis we make use of a quantum-gas microscope to explore the thermalizing dynamics of highly isolated systems of ultracold bosonic atoms in optical lattices. The ability to prepare and control quantum systems made up of hundreds of atoms makes it possible to explore regimes that represent a challenge for classical numeric simulations. A major part of this dissertation deals with Bose-Hubbard systems in the presence of quenched disorder. We begin by studying the microscopic properties of its phases near equilibrium, where by tuning the strength of the disorder, observe features consistent with the emergence of a so-called Bose-glass phase. We then continue by preparing states far from equilibrium and exploring their quantum many-body dynamics. In particular, we observe signatures of the phenomenon of "many-body localization", which implies a breakdown of quantum thermalization. In addition, we study whether localized systems can be thermalized via the coupling to a bath of few degrees of freedom, i.e. a quantum bath. We do so by preparing a mixture of two interacting atomic species, where one acts as the bath and the other as the localized system. We do observe delocalizing dynamics for large enough baths, though in regimes of weak coupling localization can survive for extremely long times. The second main topic of this thesis is the thermalization of periodically driven many-body systems, so-called Floquet thermalization. In these systems, the absence of energy conservation eventually brings any initial state into a featureless infinite-temperature one. However, for sufficiently high frequencies this thermalization process can take arbitrarily long times, which can enable the engineering of exotic long-lived prethermal states. We use the high isolation of our system, together with the high sensitivity of quantum-gas microscopy, to measure the heating rates for a range of driving frequencies and interaction regimes. Our results show a dramatic suppression of the heating as the frequency of the drive is increased, which is consistent with theoretical expectations.

DOI
10.5282/edoc.26273

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"This thesis presents research on a variety of dynamical phenomena in strongly correlated systems. We use 87Rb atoms trapped in a disordered optical lattice to realize the 3D Bose Hubbard model, with independently, dynamically tunable lattice depth and disorder strength. The equilibrium behavior of the Bose Hubbard and disordered Bose Hubbard models are understood, but there are many outstanding questions about dynamics. One area of interest is in dynamical behavior near quantum phase boundaries, such as the generation of quench-induced excitations in the presence of disorder. Another area concerns heat flow, relaxation, and thermalization. The primary focus of this thesis is driving a gas across a disorder-induced quantum phase transition from the Bose glass to the superfluid phase via quenching the disorder. We measured excitations generated during the quench and related them to crossing the equilibrium phase transition determined by quantum Monte Carlo simulations of the trapped system. The behavior we observe is reminiscent of the quantum Kibble Zurek mechanism, where the relaxation timescale diverges and local fluctuations are ""frozen"" into the system near the phase boundary. Understanding how disorder impacts the Kibble Zurek paradigm about behavior near a phase boundary provides insight into the dynamics of strongly interacting, disordered systems. The three other works discussed in this thesis concern relaxation and energy transfer in clean optical lattices. Understanding these dynamical properties of lattice gases is key to developing tools such as cooling in a lattice. In the first result, a gas comprised of two spin states was loaded into a spin-dependent optical lattice, such that one spin state experienced the lattice, and the other did not. We found that when the lattice gas was heated, energy transfer to the non-lattice gas did not occur at higher lattice depths due to the mismatch in the dispersion relations. In the second result, lattice atoms were excited to a higher band and found to decay to the ground state via two mechanisms. One decay channel involved generating excitations in the non-lattice atoms, while the other channel involved collisions between lattice atoms, where one atom decayed to the ground state and the other was excited to a higher band. The final result measured relaxation timescales by removing atoms with low quasimomentum and measuring rethermalization. The observed timescales are faster than the tunneling time and interaction time of the lattice. Proof-of-principle cooling was also demonstrated by removing atoms with higher quasimomentum and allowing the remaining atoms rethermalize to a cooler temperature."

