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Applied Physics Letters

Heralded spectroscopy with a fiber photon-pair source

Emma J. Pearce, Chris C. Phillips, Rupert F. Oulton, Alex S. Clark

Published Aug 3, 2020• 13 citations
Publisher

Abstract

The correlations between photons generated by nonlinear optical processes offer advantages for many quantum technology applications, including spectroscopy, imaging, and metrology. Here, we use spontaneous four-wave mixing in a birefringent single-mode fiber pumped by a tunable pulsed laser as a broadly tunable source of phase-matched non-degenerate photon pairs for spectroscopy. The pairs are tunable such that the idler beam measures the transmittance spectrum of a sample in the near infrared, while the visible signal beam independently reports correlation information. By the time-resolved counting of both signal and idler photons, we use photon-number correlations to remove uncorrelated noise from the probe beam. Here, we have used heralded spectroscopy to measure the absorption spectrum of gallium arsenide near its band edge, despite the idler photon spectrum being dominated by a large background from spontaneous Raman scattering.

DOI
10.1063/5.0016106

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Q uantum entanglement refers to the nonclassical dependency of physically separated quantum systems. It is an essential resource that must be freely available for implementing many of the novel functions of quantum information processing, such as database searching, clock synchronization, teleportation, computing and cryptography.1 The efficient generation and transmission of quantum entanglement is therefore of prime importance. With the ubiquitous standard optical fiber serving as the transmission medium and the widespread availability of efficient active and passive fiber devices, technological synergy between the generation and propagation components of the overall quantum network can be achieved by deploying sources of entanglement that rely on the nonlinearity of the fiber itself. 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It must be pointed out here that in a conventional wavelength-divisionmultiplexed classical optical communication line, one strives to suppress the fourphoton or four-wave mixing process, which otherwise causes cross talk between the wavelength channels and sets limits on the total data capacity of the communication line. In our experiment, the four-photon mixing takes place in a nonlinear-fiber Sagnac interferometer (NFSI), which we previously used to generate quantum-correlated twin beams in the fiber.5 The pump is a mode-locked train of ~3-ps-long pulses. The pulsed operation serves two important purposes: the NFSI amplifier can be operated at low average powers and the production of the signal/ idler fluorescence photons is confined to well-defined temporal windows, allowing use of a gated detection scheme to increase the signal-to-noise ratio. To measure the nonclassical (i.e., quantum) correlations between the signal and the idler photons, one must effectively suppress the pump photons from reaching the detectors. Since a typical pump pulse contains ~108 photons and we are interested in detecting ~0.01 signal (idler) photons/pulse, a pump-to-signal (idler) rejection ratio in excess of 100 dB is required. We achieved this specification by sending the fluorescence photons through a free-space double-grating spectral filter that separates the signal and idler photons from each other and from the pump photons not rejected by the NFSI. To demonstrate the quantum nature of the four-photon scattering at the single photon level, we assembled a photonFigure 1.C oincidence rates as a function of the single-photon rates in two different cases: signalidler fluorescence produced by a pump pulse (diamonds) and signal-idler fluorescence produced by two consecutive pump pulses (triangles). T he line represents the calculated accidental counts. T he inset shows a plot of the detected idler photons as a function of the injected pump photons (hollow circles). A second-order polynomial is shown to fit the experimental data. T he contributions of the dark counts, linear scattering and quadratic scattering are plotted separately as well. counting apparatus for detecting the signal and idler photons in coincidence. This apparatus is based on commercial InGaAs avalanche photodiodes operating in the gated Geiger mode.4 In the inset in Fig. 1, we show the number of scattered photons, NS, versus the number of pump photons, NP, injected into the NFSI. We fit the experimental data with a second-order polynomial fit, including the number of dark counts during the gate interval, ND. The fit clearly shows that the quadratic scattering ( ∝NP) in the fiber can dominate over the residual linear scattering ( ∝NP) of the pump, owing to imperfect filtering. The main body of Fig. 1 shows the coincidence-counting results. The diamonds represent the rate of coincidence counts versus the rate of the signal (idler) photons generated during the same pump pulse. The triangles represent the measured coincidence rate versus the signalphoton count rate when the signal is delayed with respect to the idler by one pulse period. For two independent photon sources, each with a count rate RS <<1, the accidental coincidence rate RC is given by RC = RS 2, regardless of the photon statistics of the sources. This quadratic relation is plotted as the solid line in Fig. 1, which fits the delayed-coincidence data (triangles) very well. These measurements show that while the fluorescence photons produced by the adjacent pump pulses are independent, those coming from the same pump pulse show a strong correlation, which is a signature of their non-classical behavior. This work was supported by the Department of Defense Multidisciplinary University Research Initiative program administered by the Army Research Office under Grants DAAD19-00-1-0177 and DAAD19-00-1-0469, and by the U.S. Office of Naval Research under Grant N00014-91-J-1268.

