Devices that harness the surprising properties of quantum systems at scale hold the possibility of revolutionary advances in information technology. Algorithms for quantum computers can take advantage of quantum parallelism to solve problems that are intractable with classical hardware, including prime factorization and simulating chemical processes. A quantum communication network that carries qubits instead of bits can leverage the irreversibility of projective measurement to guarantee secure communication. Because quantum states are fragile, building such devices requires exquisite control over many isolated quantum systems. One of the most critical capabilities is the interaction of stationary and flying qubits. In this thesis we consider how to engineer atom-light interactions as an interface for networked quantum systems. Quantum atom-light couplers require the efficient and reversible interaction of atomic and optical qubits, but the natural interaction of atoms and photons is weak. It is this very lack of interaction between light and its environment that makes light such an excellent carrier of quantum information. There are three promising strategies for stronger coherent atom-light interactions. First, the light field may be confined to a cavity so that it interacts with the atom over a longer time. Second, the light field may be focussed to a small spot with high aperture optics and matched to the natural atomic radiation pattern. Third, we may pass the light field through an ensemble of many atoms and store the qubit in a distributed state. In practice, atom-light couplers employ some combination of all three strategies. We will focus our research on the second two approaches: first by coupling one and two trapped ions with high aperture optics, and then operating a quantum optical memory with an ensemble of approximately 10 billion neutral atoms. Atoms that have been ionized and trapped in a common electromagnetic potential are an advanced few-qubit computation platform. Qubit states are associated with an electronic excitation at each atom, controlled coherently with lasers, and made to interact in two (or many) qubit gates by mutual Coulomb repulsion. One path to quantum advantage with ion-trap quantum processors is to scale small qubit registers by distributing entanglement with photonic interconnects. We consider the feasible efficiency of free-space atom-light couplers for atomic dipole transitions, and derive the atomic image by common free-space couplers. We couple a trapped-ion register with high-aperture lenses and operate a single trapped ion as a photon source. We model the dynamic character of the source and show spin-orbit coupling in the single-photon spatial mode. Although the total collection efficiency is only approximately 0.01, the source has exceptional photon-number purity A = (1.9 +/- 0:2) * 10^-3 such that the higher-order quantum nature of the field persists even after most of the field has been discarded. We derive an efficient quantum non-Gaussian witness and surpass it, the first such demonstration for a trapped-atom single-photon source. We entangle two trapped atoms by single-photon detection, and observe an interference pattern in the spatial mode of the bipartite state. Constructive interference between the entangled components enhances the emission probability by up to 29%, an example of collective enhancement by a two-atom ensemble. The efficiency of free-space atom-light couplers is limited by our capability to engineer high-precision, high-aperture optics. We fabricate ultra-precise hemispheric mirrors with numerical aperture 0.996 by single point diamond turning. The mirrors are amongst the smoothest hemispheric surfaces ever manufactured with root-mean-square (RMS) errors consistently below 25 nm. The smoothest of our mirrors has a RMS error of 14 nm and peak-to-valley error of 88 nm. A mirror with this surface is capable of suppressing or enhancing the spontaneous emission of an atom into free space by 96% in a proposed quantum electrodynamics experiment. We show how these mirrors, with a simple modification, can shape the spatial mode of a trapped atom by similar vacuum-mode engineering. We derive a near-hemispheric mirror coupling scheme that should be 72% efficient with mirrors as precise as ours. We design an ion trap for use with such high-aperture optics. With careful conditioning and control, ensembles of many atoms can be made to store and release photonic qubits on demand. Such optical quantum memories leverage the collective interaction of a light field with many billions of atoms to achieve storage and recall efficiencies approaching unity. We show how stationary light fields for photonic phase gates can be generated in optically deep ensembles, an effect which has since been observed. We implement the gradient echo memory (GEM) scheme in an ultra-high optical depth cold-atom ensemble. The performance of a practical quantum memory is contingent on the chosen qubit encoding. We extend the GEM protocol to allow the simultaneous storage of frequency separated signals and demonstrate that this `dual-rail' memory is suitable for high-fidelity frequency qubits. Dual-rail signals are recalled with 35% efficiency, 82% interference fringe visibility and 6 degrees of phase stability. We describe how the fidelity of the scheme is limited by frequency-dependent polarization rotation and how this may be addressed in an improved configuration. Finally, we demonstrate single-rail storage by GEM with 87% efficiency and 1 ms memory lifetime. Our memory surpasses the no-cloning limit for up to 600 us of storage, out-performing an optical fibre delay line by a factor of six. This is the first quantum memory to beat this important benchmark.