•Apr 1, 2016•1 citation
The experimental control and observation of quantum many-body systems has become a reality with the advent of ultracold quantum matter. The high level of isolation of these experiments, together with the development of novel measurement techniques, has revived a fundamental debate concerning the thermal equilibration of isolated quantum systems, commonly named "quantum thermalization". In this thesis we make use of a quantum-gas microscope to explore the thermalizing dynamics of highly isolated systems of ultracold bosonic atoms in optical lattices. The ability to prepare and control quantum systems made up of hundreds of atoms makes it possible to explore regimes that represent a challenge for classical numeric simulations. A major part of this dissertation deals with Bose-Hubbard systems in the presence of quenched disorder. We begin by studying the microscopic properties of its phases near equilibrium, where by tuning the strength of the disorder, observe features consistent with the emergence of a so-called Bose-glass phase. We then continue by preparing states far from equilibrium and exploring their quantum many-body dynamics. In particular, we observe signatures of the phenomenon of "many-body localization", which implies a breakdown of quantum thermalization. In addition, we study whether localized systems can be thermalized via the coupling to a bath of few degrees of freedom, i.e. a quantum bath. We do so by preparing a mixture of two interacting atomic species, where one acts as the bath and the other as the localized system. We do observe delocalizing dynamics for large enough baths, though in regimes of weak coupling localization can survive for extremely long times. The second main topic of this thesis is the thermalization of periodically driven many-body systems, so-called Floquet thermalization. In these systems, the absence of energy conservation eventually brings any initial state into a featureless infinite-temperature one. However, for sufficiently high frequencies this thermalization process can take arbitrarily long times, which can enable the engineering of exotic long-lived prethermal states. We use the high isolation of our system, together with the high sensitivity of quantum-gas microscopy, to measure the heating rates for a range of driving frequencies and interaction regimes. Our results show a dramatic suppression of the heating as the frequency of the drive is increased, which is consistent with theoretical expectations.
This thesis reports on first experiments on the observation of ergodicity breaking in a two-component, interacting fermionic gas of Potassium-40 subject to quasi-periodic optical lattices in one and two dimensions, demonstrating the breakdown of thermalization in highly excited states of isolated quantum systems. Our observations can be explained by the phenomenon of many-body localization, a non-ergodic phase of matter, whose properties can be detected with non-equilibrium probes. To probe such a phase, we first design a far-from-equilibrium initial state and then monitor how much the system remembers of this design during time evolution. This allows us to identify regimes and timescales where disorder can protect local quantum information and distinguish such cases from regimes where interactions amalgamate local information into highly nonlocal quantum correlations. We then describe how this treatment systematically breaks down in all real-world systems as the system is (necessarily) coupled to some bath-like structure. Following very recent developments, we are further able to show that order can exist even in driven quantum systems, which were earlier thought to exhibit no interesting features, corresponding to an infinite temperature state. We also extend the experimental realm to explore two dimensions and show that the dynamics emerge as a distinct interplay of interactions, disorder, and dimensions. Upon probing a putative MBL transition, we further show signatures of a new kind of slow relaxation, potentially arising due to randomness in the initial state. We close with some theoretical results on probing quantum dynamics ensuing in the absence of transport and a discussion of exciting areas for future experiments.
Periodic driving has emerged as a powerful tool in the quest to engineer new and exotic quantum phases.While driven many-body systems are generically expected to absorb energy indefinitely and reach an infinitetemperature state, the rate of heating can be exponentially suppressed when the drive frequency is large compared to the local energy scales of the system-leading to long-lived "prethermal" regimes.In this work, we experimentally study a bosonic cloud of ultracold atoms in a driven optical lattice and identify such a prethermal regime in the Bose-Hubbard model.By measuring the energy absorption of the cloud as the driving frequency is increased, we observe an exponential-in-frequency reduction of the heating rate persisting over more than 2 orders of magnitude.The tunability of the lattice potentials allows us to explore one-and twodimensional systems in a range of different interacting regimes.Alongside the exponential decrease, the dependence of the heating rate on the frequency displays features characteristic of the phase diagram of the Bose-Hubbard model, whose understanding is additionally supported by numerical simulations in one dimension.Our results show experimental evidence of the phenomenon of Floquet prethermalization and provide insight into the characterization of heating for driven bosonic systems.
