Experiments in quantum optics are motivated by fundamental questions about the quantum mechanical description of matter and light as well as by applications in quantum technologies such as quantum information processing. Exploiting the quantum character of both matter and light has turned out to be extremely rewarding for novel technological applications in the emerging fields of quantum communication and computation. Here we consider the implementation of quantum information technology with trapped ions and single photons, focusing on two key issues: the entanglement of distant atoms and the controlled interaction of a single photon with a single atom.
This thesis describes the construction of a double ion trap apparatus including the necessary frequency-stabilized laser systems, and first experiments to investigate the generation of distant atomic entanglement, the implementation of a simple quantum network and controlled single-atom single-photon interaction. The experimental setup comprises two ion traps at a distance of one meter, which are independent but identical in construction. We introduce novel realizations of a photoionization method for calcium atoms, a laser frequency stabilization scheme and a radio frequency pulse sequencer. Linear Paul traps are used to load individual or strings of calcium ions. High-numerical aperture objectives mounted on sub-micrometer positioning systems allow us to address and manipulate a single ion with strongly focused light fields and collect the emitted fluorescence photons from a large solid angle. With these bidirectional single-atom single-photon interfaces the essential building blocks of a quantum network with atoms and photons are available. One of the main objectives we pursue with the double-trap apparatus is the generation of entanglement between ions in different traps, which is one of the key tasks in a quantum network. We compare single- and two-photon schemes for probabilistic entanglement creation and analyze how the performance of the schemes depends on photon detection efficiency. As a first step towards the experimental realization of such schemes we measure the second order correlation function of fluorescence photons emitted from two distant trapped ions. We observe high-contrast quantum (Hong-Ou-Mandel) interference, proving the indistinguishability of photons emitted from different ions, which is a prerequisite for the considered entanglement schemes. To investigate the interaction of single photons and a single atom in free space we combine the ion trap apparatus with a tunable, narrowband spontaneous parametric down-conversion source. The high-numerical aperture objectives allow us to efficiently couple bandwidth-tunable photons to a single trapped ion. Such atom-photon interaction at the single-particle level is the most fundamental process in quantum optics and lies literally at the focus of many experimental implementations of quantum information processing protocols and of studies of the (quantum) limits of matter -light interaction, which were so far restricted to weak coherent light fields. Here we observe individual atomic absorption events of one photon of an entangled pair by employing a quantum jump detection scheme. To characterize and control the interaction process we modify the spectral properties of the down conversion photons and perform single-photon spectroscopy of a single ion. To go beyond experiments with cohe rent fields we study temporal correlations between the absorption of photons from the spontaneous parametric down conversion source by a single ion and the detection of the corresponding partner photon.
For the applied scheme we observe promising indications that the quantum correlations of photons produced in spontaneous parametric down conversion are preserved in the resonant interaction with a single atom. The implementation of more efficient atom-light coupling and entanglement transfer schemes with our apparatus is outlined.
Experiments in quantum optics are motivated by fundamental questions about the quantum mechanical description of matter and light as well as by applications in quantum technologies such as quantum information processing. Exploiting the quantum character of both matter and light has turned out to be extremely rewarding for novel technological applications in the emerging fields of quantum communication and computation. Here we consider the implementation of quantum information technology with trapped ions and single photons, focusing on two key issues: the entanglement of distant atoms and the controlled interaction of a single photon with a single atom.
