Ultrafast Transient States in Nonequilibrium Quantum Systems

Bin Hwang, Jenni Portman, Edward Ersoy +1 more

Parvinder Solanki, Igor Lesanovsky, Gabriele Perfetto

D. S. Chemla, J.‐Y. Bigot

Herbert F. Fotso, James K. Freericks

Recent experimental advances in ultrafast phenomena have triggered renewed interest in the dynamics of correlated quantum systems away from equilibrium. We review nonequilibrium dynamical mean-field theory studies of both the transient and the steady states of a DC field-driven correlated quantum system. In particular, we focus on the nonequilibrium behavior and how it relates to the fluctuation-dissipation theorem. The fluctuation-dissipation theorem emerges as an indicator for how the system thermalizes and for how it reaches a steady state. When the system thermalizes in an infinite temperature steady state it can pass through a succession of quasi-thermal states that approximately obey the fluctuation-dissipation theorem. We also discuss the Wigner distribution and what its evolution tells us about the nonequilibrium many-body problem.

G. Flores-Hidalgo, Rudnei O. Ramos

Gusein Bedirkhanov, Nagamalleswararao Dasari, Alexander I. Lichtenstein +1 more

Recent advances in time-resolved spectroscopies have enabled direct access to the momentum-selective nonequilibrium dynamics of correlated quantum materials, revealing a strongly momentum-dependent response of electrons and collective excitations. Interpreting these observations requires a real-time theoretical framework that consistently captures the interplay between strong local electronic correlations and nonlocal collective fluctuations, a capability that remains beyond state-of-the-art nonequilibrium approaches. Using a recently developed real-time many-body framework, we resolve the momentum-selective ultrafast dynamics of a photoexcited correlated electron system. We predict a transient nodal-antinodal anisotropy in electronic heating, providing a microscopic explanation for the momentum-dependent response debated in time-resolved photoemission and Raman experiments, and identify the nonthermal spectral-weight transfer responsible for the transient antinodal in-gap states observed in ultrafast photoemission. We further uncover a momentum-selective magnetic response, in which antiferromagnetic fluctuations undergo a strongly nonthermal, quench-like excitation far above the electronic temperature while preserving their correlation length, before relaxing through a momentum-space magnon cascade toward lower-momentum modes. Finally, by tracking the real-time local spin susceptibility, we identify a dynamical, experimentally accessible signature of local-moment formation and its photoinduced melting. Our results establish a unified microscopic picture of ultrafast electronic and magnetic dynamics, providing a framework for interpreting momentum-resolved pump-probe experiments.