The emergence of quantum physics from the page to the lab and the world at large is an exciting development of recent years. The prospects of absolutely secure communication and efficient simulation of physical systems have spurred great human effort into understanding these possibilities and turning them into realities. Photons are the most easily manipulated quantum particles and are a promising candidate for implementing these technologies. Limitations of photons include the difficulty of keeping objects that move at the speed of light, and producing strong interactions between particles that do not normally interact. The work presented in this thesis is motivated by the possibility of overcoming these limitations. The ability to faithfully store and reproduce a quantum state is essential for many quantum information technologies. Quantum memories for light have been developed over the last two decades to provide this ability. The group at the Australian National University developed the gradient echo memory (GEM): A quantum state of light can be controllably stored and released from an atomic ensemble by the use of additional optical fields and magnetic field gradients. This scheme was previously shown to preserve the quantum characteristics of the light. We used the GEM scheme with a cold rubidium ensemble to create the first optical memory that simultaneously beat the no-cloning limit, a benchmark for many of the technologies relying on quantum memories, and the loss rate for a delay line composed of optical fibre. We also created an analogue to a pulsed optical resonator using GEM with a warm rubidium vapour. This was done by replacing the circulating optical field of a resonator with light stored in the memory, and replacing the coupling of light into and out of that circulating mode with storage and recall from the memory. The bandwidth and repetition rate of this resonator were rapidly tunable as they were controlled by external optical and magnetic fields. We worked on implementing GEM with strings of thousands of atoms strongly coupled to the evanescent field of an optical nanofibre. This raised new possibilities for creating a true random access memory that would allow a more flexible use of the multi-mode capacity of GEM. We developed the theory for a novel type of stationary light in the gradient echo memory. Our stationary light scheme relies on the destructive interference of counter-propagating optical fields throughout the memory. The optical intensity scales with optical depth, as with other forms of stationary light. However, as the destructive interference could be set up over a much greater distance, more of the optical depth is available for generating stationary light. Finally, we studied how a control-phase gate for single-photon optical states could be implemented using a nonlinear interaction with stationary light. The stationary light generated by one state modulates the phase of another state stored in the memory. The second state modifies the stationary light, also producing a back-action on the first state and generating the required cross-phase shift.
Experiments in quantum optics are motivated by fundamental questions about the quantum mechanical description of matter and light as well as by applications in quantum technologies such as quantum information processing. Exploiting the quantum character of both matter and light has turned out to be extremely rewarding for novel technological applications in the emerging fields of quantum communication and computation. Here we consider the implementation of quantum information technology with trapped ions and single photons, focusing on two key issues: the entanglement of distant atoms and the controlled interaction of a single photon with a single atom.
This thesis describes the construction of a double ion trap apparatus including the necessary frequency-stabilized laser systems, and first experiments to investigate the generation of distant atomic entanglement, the implementation of a simple quantum network and controlled single-atom single-photon interaction. The experimental setup comprises two ion traps at a distance of one meter, which are independent but identical in construction. We introduce novel realizations of a photoionization method for calcium atoms, a laser frequency stabilization scheme and a radio frequency pulse sequencer. Linear Paul traps are used to load individual or strings of calcium ions. High-numerical aperture objectives mounted on sub-micrometer positioning systems allow us to address and manipulate a single ion with strongly focused light fields and collect the emitted fluorescence photons from a large solid angle. With these bidirectional single-atom single-photon interfaces the essential building blocks of a quantum network with atoms and photons are available. One of the main objectives we pursue with the double-trap apparatus is the generation of entanglement between ions in different traps, which is one of the key tasks in a quantum network. We compare single- and two-photon schemes for probabilistic entanglement creation and analyze how the performance of the schemes depends on photon detection efficiency. As a first step towards the experimental realization of such schemes we measure the second order correlation function of fluorescence photons emitted from two distant trapped ions. We observe high-contrast quantum (Hong-Ou-Mandel) interference, proving the indistinguishability of photons emitted from different ions, which is a prerequisite for the considered entanglement schemes. To investigate the interaction of single photons and a single atom in free space we combine the ion trap apparatus with a tunable, narrowband spontaneous parametric down-conversion source. The high-numerical aperture objectives allow us to efficiently couple bandwidth-tunable photons to a single trapped ion. Such atom-photon interaction at the single-particle level is the most fundamental process in quantum optics and lies literally at the focus of many experimental implementations of quantum information processing protocols and of studies of the (quantum) limits of matter -light interaction, which were so far restricted to weak coherent light fields. Here we observe individual atomic absorption events of one photon of an entangled pair by employing a quantum jump detection scheme. To characterize and control the interaction process we modify the spectral properties of the down conversion photons and perform single-photon spectroscopy of a single ion. To go beyond experiments with cohe rent fields we study temporal correlations between the absorption of photons from the spontaneous parametric down conversion source by a single ion and the detection of the corresponding partner photon.