•Jan 1, 2002•5 citations
The correlations between photons generated by nonlinear optical processes offer advantages for many quantum technology applications, including spectroscopy, imaging, and metrology. Here, we use spontaneous four-wave mixing in a birefringent single-mode fiber pumped by a tunable pulsed laser as a broadly tunable source of phase-matched non-degenerate photon pairs for spectroscopy. The pairs are tunable such that the idler beam measures the transmittance spectrum of a sample in the near infrared, while the visible signal beam independently reports correlation information. By the time-resolved counting of both signal and idler photons, we use photon-number correlations to remove uncorrelated noise from the probe beam. Here, we have used heralded spectroscopy to measure the absorption spectrum of gallium arsenide near its band edge, despite the idler photon spectrum being dominated by a large background from spontaneous Raman scattering.
Quantum-correlated photon pairs with tunable wavelength are highly desirable in a number of quantum technologies. In this letter, we demonstrate a wavelength tunable source of the correlated photon pairs based on pulse-pumped spontaneous four-wave mixing in photonic-crystal fiber. The wavelengths of the correlated signal and idler photons can be continuously tuned at room temperature by adjusting the wavelength of pump originating from an ytterbium-doped fiber laser. The tuning range of the idler photons is 757-880 nm and the range of the signal photons is 1310-1610 nm, which covers the 1310- and 1550-nm telecom bands.
Abstract We report an experimental implementation of linear absorption spectroscopy using a fiber source of frequency-correlated photon pairs. The object under study is illuminated by a signal beam of a photon pair entangled in frequency. Due to the tight correlation of entangled photons, the absorption spectrum of the object can be measured from the idler beam, counting coincidences in both channels. The main advantages of ghost optics are analyzed, including significant noise reduction due to detecting only paired coincidences and cutting off all single background photons, as well as the potential sensitivity of studying samples, which is especially important when working with biological objects.
Optical quantum technologies such as quantum sensing, quantum cryptography and quantum computation all utilize properties of non-classical light, such as precise photon-number and entangled photon-pair states, to surpass technologies based on the classical light. A common route for obtaining heralded single photons is spontaneous four-wave mixing in optical fibers, allowing for a well-defined spatial mode, for high efficiency integration into optical fiber networks. These fibers are typically pumped using large, commercial, pulsed lasers requiring high-power (~10 W) pump lasers and are limited to ~MHz repetition rate. Here we propose a cost- efficient, compact and mobile alternative. Photon pairs at 660 nm and 960 nm will be created using four-wave mixing in commercial birefringent optical fiber, pumped using transform limited picosecond pulses with GHz repetition rates derived from a 785 nm CW laser diode using cavity-enhanced optical frequency comb generation. The pulses are predicted to have average power of 275 mW, a peak power of >40 W, and predicted photon yield of >2000 pairs detected per second. This design will be later utilized to implement a quantum illumination scheme based on a coincidence count between idler and signal photons -- instead of joint measurement between signal and idler. This will allow for quantum advantage over classic LIDAR without the requirement for maintaining an interferometric stability in free space.
We study the generation of photon pairs by spontaneous four-wave mixing (SFWM) in photonic crystal optical fibers. We show that it is possible to engineer two-photon states with specific spectral entanglement properties suitable for quantum information processing applica- tions. In this work, we concentrate on inner-loop phasematching, for which signal and idler photons can be generated at a small spectral separation from the pump, while sufficiently removed from the pump to ensure the absence of background photons produced by spontaneous Raman scattering. We present specific source designs which permit both symmetric and asymmetric factorable states, which allow herald- ing of pure-state, single-photon wavepackets without the need for spectral post-filtering. Additionally, we present numerical results for the conversion efficiency, where we compare sources based on inner- and outer-loop phasematching.