This thesis describes the construction of a double ion trap apparatus including the necessary frequency-stabilized laser systems, and first experiments to investigate the generation of distant atomic entanglement, the implementation of a simple quantum network and controlled single-atom single-photon interaction. The experimental setup comprises two ion traps at a distance of one meter, which are independent but identical in construction. We introduce novel realizations of a photoionization method for calcium atoms, a laser frequency stabilization scheme and a radio frequency pulse sequencer. Linear Paul traps are used to load individual or strings of calcium ions. High-numerical aperture objectives mounted on sub-micrometer positioning systems allow us to address and manipulate a single ion with strongly focused light fields and collect the emitted fluorescence photons from a large solid angle. With these bidirectional single-atom single-photon interfaces the essential building blocks of a quantum network with atoms and photons are available. One of the main objectives we pursue with the double-trap apparatus is the generation of entanglement between ions in different traps, which is one of the key tasks in a quantum network. We compare single- and two-photon schemes for probabilistic entanglement creation and analyze how the performance of the schemes depends on photon detection efficiency. As a first step towards the experimental realization of such schemes we measure the second order correlation function of fluorescence photons emitted from two distant trapped ions. We observe high-contrast quantum (Hong-Ou-Mandel) interference, proving the indistinguishability of photons emitted from different ions, which is a prerequisite for the considered entanglement schemes. To investigate the interaction of single photons and a single atom in free space we combine the ion trap apparatus with a tunable, narrowband spontaneous parametric down-conversion source. The high-numerical aperture objectives allow us to efficiently couple bandwidth-tunable photons to a single trapped ion. Such atom-photon interaction at the single-particle level is the most fundamental process in quantum optics and lies literally at the focus of many experimental implementations of quantum information processing protocols and of studies of the (quantum) limits of matter -light interaction, which were so far restricted to weak coherent light fields. Here we observe individual atomic absorption events of one photon of an entangled pair by employing a quantum jump detection scheme. To characterize and control the interaction process we modify the spectral properties of the down conversion photons and perform single-photon spectroscopy of a single ion. To go beyond experiments with cohe rent fields we study temporal correlations between the absorption of photons from the spontaneous parametric down conversion source by a single ion and the detection of the corresponding partner photon.
For the applied scheme we observe promising indications that the quantum correlations of photons produced in spontaneous parametric down conversion are preserved in the resonant interaction with a single atom. The implementation of more efficient atom-light coupling and entanglement transfer schemes with our apparatus is outlined.
Irhe field of quantum information processing (QIP) has evolved rapidly in the last decade. Strings of single rapped ions have proven to be one of the most promising candidates for the implementation of quantum information processing tasks such as universal gate operations or eleportation. Besides the challenge of scaling up these quantum processors to a larger number of ions, another important problem is to interconnect different processors on a macroscopic scale and integrate them into a quantum network. Irhis thesis describes the construction of a new experiment dedicated to the study of quantum communication and quantum networking with laser cooled single ions and first experiments carried out with it. Two linear Paul traps for 4DCa+ have been set up at a distance of one meter. Two-photon interference of the fluorescence light of two remotely trapped single ions could be observed with a contrast of 80%. This proves the suitability of the setup for the creation of remote entanglement, an important building block for quantum networking. Irhe first part of the thesis describes the experimental setup that ~as constructed from scratch. It consists of a newly designed trap apparatus and the laser setup. The apparatus was designed to ulfill the requirement of interferometric stability, which is a pre requisite for one remote entanglement protocol. Another important feature are two high numerical aperture in-vacuum lenses hat optimize the collection efficiency of photons scattered by he ions. In order to frequency-stabilize the laser systems, a ransfer stabilization scheme referenced to a transition in atomic ~s has been developed. The stabilization chain comprises low-cost open transfer cavities and offers very good long term stability. Irhe second part of the thesis presents the experimental results starting with the calibration of the two traps through excitation spectra. After that, the realization of two-photon interference rom single ions under continuous excitation is presented. The model analysis of the data usinq eiqht level Bloch equations reveals the individual coherence properties of the interfering ~ingle photons. The coherence time of the fluorescence light does not exceed 20- ns, indicating that incoherent scattering is ~ominant. fA,n analysis of the efficiency of methods for remote entanglement relying on two-photon and single-photon interference, focussing on he role of the detection efficiency is discussed. It is revealed hat Single-photon schemes are more efficient if the detection ~fficiency is low (like in present experiments). The created setup is suitable for the realization of both types of protocols, based pn single- and two-photon interference. Jhe conditioned dynamics of photon emission of a single ion are studied using correlation functions. The engineering of second ~rder correlation functions used as a tool which relies on conditional dynamics, might have interesting applications in probabilistic quantum information processing. pingle-atom single-photon interfaces are an important application in quantum networks. As opposed to the emission of single photons by single atoms, the absorption of Single photons by single atoms cannot be controlled in a similar way. With the future goal of realizing a heralded absorption of a single photon by a single atom, one of the ion traps was linked to a Spontaneous Parametric Down Conversion source. Quantum jump spectroscopy on a single ion using single photons from this source is shown. Finally the reported two-photon interference could be extended also to pulsed excitation. This marks an important technological step towards remote entanglement.
