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SPIE Quantum Technologies

Dynamic Purcell-enhanced emission from erbium ions coupled to a microcavity (Conference Presentation)

Chetan Deshmukh, Bernardo Casabone, Hugues de Riedmatten, Diana Serrano, Shuping Liu, Alban Ferrier, Philippe Goldner, David Hunger

Published Apr 3, 2020• 0 citations
Publisher

Abstract

Single quantum emitters coupled to optical cavities in the Purcell regime can be used as high-efficiency spin-photon interfaces that are essential for building a quantum network. Furthermore, the dynamical control of the spontaneous emission rate of quantum emitters can have important implications in quantum technologies, e.g. for shaping the emitted photons waveform, or for driving coherently the optical transition while preventing photon emission. Here we demonstrate the dynamical Purcell-enhanced emission of a mesoscopic ensemble of erbium ions doped into nanocrystals coupled to a fully-tunable high-finesse fiber-based optical microcavity. Erbium has excellent optical and spin coherence properties at cryogenic temperatures and, in addition, has a transition in the telecom band that can facilitate integration into existing commercial telecom fibers. We show that we can tune the cavity on and out of resonance at a rate of above 8 KHz, which is two orders of magnitude faster that the natural lifetime of the erbium ions (55 Hz), and a factor of five faster than the Purcell enhanced emission (1.8 KHz). This allows us to shape in real time the Purcell enhanced emission of the ions and to achieve full control over the emitted photon’s waveforms. With moderate improvements in our detection efficiency and cavity finesse, this capability will allow for the generation of single telecom photons with controllable wave-shape from single erbium ions and for the realization of quantum processing between rare-earth ion qubits using dipolar interactions.