Periodic driving has emerged as a powerful tool in the quest to engineer new and exotic quantum phases. While driven many-body systems are generically expected to absorb energy indefinitely and reach an infinite-temperature state, the rate of heating can be exponentially suppressed when the drive frequency is large compared to the local energy scales of the system -- leading to long-lived 'prethermal' regimes. In this work, we experimentally study a bosonic cloud of ultracold atoms in a driven optical lattice and identify such a prethermal regime in the Bose-Hubbard model. By measuring the energy absorption of the cloud as the driving frequency is increased, we observe an exponential-in-frequency reduction of the heating rate persisting over more than 2 orders of magnitude. The tunability of the lattice potentials allows us to explore one- and two-dimensional systems in a range of different interacting regimes. Alongside the exponential decrease, the dependence of the heating rate on the frequency displays features characteristic of the phase diagram of the Bose-Hubbard model, whose understanding is additionally supported by numerical simulations in one dimension. Our results show experimental evidence of the phenomenon of Floquet prethermalization, and provide insight into the characterization of heating for driven bosonic systems.
One of the distinguishing achievements of physics has been the ability to describe the Universe based upon underlying microscopic principles. When there are many participating objects being governed by these microscopic principles, the resultant behavior often harbors emergent collective phenomena that may not be obviously related to the microscopic description. Phase transitions, quantum or classical, are a canonical example of such many-body phenomena that are understood in equilibrium through a framework of thermodynamic constraints, statistical ensembles, and a growth of system-wide correlations at the transition. However, a new class of quantum phase transitions has recently emerged for non-equilibrium systems with behavior that is not captured by this traditional framework. In the case of isolated quantum systems, these transitions occur among excited eigenstates and requires knowledge of the structure of these individual eigenstates in the quantum system. Understanding what drives such a phase transition requires a deeper microscopic knowledge of the role of correlations at the transition. \nThe use of ultracold atoms in optical lattices has paved the way for faithfully realizing quantum phase transitions. In particular, the advent of the quantum gas microscope realized an experimental platform that is highly controllable and provides microscopic access to the many-bodied wave functions. All experiments presented in this thesis use such a quantum gas microscope architecture where a quantum degenerate gas of Rb is used to probe the behavior of non-equilibrium quantum systems in one spatial dimension.\nThis thesis briefly discusses some studies of entanglement in equilibrium quantum phase transitions near the ground state of the system. In the first experiment, we directly measure the second-order R\\'enyi entanglement entropy that develops as a Bose-Hubbard system transitions from a Mott insulator to a superfluid. This is followed by a study of entanglement growth at the transition in the transverse Ising model. \nThese studies progress to the investigation of two particular non-equilibrium quantum phases and their transition into one another: quantum thermalization and many-body localization. We investigate the development of entanglement entropy that mimics thermodynamic entropy for an isolated quantum system which locally thermalizes under its own unitary dynamics. We then investigate the only known robust exception to this thermalizing behavior by studying the onset of many-body localization due to disorder. We observe the breakdown of thermalization in this phase and the logarithmically slow growth of entanglement throughout the system, which identifies the localized system to be an interacting one. Lastly, we investigate the role of correlations in the critical dynamics that emerge at high-orders where the system transitions from thermalizing behavior to many-body localization.