The interaction of single photons with single atoms is a fundamental process in quantum optics which manifests the quantum mechanical nature of light and matter. As an experimentally controlled process it enables the implementation of quantum technological applications, such as quantum information processing and quantum metrology. In the last decades, substantial progress has been attained to experimentally control and manipulate single atoms.
For example, single or multiple ions can be stored in an ion trap and their quantum states can be controlled with great precision. At the same time, experimental techniques to generate and control single photons and entangled photon pairs have been widely developed. However, only modest progress has been attained in controlling the interaction of single atoms with sin~le photons. The aim of this thesis project was to experimentally study he absorption of single photons and entangled photons pairs by single trapped DCa· ions. To this end, a source of polarization-entangled photon pairs based on the process of spontaneous parametric down-conversion (SPDC) was designed and constructed . Generating photon pairs whose interaction with an atom can be controlled imposed stringent requirements on the bandwidth, tunability, stability and brightness of the source, making its setup much more complex than usual SPDC sources. In a parallel project, a set of two separate ion traps were built, capable of storing a single or a set of a few 4DCa· ions.
he first part of the thesis documents the design, construction , operation and characterization of the entangled photon pair source. The characterization proves all the necessary requirements for the photons to interact with either of two transitions, D312 P312 and D5i2 P312 at 850 and 854 nm respectively, in 4DCa· One of the crucial requirements was to make the source bandwidth match the bandwidth of these transitions (22MHz). This was not straightforward since the typical emission bandwidths of the SPDC process is several orders of magnitude higher (1 05MHz). The ion trap setup is also briefly described. One of its crucial features is the inclusion of two high numerical-aperture objectives very close to the ion trap, allowing to enhance the interaction efficiency of the SPDC photons with the ion, and to efficiently collect the fluorescence light they emit. In a second part of the thesis, a concise description of the schemes and techniques used to detect the absorption of single photons by a single trapped ion is given, including a heoretical treatment of the methods used to analyze the data.
he core part of the thesis describes the methods used to couple the entangled photon source to one of the ion traps, and explains the results obtained with the combined setup. First it shows how the source is configured to produce heralded single photons. It then presents experiments in which the absorption by a single ion of photons produced by the source is detected, and how these absorption events are time-correlated with the detection of the heralding photon. These experiments are performed under several conditions, with a growing level of control over the interaction process. Finally, two proof-of-principle experiments are presented. In the first one, the ion is pumped to polarization-sensitive Zeeman substates and the polarization dependence of the correlated absorption rate is observed. This is a first step toward more advanced experiments in which the polarization entanglemen of the photon pairs is transferred to the entanglement of one photon with one atom or to two distant atoms. A second experiment performs heralded single photon spectroscopy on a single ion, showing the expected frequency dependence of the absorption process.
Finally, methods to extend these experiments to implement entanglement transfer from photons to atoms are outlined. In particular, it is shown how the efficiency of the source can be improved to make these experiments feasible.
Quantum networking is an established and growing field of research, with applications in many other fields of quantum technology, as well as fundamental research in quantum mechanics. A quantum network consists of multiple quantum devices that can interchange quantum information or be entangled with each other. Trapped ions coupled to optical cavities are among the most promising platforms in quantum technology broadly and networking specifically, with the ability to initialise and store quantum states in the ions and, via the cavity, transfer those states onto photons, which can interact with distant systems. This thesis describes two experiments using an ion trap with integrated high finesse optical cavity as a source of single photons. In the first, the photons were converted to a standard telecommunications wavelength through quantum frequency conversion and transmitted over 10 km of optical fibre. The attenuation experienced by the photons in optical fibre without frequency conversion would make transmission over such a long distance impractical. The converted photons were shown to maintain their nonclassical statistics, meaning such a system could be used to create quantum networks over long distances. A novel scheme for producing single photons from the ion-cavity system was demonstrated. This scheme significantly reduces the impact of decoherence in the system compared to commonly used schemes through selection of the initial state of the ion. This scheme may be directly applied to ion-photon entanglement and would lead to improved fidelity in ion-ion entanglement or state transfer. Both experiments represent significant steps towards the building of quantum networks based on ions coupled to optical cavities. They lay the groundwork for future experiments using the same system to entangle ions with photons and eventually with ions in other traps.
