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EPJ Quantum Technology

Second-order effects in parametric-resonance magnetometers based on atomic alignment

François Beato, Agustin Palacios-Laloy

Published May 7, 2020• 17 citations
Publisher

Abstract

Abstract Optically-pumped magnetometers (OPM) based on parametric resonance allow real-time tri-axial measurement of very small magnetic fields with a single optical access to the gas cell. Most of these magnetometers rely on circularly polarized pumping light. We focus here on the ones relying on linearly polarized light, yielding atomic alignment. For these magnetometers we investigate three second order effects which appear in the usual regimes of operation, so to clarify if they translate to metrological problems like systematic errors or increased noise. The first of these effects is the breakdown of the three-step approach when the optical beam has a large intensity. The second one is the breakdown of the rotating wave approximation when the frequencies of the RF fields are not much larger than the rates of other atomic processes. The third one is the tensor light-shift which appears when the light is slightly detuned from resonance. This work should help to clarify the accuracy reachable with OPM, which is an important question notably for medical imaging applications.

DOI
10.1140/epjqt/s40507-020-00083-7

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Abstract Optically-pumped magnetometers (OPM) based on parametric resonance allow real-time tri-axial measurement of very small magnetic fields with a single optical access to the gas cell. Most of these magnetometers rely on circularly polarized pumping light. We focus here on the ones relying on linearly polarized light, yielding atomic alignment. For these magnetometers we investigate three second order effects which appear in the usual regimes of operation, so to clarify if they translate to metrological problems like systematic errors or increased noise. The first of these effects is the breakdown of the three-step approach when the optical beam has a large intensity. The second one is the breakdown of the rotating wave approximation when the frequencies of the RF fields are not much larger than the rates of other atomic processes. The third one is the tensor light-shift which appears when the light is slightly detuned from resonance. This work should help to clarify the accuracy reachable with OPM, which is an important question notably for medical imaging applications.
Optically pumped magnetometers usually rely on optical pumping using circularly or linearly polarized light. We study here zero-field magnetometers pumped with elliptically polarized light, preparing both atomic orientation and alignment with complementary geometries. We start by extending the three-step approach for elliptically polarized pumping. This allows us to study the Hanle effect in elliptical polarization by comparing the analytical absorption signals with experiments made on 4He^{4}\mathrm{He}4He metastable state. We then study parametric resonance magnetometers based on elliptical polarization by using the dressed-atom formalism with one and two radio-frequency fields. The results show good agreement with the experimental measurements and interesting perspectives for magnetometry where symmetry breaking by pumping light is mitigated.
In parametric-resonance magnetometers (PRMs), optically pumped atoms subject to rf fields allow one to measure the components of a very low magnetic field. Here, instead of using a circularly polarized light for creating atomic orientation, as in previous works, a linearly polarized light is used for creating atomic alignment. A dressed-atom formalism introduced by Polonsky and Cohen-Tannoudji is extended and allows one to map this situation to a simpler Hanle effect on aligned atoms. Analytical expressions for all alignment tensor components and photodetection signals are obtained for both the Hanle magnetometer and PRMs. A two-rf field alignment PRM is shown to display several improvements from its orientation counterpart, providing a secular third axis sensitivity and a lower degradation from the one-axis sensitivity obtained by using a single rf field. These specificities are shown to result from the apparent depolarization of the pumping light acting on the atom dressed by two-rf fields. Experimental measurements showing a good agreement with the theoretical predictions are presented.
Optically pumped magnetometers (OPMs) are revolutionizing the task of magnetic-field sensing due to their extremely high sensitivity combined with technological improvements in miniaturization which have led to compact and portable devices. OPMs can be based on spin-oriented or spin-aligned atomic ensembles which are spin polarized through optical pumping with circular or linear polarized light, respectively. Characterization of OPMs and the dynamical properties of their noise is important for applications in real-time sensing tasks. In our work, we experimentally perform spin noise spectroscopy of an alignment-based magnetometer. Moreover, we propose a stochastic model that predicts the noise power spectra exhibited by the device when, apart from the strong magnetic field responsible for the Larmor precession of the spin, white noise is applied in the perpendicular direction aligned with the pumping-probing beam. By varying the strength of the noise applied as well as the linear-polarization angle of incoming light, we verify the model to accurately predict the heights of the Larmor-induced spectral peaks and their corresponding linewidths. Our work paves the way for alignment-based magnetometers to become operational in real-time sensing tasks. Published by the American Physical Society 2024
Light shift arising from the circularly polarized pump beam in atomic magnetometers can induce an undesired magnetic response, and thus affect their accuracy. Here, the light shift and the corresponding cross-talk effect in the magnetometer have been investigated, and a scheme with an additional off-resonant pump beam with an appropriate polarization and intensity has been proposed to effectively reject the light shift. And the experimental results reproduce the expected behavior. This scheme provides a powerful tool to reject the light shift in optical pumping systems, in particular, the hybrid optically pumped systems.
Optically pumped magnetometers are important instruments for imaging biological magnetic signals without the need for cryogenic cooling. These magnetometers are presently available in the commercial market and utilize the principles of atomic alignment or orientation, enabling remarkable sensitivity and precision in the measurement of magnetic fields. This research focuses on utilizing a spin-aligned atomic ensemble for magnetometry at zero field. An approach is introduced which involves evaluating how the linear polarization of light rotates as it passes through the atomic vapor to null the magnetic field. Analytical expressions are derived for the resulting spin alignment and photodetection signals. Experimental results are provided, demonstrating good agreement with the theoretical predictions. The sensitivity and bandwidth of the magnetometer are characterized based on the detected polarization rotation signal. Lastly, the practical utility of the magnetometer for medical applications is demonstrated by successfully detecting a synthetic cardiac signal.
We report a laser-pumped 4He atomic magnetometer with light shift suppression through the atomic sensor itself. A linearly polarized light is used to optically align the 4He metastable atoms and we monitor the magneto-optical double resonance (MODR) signals produced by the left- and right-circularly orthogonal components. It is shown that light shift leads to the atomic alignment to orientation conversion effect, and thus, the difference between the two MODR signals. One of these two MODR signals is locked at the Larmor frequency and is used to measure the ambient magnetic field, while the differential signal is, simultaneously, fed back to suppress the light shift. The scheme could be of the advantage to the design of compact magnetometers by reducing the systematic errors due to light shift.