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Scientific Reports

Generation of infrared photon pairs by spontaneous four-wave mixing in a CS2-filled microstructured optical fiber

Mina Afsharnia, Saher Junaid, Sina Saravi, Mario Chemnitz, Katrin Wondraczek, Thomas Pertsch, Markus Alexander Schmidt, Frank Setzpfandt

Published Jan 10, 2024• 15 citations
Publisher

Abstract

Abstract We experimentally demonstrate frequency non-degenerate photon-pair generation via spontaneous four-wave mixing from a novel CS 2 -filled microstructured optical fiber. CS 2 has high nonlinearity, narrow Raman lines, a broad transmission spectrum, and also has a large index contrast with the microstructured silica fiber. We can achieve phase matching over a large spectral range by tuning the pump wavelength, allowing the generation of idler photons in the infrared region, which is suitable for applications in quantum spectroscopy. Moreover, we demonstrate a coincidence-to-accidental ratio of larger than 90 and a pair generation efficiency of about $$10^{-2}$$ 10 - 2 per pump pulse, which shows the viability of this fiber-based platform as a photon-pair source for quantum technology applications.

DOI
10.1038/s41598-024-51482-0

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We report efficient generation of correlated photon pairs through degenerate four-wave mixing in a microstructure fiber. With 735.7 nm pump pulses producing correlated signal (688.5 nm) and idler (789.8 nm) photons in a 1.8 m microstructure fiber, we detect photon pairs at a rate of 37.6 kHz with a coincidence/ accidental contrast of 10:1 with deltalambda = 0.7 nm. This is the highest rate to our knowledge reported to date in a fiber-based photon source. The light source is highly nonclassical as defined by the Zou-Wang-Mandel inequality, which is violated by 1100 times the uncertainty.

Optics Letters•Dec 15, 2005•109 citations
Abstract We experimentally demonstrate frequency non-degenerate photon-pair generation via spontaneous four-wave mixing from a novel CS 2 -filled microstructured optical fiber. CS 2 has high nonlinearity, narrow Raman lines, a broad transmission spectrum, and also has a large index contrast with the microstructured silica fiber. We can achieve phase matching over a large spectral range by tuning the pump wavelength, allowing the generation of idler photons in the infrared region, which is suitable for applications in quantum spectroscopy. Moreover, we demonstrate a coincidence-to-accidental ratio of larger than 90 and a pair generation efficiency of about 10−210^{-2}10−2 10 - 2 per pump pulse, which shows the viability of this fiber-based platform as a photon-pair source for quantum technology applications.
Single photon sources are a key element for quantum computing, quantum key distribution (QKD) and quantum communications. In particular, producing single photons at telecommunications wavelengths is valuable for QKD protocols and would enable realizing the quantum internet. The preferred method for their generation has long been spontaneous down conversion in bulk crystals, which suffers from connection loss to fiber networks. In-fiber spontaneous four-wave mixing provides a viable alternative as a photon pair source due to being compatible with existing fiber networks. We present an all-fiber photon pair source based on degenerate four-wave mixing in a 400 m Highly-Nonlinear fiber, with signal and idler wavelengths generated at 1552.5 nm and 1557 nm respectively. The source consists of CW pump laser operating at 1554.75 nm, which is slightly detuned from the zero group velocity dispersion wavelength into the normal dispersion regime. After pair generation in the highly-nonlinear fiber, three arrayed waveguide gratings are employed to spatially separate signal and idler, and provides a 120 dB pump power reduction. Firstly the source is modelled and experimentally characterized in the well known classical regime of stimulated four-wave mixing. The effect of fiber cooling on spontaneous Raman scattering is modelled and characterized, and a 30% reduction in spontaneous emission is found when cooling the fiber to -77°C. In the low power regime the coincidence to accidental count ratio is simulated and measured. An increase in the coincidence to accidental count ratio is observed when cooling the fiber.
A continuous-wave (CW) photon-pair source operating in the L-band was successfully realized based on spontaneous four-wave mixing (SFWM) by using short length of a birefringent ZBLAN fiber. A type-III phase-matched SFWM process was utilized by pumping a birefringent ZBLAN fiber with pump photons polarized along the slow axis, where signal and idler photons were generated with polarizations aligned to the vertical axis of the birefringent ZBLAN fiber. The phase-matching curve was calculated, and the joint spectral intensity was analyzed under 1310 nm pumping conditions. Then, we experimentally generated signal and idler photons with center wavelengths of 1117 and 1578 nm using a 1310 nm CW laser as a pump light source and measured their quantum optical properties. The maximum coincidence-to-accidental ratio was calculated to be 22, resulting in a photon-pair brightness of 3.16 × 10 4 pairs/s/nm/mW. The results show the feasibility of using ZBLAN fibers in quantum optics as an efficient platform for generating a quantum light source.
Summary form only given. Single-photon sources are key components in applications of photonic quantum technologies such as quantum key distribution (QKD) [1]. One way of realizing single-photon sources is generation of photon pairs (PP) using spontaneous four-wave mixing (FWM): two photons from a pump p annihilate and create two side-band photons at frequencies determined partly by the energy conservation 2ωρ= ω1+ ω2, where ωp,ω1,ω2are the frequencies of the pump and the two side-bands, respectively, and partly by the phase-matching condition. PP generated spontaneously arrive at indeterministic times but even so, they are useful for QKD because one of the photons can be heralded by detecting the other. The heralded photons are then used for transmitting the quantum key.We propose a higher order mode scheme for generating PP in silica fibers; the side-band photons are generated at center wavelength λ1 = 810 nm in the linearly polarized LP02-mode and at λ2 = 1550 nm in the LP01mode, respectively, by pumping in the LP11-mode at λ7, = 1064 nm, where laser sources are readily available. The 810 nm photon is detectable with relatively cheap and efficient silicon-based single-photon detectors, and the heralded 1550 nm photon is mode-matched with transmission fibers in the low-loss spectral window. We design a silica fiber that phase matches these modes and wavelengths while it also reduces the impacts of core radius fluctuations (CRF) caused by fabrication imperfections; the fiber design is inspired by B. P.-P. Kuo et al. [3] and a sketch of the refractive index profile is shown in Fig. 1(a). The scalar wave equation is solved using appropriate Sellmeier data for Germanium-doped silica and the calculated effective indexes for the three modes versus wavelength are shown in Fig. 1(b) together with the core and cladding refractive indexes; the inset shows the wavelength configuration of the pump and two side-bands; phase matching is achieved when the effective indexes of the three modes lie on a straight line [2]. The nonlinear overlap of the waves in this configuration is approximately 18% of the corresponding overlap where all waves are in the LP01-mode.
We report efficient generation of correlated photon pairs through degenerate four-wave mixing in a microstructure fiber. With 735.7 nm pump pulses producing correlated signal (688.5 nm) and idler (789.8 nm) photons in a 1.8 m microstructure fiber, we detect photon pairs at a rate of 37.6 kHz with a coincidence/ accidental contrast of 10:1 with deltalambda = 0.7 nm. This is the highest rate to our knowledge reported to date in a fiber-based photon source. The light source is highly nonclassical as defined by the Zou-Wang-Mandel inequality, which is violated by 1100 times the uncertainty.