DOI
10.1117/12.2556282

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Single quantum emitters coupled to optical cavities in the Purcell regime can be used as high-efficiency spin-photon interfaces that are essential for building a quantum network. Furthermore, the dynamical control of the spontaneous emission rate of quantum emitters can have important implications in quantum technologies, e.g. for shaping the emitted photons waveform, or for driving coherently the optical transition while preventing photon emission. Here we demonstrate the dynamical Purcell-enhanced emission of a mesoscopic ensemble of erbium ions doped into nanocrystals coupled to a fully-tunable high-finesse fiber-based optical microcavity. Erbium has excellent optical and spin coherence properties at cryogenic temperatures and, in addition, has a transition in the telecom band that can facilitate integration into existing commercial telecom fibers. We show that we can tune the cavity on and out of resonance at a rate of above 8 KHz, which is two orders of magnitude faster that the natural lifetime of the erbium ions (55 Hz), and a factor of five faster than the Purcell enhanced emission (1.8 KHz). This allows us to shape in real time the Purcell enhanced emission of the ions and to achieve full control over the emitted photon’s waveforms. With moderate improvements in our detection efficiency and cavity finesse, this capability will allow for the generation of single telecom photons with controllable wave-shape from single erbium ions and for the realization of quantum processing between rare-earth ion qubits using dipolar interactions.
The interaction of single quantum emitters with an optical cavity enables the realization of efficient spin-photon interfaces, an essential resource for quantum networks. The dynamical control of the spontaneous emission rate of quantum emitters in cavities has important implications in quantum technologies, e.g., for shaping the emitted photons' waveform or for driving coherently the optical transition while preventing photon emission. Here we demonstrate the dynamical control of the Purcell enhanced emission of a small ensemble of erbium ions doped into a nanoparticle. By embedding the nanoparticles into a fully tunable high finesse fiber based optical microcavity, we demonstrate a median Purcell factor of 15 for the ensemble of ions. We also show that we can dynamically control the Purcell enhanced emission by tuning the cavity on and out of resonance, by controlling its length with sub-nanometer precision on a time scale more than two orders of magnitude faster than the natural lifetime of the erbium ions. This capability opens prospects for the realization of efficient nanoscale quantum interfaces between solid-state spins and single telecom photons with controllable waveform, for non-destructive detection of photonic qubits, and for the realization of quantum gates between rare-earth ion qubits coupled to an optical cavity.
Abstract The interaction of single quantum emitters with an optical cavity enables the realization of efficient spin-photon interfaces, an essential resource for quantum networks. The dynamical control of the spontaneous emission rate of quantum emitters in cavities has important implications in quantum technologies, e.g., for shaping the emitted photons’ waveform or for driving coherently the optical transition while preventing photon emission. Here we demonstrate the dynamical control of the Purcell enhanced emission of a small ensemble of erbium ions doped into a nanoparticle. By embedding the nanoparticles into a fully tunable high finesse fiber based optical microcavity, we demonstrate a median Purcell factor of 15 for the ensemble of ions. We also show that we can dynamically control the Purcell enhanced emission by tuning the cavity on and out of resonance, by controlling its length with sub-nanometer precision on a time scale more than two orders of magnitude faster than the natural lifetime of the erbium ions. This capability opens prospects for the realization of efficient nanoscale quantum interfaces between solid-state spins and single telecom photons with controllable waveform, for non-destructive detection of photonic qubits, and for the realization of quantum gates between rare-earth ion qubits coupled to an optical cavity.
Rare earth emitters enable critical quantum resources including spin qubits, single photon sources, and quantum memories. Yet, probing of single ions remains challenging due to low emission rate of their intra-4f optical transitions. One feasible approach is through Purcell-enhanced emission in optical cavities. The ability to modulate cavity-ion coupling in real-time will further elevate the capacity of such systems. Here, we demonstrate direct control of single ion emission by embedding erbium dopants in an electro-optically active photonic crystal cavity patterned from thin-film lithium niobate. Purcell factor over 170 enables single ion detection, which is verified by second-order autocorrelation measurement. Dynamic control of emission rate is realized by leveraging electro-optic tuning of resonance frequency. Using this feature, storage, and retrieval of single ion excitation is further demonstrated, without perturbing the emission characteristics. These results promise new opportunities for controllable single-photon sources and efficient spin-photon interfaces.
Erbium incorporated in a ceria (CeO2) host offers strong potential as a spin qubit platform, providing a pathway toward telecom-compatible quantum memory. But erbium is a dim emitter due to its long excited state lifetime. Methods to enhance its emission rate and efficiency through nanophotonic cavity integration are therefore essential. In this work, we demonstrate cavity-enhanced emission from erbium doped CeO2. We couple colloidally synthesized erbium doped CeO2 nanocrystals to a silicon nanobeam cavity and show a 30-fold improvement in emitter brightness combined with a 2-fold lifetime enhancement. We estimate a lower bound of 12 for the Purcell factor of cavity-coupled emitters after accounting for non-radiative decay. These results pave the way towards utilizing colloidally synthesized optically addressable spin qubits emitting at telecom wavelength for quantum networking and distributed quantum computing.
Many quantum information protocols require the storage and manipulation of information over long times, and its exchange between nodes of a quantum network across long distances. Implementing these protocols requires an advanced quantum hardware, featuring, for example, a register of long-lived and interacting qubits with an efficient optical interface in the telecommunication band. Here we present the Purcell-enhanced detection of single solid-state ions in erbium-doped nanoparticles placed in a fiber cavity, emitting photons at 1536 nm. The open-access design of the cavity allows for complete tunability in both space and frequency, selecting individual particles and ions. The ions are confined in a volume two orders of magnitude smaller than in previous realizations, increasing the probability of finding ions separated by only a few nanometers, which could then interact. We report the detection of individual spectral features presenting saturation of the emission count rate and linewidth, as expected for two-level systems. We also report an uncorrected g(2)(0) of 0.24(5) for the emitted field, confirming the presence of a single emitter. Our fully fiber-integrated system is an important step towards the realization of the initially envisioned quantum hardware.
Electro-optical control of on-chip photonic devices is an essential tool for efficient integrated photonics. Lithium niobate on insulator (LNOI) is an emerging platform for on-chip photonics due to its large electro-optic coefficient and high nonlinearity [1]. Integrating quantum emitters into LNOI would extend their versatile use in classic photonics to quantum computing and communication [2, 3]. Here, we incorporate single rare-earth ions (REI) quantum emitters in electro-optical tunable lithium niobite (LN) thin films and demonstrate control of LN microcavities coupled to REI over a frequency range of 160 GHz with 5 \mus switching speed. Dynamical control of the cavities enables the modulation of the Purcell enhancement of the REIs with short time constants. Using the Purcell enhancement, we show evidence of detecting single Yb3+ ions in LN cavities. Coupling quantum emitters in fast tunable photonic devices is an efficient method to shape the waveform of the emitter [4]. It also offers a platform to encode quantum information in the integration of a spectral-temporal-spatial domain to achieve high levels of channel multiplexing, as well as an approach to generate deterministic single-photon sources [5, 6].