For the applied scheme we observe promising indications that the quantum correlations of photons produced in spontaneous parametric down conversion are preserved in the resonant interaction with a single atom. The implementation of more efficient atom-light coupling and entanglement transfer schemes with our apparatus is outlined.
Recent experimental advances in preparing regular defect-free 2D arrays of atoms with optical traps have offered new opportunities to engineer strong collective couplings between light and atoms as quantum optical dipoles. Applications of such collective light-matter interactions include the realization of atom-thick mirrors, retrieval of quantum memories with high efficiency, or the implementation of topological quantum optics. I will present novel applications in the context of quantum networking. First, I will discuss the design of a chiral photonic quantum link, where distant single atoms interact by exchanging photons propagating in a unique direction in free space. This is achieved by coupling both single atoms, representing qubits implemented using a pair of Rydberg states, to bi-layer atomic arrays which act as quantum phased-array antennas. Exploiting the combination of a “Rydberg-dressing” laser and a control laser driving the atomic arrays, an effective Rydberg dipole-dipole interaction can be engineered between atoms and atomic arrays as quantum emitters, allowing to match the spatial modes of spontaneously emitted and absorbed photons to a Gaussian mode of interest. In this way, we realize a chiral quantum interface, i.e., where atoms couple to photonic modes with a unique direction of propagation. This setup provides a basic building block of a novel platform for quantum networks in free space, i.e., without requiring coupling atoms to modes of cavities or nanostructures, which I will illustrate with the deterministic coherent transfer of quantum states between single atoms with high fidelity. Second, I will discuss the collective radiation properties of two distant single-layer atomic arrays acting as quantum memories. This system can support a long-lived non-local superposition state of atomic excitations exhibiting strong subradiance. This “dark” mode consists of an atomic excitation which is delocalized between the two distant atomic arrays, in such a way that the overall radiation is strongly suppressed by quantum interference. I will describe the preparation of these states and their application as resource of non-local entanglement. In particular, by weakly driving the arrays, the state of the quantum memories, localized in each array, can be transferred to this “non-local” subradiant state, allowing again for a deterministic coherent quantum state transfer with high fidelity between the memories. Finally, I will discuss experimental realizations using cold atoms in optical trap arrays, and the effect of experimental imperfections in the arrays, such as finite defect probability, temperature, and depth of the optical traps.
A leading strategy for the creation of a scalable quantum computer is through a networked architecture. This would comprise stationary nodes for quantum information processing and photonic channels for their communication and entanglement distribution. In this scheme a coherent interface between light and matter is a critical component, facilitating the deterministic and reversible transfer of quantum information between stationary and travelling qubits. This requirement may be fulfilled by a high finesse optical cavity, whose radiation field is strongly coupled to a trapped quantised emitter. Neutral atoms are an ideal species for the development of such a device, given their inherent compatibility with dielectric mirror surfaces. However, an outstanding challenge in building an elementary network of neutral atom-cavity systems is in establishing a single atom dipole trap within each cavity mode. This thesis presents the development of an open-access cavity suitable for single atom localisation, whilst maintaining strong atom-cavity coupling, {g0,κ,γ} = {11,2.1,3} × 2πMHz, and the efficient extraction of generated photons, η=0.5. We consider cavity design methodology, deriving a connection between the physical properties of the optical resonator and its intended role in the production of single photons. An experimental platform is developed for the creation of cavity mirrors by laser ablation, with a high degree of geometrical control. This is used to produce a set of pyramidal micro-mirrors, demonstrated to represent a favourable alternative to the widespread adoption of fibre-tip cavities. These pyramidal mirrors are shown to support multi-feature resonators, allowing several atom-cavity interfaces to be formed using a pair of substrates. By developing a novel procedure for mirror alignment, a hybrid mirror cavity is fabricated and integrated into an experimental architecture tailored for atomic trapping. Suitability of the cavity for future experimentation is demonstrated by frequency stabilisation to an atomic resonance of 87Rb.