Q uantum entanglement refers to the nonclassical dependency of physically separated quantum systems. It is an essential resource that must be freely available for implementing many of the novel functions of quantum information processing, such as database searching, clock synchronization, teleportation, computing and cryptography.1 The efficient generation and transmission of quantum entanglement is therefore of prime importance. With the ubiquitous standard optical fiber serving as the transmission medium and the widespread availability of efficient active and passive fiber devices, technological synergy between the generation and propagation components of the overall quantum network can be achieved by deploying sources of entanglement that rely on the nonlinearity of the fiber itself. Such fiber-based sources of quantum entanglement would also have the advantage of modal purity over their crystal counterparts,2,3 which is very important for realizing complex networks that involve many quantum operations. In our quest to develop fiber-based devices for quantum information processing, we have recently demonstrated an allfiber source of quantum-correlated photon pairs.4 The operating physical mechanism in this source is nondegenerate fourphoton mixing, wherein two pump photons scatter through the Kerr nonlinearity of the fiber to create simultaneous signal and idler photons. Our experiment is conducted near the zero-dispersion wavelength of standard dispersion-shifted fiber, where such scattering is enhanced owing to phase matching of the photon wave functions. It must be pointed out here that in a conventional wavelength-divisionmultiplexed classical optical communication line, one strives to suppress the fourphoton or four-wave mixing process, which otherwise causes cross talk between the wavelength channels and sets limits on the total data capacity of the communication line. In our experiment, the four-photon mixing takes place in a nonlinear-fiber Sagnac interferometer (NFSI), which we previously used to generate quantum-correlated twin beams in the fiber.5 The pump is a mode-locked train of ~3-ps-long pulses. The pulsed operation serves two important purposes: the NFSI amplifier can be operated at low average powers and the production of the signal/ idler fluorescence photons is confined to well-defined temporal windows, allowing use of a gated detection scheme to increase the signal-to-noise ratio. To measure the nonclassical (i.e., quantum) correlations between the signal and the idler photons, one must effectively suppress the pump photons from reaching the detectors. Since a typical pump pulse contains ~108 photons and we are interested in detecting ~0.01 signal (idler) photons/pulse, a pump-to-signal (idler) rejection ratio in excess of 100 dB is required. We achieved this specification by sending the fluorescence photons through a free-space double-grating spectral filter that separates the signal and idler photons from each other and from the pump photons not rejected by the NFSI. To demonstrate the quantum nature of the four-photon scattering at the single photon level, we assembled a photonFigure 1.C oincidence rates as a function of the single-photon rates in two different cases: signalidler fluorescence produced by a pump pulse (diamonds) and signal-idler fluorescence produced by two consecutive pump pulses (triangles). T he line represents the calculated accidental counts. T he inset shows a plot of the detected idler photons as a function of the injected pump photons (hollow circles). A second-order polynomial is shown to fit the experimental data. T he contributions of the dark counts, linear scattering and quadratic scattering are plotted separately as well. counting apparatus for detecting the signal and idler photons in coincidence. This apparatus is based on commercial InGaAs avalanche photodiodes operating in the gated Geiger mode.4 In the inset in Fig. 1, we show the number of scattered photons, NS, versus the number of pump photons, NP, injected into the NFSI. We fit the experimental data with a second-order polynomial fit, including the number of dark counts during the gate interval, ND. The fit clearly shows that the quadratic scattering ( ∝NP) in the fiber can dominate over the residual linear scattering ( ∝NP) of the pump, owing to imperfect filtering. The main body of Fig. 1 shows the coincidence-counting results. The diamonds represent the rate of coincidence counts versus the rate of the signal (idler) photons generated during the same pump pulse. The triangles represent the measured coincidence rate versus the signalphoton count rate when the signal is delayed with respect to the idler by one pulse period. For two independent photon sources, each with a count rate RS <<1, the accidental coincidence rate RC is given by RC = RS 2, regardless of the photon statistics of the sources. This quadratic relation is plotted as the solid line in Fig. 1, which fits the delayed-coincidence data (triangles) very well. These measurements show that while the fluorescence photons produced by the adjacent pump pulses are independent, those coming from the same pump pulse show a strong correlation, which is a signature of their non-classical behavior. This work was supported by the Department of Defense Multidisciplinary University Research Initiative program administered by the Army Research Office under Grants DAAD19-00-1-0177 and DAAD19-00-1-0469, and by the U.S. Office of Naval Research under Grant N00014-91-J-1268.