Long-range transport of quantum information across a network is most readily achieved through the use of photons as the information carriers. The nodes of such a quantum network are most naturally a quantum memory or information processor, which typically do not rely upon photonic qubits. Realizing a large-scale distributed quantum network therefore requires an efficient interface between the two physical manifestations of the quantum information. The most promising platform for realizing a quantum computer is the manipulation of trapped atomic ions, as this system has demonstrated all the fundamental requirements to realize a quantum computer. Additionally, trapped ions posses long coherence times necessary for quantum memories. The interface between atomic and photonic qubits relies on a high photon emission rate into the collected solid angle. Most methods of photon collection for quantum networks use a high numerical aperture microscope objective, which only collects on the order of 1% of all the emitted photons. This results in a small probability of successfully linking two quantum nodes. In this work, I present the design, simulation, and implementation of a trapped ion cavity QED system capable of improving the photon collection efficiency. A single ytterbium ion is coupled to a high-finesse optical cavity. The photon scatter rate into the cavity mode is enhanced by a factor of 130 over the free-space scatter rate into the cavity solid angle. This represents the first step towards realizing a protocol to entangle the polarization of an emitted photon to the Zeeman sublevels of the ion with high photon collection efficiency. Simulations of the experimental system indicate that with an optical cavity up to 4% of the light emitted by the ion can be collected.
Devices that harness the surprising properties of quantum systems at scale hold the possibility of revolutionary advances in information technology. Algorithms for quantum computers can take advantage of quantum parallelism to solve problems that are intractable with classical hardware, including prime factorization and simulating chemical processes. A quantum communication network that carries qubits instead of bits can leverage the irreversibility of projective measurement to guarantee secure communication. Because quantum states are fragile, building such devices requires exquisite control over many isolated quantum systems. One of the most critical capabilities is the interaction of stationary and flying qubits. In this thesis we consider how to engineer atom-light interactions as an interface for networked quantum systems. Quantum atom-light couplers require the efficient and reversible interaction of atomic and optical qubits, but the natural interaction of atoms and photons is weak. It is this very lack of interaction between light and its environment that makes light such an excellent carrier of quantum information. There are three promising strategies for stronger coherent atom-light interactions. First, the light field may be confined to a cavity so that it interacts with the atom over a longer time. Second, the light field may be focussed to a small spot with high aperture optics and matched to the natural atomic radiation pattern. Third, we may pass the light field through an ensemble of many atoms and store the qubit in a distributed state. In practice, atom-light couplers employ some combination of all three strategies. We will focus our research on the second two approaches: first by coupling one and two trapped ions with high aperture optics, and then operating a quantum optical memory with an ensemble of approximately 10 billion neutral atoms. Atoms that have been ionized and trapped in a common electromagnetic potential are an advanced few-qubit computation platform. Qubit states are associated with an electronic excitation at each atom, controlled coherently with lasers, and made to interact in two (or many) qubit gates by mutual Coulomb repulsion. One path to quantum advantage with ion-trap quantum processors is to scale small qubit registers by distributing entanglement with photonic interconnects. We consider the feasible efficiency of free-space atom-light couplers for atomic dipole transitions, and derive the atomic image by common free-space couplers. We couple a trapped-ion register with high-aperture lenses and operate a single trapped ion as a photon source. We model the dynamic character of the source and show spin-orbit coupling in the single-photon spatial mode. Although the total collection efficiency is only approximately 0.01, the source has exceptional photon-number purity A = (1.9 +/- 0:2) * 10^-3 such that the higher-order quantum nature of the field persists even after most of the field has been discarded. We derive an efficient quantum non-Gaussian witness and surpass it, the first such demonstration for a trapped-atom single-photon source. We entangle two trapped atoms by single-photon detection, and observe an interference pattern in the spatial mode of the bipartite state. Constructive interference between the entangled components enhances