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Light force manipulation of gallium atoms

Steven J. Rehse, Lee, Siu Au, advisor, Menoni, Carmen, committee member, Lundeen, Stephen, committee member, Sites, James, committee member

Published Jan 1, 2002• 1 citation
Publisher

Abstract

We have demonstrated the first one-dimensional laser cooling of neutral gallium atoms. We identified the 4p2P3/2(F=3) → 4d2D5/2(F=4) transition at 294.45 nm as a cycling transition suitable for laser cooling. We developed a frequency stabilized tunable UV laser capable of generating over 90 mW for use at that wavelength. A careful spectroscopy of the hyperfine structure was performed on the 294.45 nm transition. This spectroscopy significantly improved the measurement of the Ga hyperfine constants and corrected existing errors in the literature.

DOI
10.25675/3.025730

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We have demonstrated the first one-dimensional laser cooling of neutral gallium atoms. We identified the 4p2P3/2(F=3) → 4d2D5/2(F=4) transition at 294.45 nm as a cycling transition suitable for laser cooling. We developed a frequency stabilized tunable UV laser capable of generating over 90 mW for use at that wavelength. A careful spectroscopy of the hyperfine structure was performed on the 294.45 nm transition. This spectroscopy significantly improved the measurement of the Ga hyperfine constants and corrected existing errors in the literature.
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Laser cooling experiments developed in the last decade enable physicists to slow down and spatially confine neutral atoms of a gas, thus lowering the temperature of trapped atoms into the μK range. One of the challenges associated with laser cooling is to stabilize a laser so that its output frequency matches that of a hyperfine structure transition and has an absolute stability of several MHz. In this project, we establish the groundwork for future laser cooling experiments with Rb by performing saturated-absorption Doppler-free spectroscopy studies. We acquire Doppler-free spectra of Rb that resolve individual hyperfine structure transitions, including the transition that the laser must excite in laser cooling experiments. The spectra we obtained can readily be repeated and the experimental apparatus can provide the feedback for an electronic laser stabilization circuit.
We have laser collimated a gallium atomic beam in one dimension using the linear-perpendicular-linear polarization gradient technique. Operating on the cycling $4{p}^{\phantom{\rule{0.2em}{0ex}}2}{P}_{3∕2}(F=3)\ensuremath{\rightarrow}4{d}^{\phantom{\rule{0.3em}{0ex}}2}{D}_{5∕2}(F=4)$ transition at 294.45nm294.45\phantom{\rule{0.3em}{0ex}}\text{nm}294.45nm, the full angular divergence of the atomic beam was reduced to 0.3mrad0.3\phantom{\rule{0.3em}{0ex}}\text{mrad}0.3mrad, corresponding to a transverse velocity of $\ifmmode\pm\else\textpm\fi{}11\phantom{\rule{0.3em}{0ex}}\text{cm}∕\mathrm{s}$, about one-half the Doppler cooling limit. The dependence of the cooling efficiency on the laser detuning and power was investigated. Optical pumping of the atoms out of the 4p2P3∕2(F=3)4{p}^{\phantom{\rule{0.2em}{0ex}}2}{P}_{3∕2}(F=3)4p2P3∕2​(F=3) state by the cooling laser was observed. Repumping schemes were investigated and found to successfully repopulate the cooled F=3F=3F=3 hyperfine state.
We perform laser spectroscopy of Yb+{}^{+}+ ions on the 4f146s2S1/2{f}^{14}6s{\phantom{\rule{0.16em}{0ex}}}^{2}\phantom{\rule{-0.16em}{0ex}}{S}_{1/2}f146s2S1/2​-4f135d6s4{f}^{13}5d6s4f135d6s 3D[3/2]1/2{}^{3}\phantom{\rule{-0.16em}{0ex}}D{[3/2]}_{1/2}3D[3/2]1/2​ transition at 297 nm. The frequency measurements for 170{}^{170}170Yb+{}^{+}+, 172{}^{172}172Yb+{}^{+}+, 174{}^{174}174Yb+{}^{+}+, and 176{}^{176}176Yb+{}^{+}+ reveal the specific mass shift as well as the field shifts. In addition, we demonstrate laser cooling of Yb+{}^{+}+ ions using this transition and show that light at 297 nm can be used as the second step in the photoionization of neutral Yb atoms.
The hyperfine transitions in the 399 nm ${^{1}S}_{0}\ensuremath{\leftrightarrow}{^{1}P}_{1}$ line in 173Yb^{173}\text{Y}\text{b}173Yb overlap with the transition in 172Yb^{172}\text{Y}\text{b}172Yb. We use transverse laser cooling on this line to selectively deflect 173Yb^{173}\text{Y}\text{b}173Yb atoms from a thermal beam containing both isotopes. We then use an acousto-optic modulator to span the frequency difference between the hyperfine transitions, and hence measure hyperfine structure in the 1P1{^{1}P}_{1}1P1​ state. Our precise values for the hyperfine constants, ${A}_{173}=57.693\ifmmode\pm\else\textpm\fi{}0.006\text{ }\text{MHz}$ and ${B}_{173}=609.028\ifmmode\pm\else\textpm\fi{}0.056\text{ }\text{MHz}$, improve previous values significantly.