A system of ultracold atoms in an optical lattice provides a powerful platform for quantum simulation. In our laboratory, we use a quantum gas microscope to tune lattice parameters not only in a global scale but also at the level of individual sites. This allows us to control and detect the quantum state of interacting many-body systems as well as to engineer a broad class of Hamiltonians with high fidelity. Leveraging this versatility, we can realize several types of strongly correlated bosonic systems, which present intriguing behaviors and implement novel phases of matter. Analyzing snapshots of the atomic distribution with single-site resolution, we measure correlations and entanglement within these systems to reveal their main features, including non-equilibrium dynamics and quantum phase transitions. In this thesis, I present the works performed by our team for four different types of systems. First of all, I briefly introduce the behavior of a 1D disordered system in the critical regime between the thermal and the many-body-localized phases. In particular, we discuss what happens when a disordered and a non-disordered region are coupled via a single site. We find evidence for accelerated transport of thermal inclusion into the localized region, which shows the existence of a quantum avalanche, i.e. thermalization via accelerated transport throughout the localized system. In the second part, we realize a fractional quantum Hall state using an artificial gauge field, by implementing an adiabatic preparation protocol. We identify a topological phase transition in our system and characterize several key physical features expected for a Laughlin state by measuring density correlations and Hall conductivity. The next topic of this thesis relates to quantum magnetism. Mapping nearest hopping in a tilted optical lattice to spin flips, we realize a finite one-dimensional chain of 1/2-spins with closed boundary conditions. We perform an in-depth investigation on behaviors shown across the quantum phase transition between paramagnetic and antiferromagnetic ground states, including the evolution of the magnetization and Néel order parameter. Also, we find evidence for quantum superposition at the many-body level as a result of geometric frustration. In the last chapter, I report the experimental realization of a novel dipolar Bose-Hubbard Hamiltonian, based on a strongly tilted lattice system. When the tilt becomes the dominant energy scale, the Hamiltonian is fragmented, and the system behaves in a way that conserves dipole moment. Starting from a 1D chain of unity filled sites, we generate individual dipolar and anti-dipolar excitations at desired pinpoints. We observe quantum walks of these dipolar quasi-particles as well as their scattering dynamics, which allows us to study this new type of Hamiltonian using a bottom-up approach.
"This thesis presents research on a variety of dynamical phenomena in strongly correlated systems. We use 87Rb atoms trapped in a disordered optical lattice to realize the 3D Bose Hubbard model, with independently, dynamically tunable lattice depth and disorder strength. The equilibrium behavior of the Bose Hubbard and disordered Bose Hubbard models are understood, but there are many outstanding questions about dynamics. One area of interest is in dynamical behavior near quantum phase boundaries, such as the generation of quench-induced excitations in the presence of disorder. Another area concerns heat flow, relaxation, and thermalization. The primary focus of this thesis is driving a gas across a disorder-induced quantum phase transition from the Bose glass to the superfluid phase via quenching the disorder. We measured excitations generated during the quench and related them to crossing the equilibrium phase transition determined by quantum Monte Carlo simulations of the trapped system. The behavior we observe is reminiscent of the quantum Kibble Zurek mechanism, where the relaxation timescale diverges and local fluctuations are ""frozen"" into the system near the phase boundary. Understanding how disorder impacts the Kibble Zurek paradigm about behavior near a phase boundary provides insight into the dynamics of strongly interacting, disordered systems. The three other works discussed in this thesis concern relaxation and energy transfer in clean optical lattices. Understanding these dynamical properties of lattice gases is key to developing tools such as cooling in a lattice. In the first result, a gas comprised of two spin states was loaded into a spin-dependent optical lattice, such that one spin state experienced the lattice, and the other did not. We found that when the lattice gas was heated, energy transfer to the non-lattice gas did not occur at higher lattice depths due to the mismatch in the dispersion relations. In the second result, lattice atoms were excited to a higher band and found to decay to the ground state via two mechanisms. One decay channel involved generating excitations in the non-lattice atoms, while the other channel involved collisions between lattice atoms, where one atom decayed to the ground state and the other was excited to a higher band. The final result measured relaxation timescales by removing atoms with low quasimomentum and measuring rethermalization. The observed timescales are faster than the tunneling time and interaction time of the lattice. Proof-of-principle cooling was also demonstrated by removing atoms with higher quasimomentum and allowing the remaining atoms rethermalize to a cooler temperature."