the emission probability by up to 29%, an example of collective enhancement by a two-atom ensemble. The efficiency of free-space atom-light couplers is limited by our capability to engineer high-precision, high-aperture optics. We fabricate ultra-precise hemispheric mirrors with numerical aperture 0.996 by single point diamond turning. The mirrors are amongst the smoothest hemispheric surfaces ever manufactured with root-mean-square (RMS) errors consistently below 25 nm. The smoothest of our mirrors has a RMS error of 14 nm and peak-to-valley error of 88 nm. A mirror with this surface is capable of suppressing or enhancing the spontaneous emission of an atom into free space by 96% in a proposed quantum electrodynamics experiment. We show how these mirrors, with a simple modification, can shape the spatial mode of a trapped atom by similar vacuum-mode engineering. We derive a near-hemispheric mirror coupling scheme that should be 72% efficient with mirrors as precise as ours. We design an ion trap for use with such high-aperture optics. With careful conditioning and control, ensembles of many atoms can be made to store and release photonic qubits on demand. Such optical quantum memories leverage the collective interaction of a light field with many billions of atoms to achieve storage and recall efficiencies approaching unity. We show how stationary light fields for photonic phase gates can be generated in optically deep ensembles, an effect which has since been observed. We implement the gradient echo memory (GEM) scheme in an ultra-high optical depth cold-atom ensemble. The performance of a practical quantum memory is contingent on the chosen qubit encoding. We extend the GEM protocol to allow the simultaneous storage of frequency separated signals and demonstrate that this `dual-rail' memory is suitable for high-fidelity frequency qubits. Dual-rail signals are recalled with 35% efficiency, 82% interference fringe visibility and 6 degrees of phase stability. We describe how the fidelity of the scheme is limited by frequency-dependent polarization rotation and how this may be addressed in an improved configuration. Finally, we demonstrate single-rail storage by GEM with 87% efficiency and 1 ms memory lifetime. Our memory surpasses the no-cloning limit for up to 600 us of storage, out-performing an optical fibre delay line by a factor of six. This is the first quantum memory to beat this important benchmark.
Trapped ion quantum networking aims at distributing quantum information between distant parties. Entanglement links between distant ions are mediated with photonic qubits, necessitating the need for efficient ion-photon interfaces. This thesis reports on progress towards improving the main limitations of creating a practical quantum network by using diffractive optics for high numerical aperture imaging of trapped ions. The diffractive optics are near-planar, patterned structures which are fabricated to collimate a large fraction of ion uorescence, with low aberration, for high resolution imaging. Patterning the central grounding electrode on a chip trap allows the ion to be within less than 100 microns of the surface. Large scale quantum networks will require a large number of ions and ion-photon interfaces. To scale the ion trap system, microfabricated surface traps can be used allowing for the opportunity to etch diffractive mirrors directly onto the trap surface. Collecting ion uorescence with the diffractive mirror, we show the highest ion-single mode optical fibre coupling efficiency, which enhances the entanglement rate of a quantum network. We then build a high resolution UV spectrometer to distinguish between frequency entangled photonic qubits. Frequency qubits offer more robust encoding when compared with polarisation qubits, as a result of energy conservation. Using the spectrometer we demonstrate correlations between the ion's internal state and the frequency state of an entangled photonic qubit. Quantum networks will require local quantum information processing using ion-ion gates to distribute entanglement over the entire network. Typically, the speed of these gates is presently limited to ~10 µs by the secular trap frequency. We demonstrate the first steps towards a fast ion-ion gate, not limited by the secular frequency, based on strong optical forces generated by the coherent, resonant absorption and stimulated emission of light from an ultrafast, pulsed laser. A full-scale quantum network will require many ion trap installations each with their own laser systems. For this challenge we demonstrate simple, robust, and cost-effective methods to lock the 399 nm photoionisation laser, based on polarisation spectroscopy through a hollow cathode lamp, and an opto-mechanical switch which allows locking of multiple lasers to a wavelength meter. Another scalable diffractive optic used is a phase Fresnel lens integrated into a 3D quadrupole ion trap system. The limits of imaging with this lens are tested by demonstrating force sensing at a sub-attoNewton level with super-resolution imaging techniques to find the ion location.