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CRC Press eBooks

Propagation of Nonclassical Light

Izo I. Abram

Published Aug 12, 2020• 0 citations
Publisher

Abstract

Classical optics describes quite successfully the propagation of laser light, both in free-space and inside a transparent medium. On the other hand, neither classical optics nor the conventional formulation of quantum optics can address adequately the propagation of nonclassical light. Nonclassical states of light are usually described by second-quantization operators acting onto the vacuum state of the radiation field, and the corresponding expectation values of the electric and magnetic fields are often zero. Clearly, the description of propagation of nonclassical light requires a direct quantum mechanical treatment of the spatial progression of the field operators. This chapter outlines the main features of propagative quantum optics, and examines more particularly the treatment of propagation through a linear (refractive) medium, and across a refractive interface. In order to facilitate the discussion of the physical ideas, a plane-wave propagation geometry, which greatly simplifies the mathematical treatment, is used.

DOI
10.1201/9781003069539-9

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Classical optics describes quite successfully the propagation of laser light, both in free-space and inside a transparent medium. On the other hand, neither classical optics nor the conventional formulation of quantum optics can address adequately the propagation of nonclassical light. Nonclassical states of light are usually described by second-quantization operators acting onto the vacuum state of the radiation field, and the corresponding expectation values of the electric and magnetic fields are often zero. Clearly, the description of propagation of nonclassical light requires a direct quantum mechanical treatment of the spatial progression of the field operators. This chapter outlines the main features of propagative quantum optics, and examines more particularly the treatment of propagation through a linear (refractive) medium, and across a refractive interface. In order to facilitate the discussion of the physical ideas, a plane-wave propagation geometry, which greatly simplifies the mathematical treatment, is used.
We have developed a quantum-mechanical formalism which permits the treatment of light propagation within the conceptual framework of quantum optics. The formalism rests on the calculation of the momentum operator for the radiation field, and yields directly a description for the spatial progression of the electromagnetic waves. In this paper we give a quantum-mechanical treatment for refraction and reflection by applying our formalism to propagation through a linear dielectric. The fidelity with which this formalism reproduces all results known from classical optics demonstrates its validity.
Starting with the canonical quantization procedure for the electromagnetic field inside an effective (linear or nonlinear) medium, we present a direct-space formulation of the theory of quantum optics. This approach does not use the conventional modal decomposition of the field, but relies on the electromagnetic momentum operator defined in terms of local electric- and magnetic-field operators. The momentum operator contains all the information on the spatial characteristics of the field, and can describe the translation of a short light pulse in a nonlinear medium, without a modal analysis of the pulse. Propagation is described through an operatorial wave equation that relates the temporal evolution of an electromagnetic pulse to its spatial progression. Through this equation, the direct-space approach to quantum optics can treat traveling-wave nonlinear-optical phenomena and, at the same time, account for their quantum statistics. The theory is applied to squeezed-light generation by the parametric down-conversion of a short laser pulse, as an illustration.
We will begin our journey through the background of quantum optics with an elementary, but quantitative, classical theory of radiative fields.Wewill first briefly outline the electromagnetic (EM) theory of radiation, and describe how the EM radiation may be understood as a wavewhich can be represented by a set of harmonic oscillators. We shall describe how the free or non-interacting EM field may be understood as a collection of harmonic oscillators which is quantized in the standard manner, and whose energy cannot be zero as a consequence of the basic non-commutability of the canonical field variables. This chapter discusses the properties of plane EM waves and normalization of the EM field in one dimension. This is followed by a description of the Hamiltonian and the amplitudes of the EM field in terms of the annihilation and creation operators. Based on this chapter, it is possible to considerably simplify the formulation of the physical basis for the mathematical description of the major problems of quantum optics.
In this chapter we shall be using the formalism of Chapter 4 to describe some properties of the quantized free electromagnetic field, emphasizing the analogies and differences with classical electromagnetism. The analogies explain why classical optics was so successful, to the extent that, even though light was not quantized, it was able to describe almost all known optical phenomena up until the 1970s. The differences highlight typical quantum behaviour, with no classical equivalent, which lies at the heart of modern quantum optics. The chapter begins by presenting formal ways of describing the main components of quantum optics experiments, namely, photodetectors and semi-reflecting mirrors. One can then understand homodyne detection, used to measure field quadrature components, even at optical frequencies for which no detector is fast enough to follow the oscillations of the field itself. Section 5.2 deals with the quantum vacuum where, in contrast to the classical vacuum, radiation has properties, in particular, fluctuations, with which one can associate physical effects. We then discuss in Section 5.3 some quantum radiation states in the simple case where a single mode l of the field is excited (non-vacuum). We introduce the idea of a quasiclassical state, or coherent state, used to make the link with classical optics. We shall also study other states, those with a definite number of photons, or squeezed states, which exhibit typically quantum properties, quite inconceivable in classical electromagnetism, and we shall show how these properties can be understood by reference to the Heisenberg relations, with an extremely useful graphical representation.
Introduction Up to now the electromagnetic field has been treated as a classical field, describable by c -number functions. The great success of classical electromagnetic theory in accounting for a variety of optical phenomena, particularly those connected with wave propagation, interference and diffraction, amply justifies the classical approach. Moreover, as we have seen in the preceding chapters, in some cases the classical wave theory also gives a good account of itself in the treatment of the interaction of electromagnetic fields. For example, it is able to describe such seemingly non-classical effects as photoelectric bunching and the photo-electric counting statistics. It might almost seem that there is little justification for going beyond the domain of classical wave theory in optics. On the other hand, it can be argued that optics lies well and truly in the quantum domain, in the sense that we often encounter situations in which very few quanta or photons are present. In the microwave region of the electromagnetic spectrum, and at still longer wavelengths, the number of photons in each mode of the field is usually very large, and we are justified in treating the system classically. However, in the optical region the situation is usually just the opposite. As we show in Section 13.1, for light produced by practically all sources other than lasers, the average number of photons per mode is typically much less than unity.
Classical, semi-classical, and quantum-field descriptions for the interaction of light with matter are systematically discussed. Applications of interest include precise determinations of the linear and the non-linear electromagnetic response relevant to resonant pump-probe optical phenomena, such as electromagnetically induced transparency. In the quantum-mechanical description of matter systems, we introduce a general reduced-density-matrix framework. Time-domain (equation-of-motion) and frequency-domain (resolvent-operator) formulations are developed in a unified and self-consistent manner, using a Liouville-space operator representation. A preliminary semi-classical perturbation treatment of the electromagnetic interaction is adopted, in which the electromagnetic field is described as a classical field satisfying the Maxwell equations. Compact Liouville-space operator expressions are derived for the linear and the general (nth order) non-linear electromagnetic-response tensors describing moving many-electron systems. The tetradic matrix elements of the Liouville-space self-energy operators, which are introduced in the time-domain and frequency-domain formulations, are evaluated for environmental collisional and radiative interactions, in order to provide explicit forms for the quantum kinetic equations and the spectral-line shape formulas. It is emphasized that a quantized-field approach is essential for a fully self-consistent quantum-mechanical description of the interacting light-matter system.