Long-range transport of quantum information across a network is most readily achieved through the use of photons as the information carriers. The nodes of such a quantum network are most naturally a quantum memory or information processor, which typically do not rely upon photonic qubits. Realizing a large-scale distributed quantum network therefore requires an efficient interface between the two physical manifestations of the quantum information. The most promising platform for realizing a quantum computer is the manipulation of trapped atomic ions, as this system has demonstrated all the fundamental requirements to realize a quantum computer. Additionally, trapped ions posses long coherence times necessary for quantum memories. The interface between atomic and photonic qubits relies on a high photon emission rate into the collected solid angle. Most methods of photon collection for quantum networks use a high numerical aperture microscope objective, which only collects on the order of 1% of all the emitted photons. This results in a small probability of successfully linking two quantum nodes. In this work, I present the design, simulation, and implementation of a trapped ion cavity QED system capable of improving the photon collection efficiency. A single ytterbium ion is coupled to a high-finesse optical cavity. The photon scatter rate into the cavity mode is enhanced by a factor of 130 over the free-space scatter rate into the cavity solid angle. This represents the first step towards realizing a protocol to entangle the polarization of an emitted photon to the Zeeman sublevels of the ion with high photon collection efficiency. Simulations of the experimental system indicate that with an optical cavity up to 4% of the light emitted by the ion can be collected.
The power of quantum computation derives from algorithmic methods that exploit the availability of quantum superposition and entanglement to perform computations that are intractable with classical devices. The race is on to develop hardware that will unleash the promise of quantum algorithms. A handful of different types of hardware are currently being developed with the greatest efforts directed at superconducting, quantum-dot, trapped-ion, photonic, and neutral-atom approaches [1]. While all approaches have strengths and weaknesses, and are at different stages of development, the challenge of creating a practical design that can be scaled to a million or more qubits has not yet been met with any of the existing platforms. One may wonder if we really need a million qubits for a useful quantum computer. The answer depends on our ambition level. On the one hand it is widely believed that a quantum computer with less than 100 reliable qubits will be able to demonstrate a quantum advantage for a well defined computational problem [2]. Demonstration of a quantum computational advantage will generate great excitement in the halls of academia, but will have little broader import. A problem of great practical interest such as ab initio design of chemicals for increasing the yield of fertilizers for crop production, to name but one example, may also require just a few hundred qubits, provided computational sequences with circuit depth of 1010 or more operations can be reliably performed [3]. However, given the current performance of qubit hardware, which has demonstrated error rates not less than ∼10−3, computations with depth 1010 will only produce random outcomes of negligible value. The solution lies in the construction of error-correction circuitry operating on logical qubits, each composed of many physical qubits, which will enable logical error rates many orders of magnitude smaller than physical error rates. Although error correction is remarkably efficient for classical computing devices—Hamming codes detect and correct errors while only requiring roughly 10% overhead in the number of physical bits—quantum error correction is notoriously expensive. New approaches to error correction are the subject of intensive research with one promising direction being the development of codes that are optimized to suppress the dominant error mechanism in a particular physical platform [4,5]. Nevertheless, with physical error rates of 10−4, a plausible target for current qubit systems, the overhead required to reach logical error rates of 10−10 may be measured in thousands of physical qubits for each logical qubit. Thus a quantum computer able to perform deep calculations on a few hundred logical qubits could require a million physical qubits. A consequence of the cost of quantum error correction is that any viable approach to large-scale quantum computing needs to combine high-fidelity quantum logic operations with a capability for integrating large numbers of physical qubits. From this perspective neutral-atom qubits appear particularly promising [6] as they have already demonstrated control of more qubits than any other platform with recent experiments in 1D [7], 2D [8,9], and 3D [10] geometries showing control of up to 50 atomic qubits. Large qubit arrays can potentially be prepared in 1D, 2D, or 3D geometries. The number of proximal qubits increases with the dimensionality, which is advantageous for implementation of error correction code words, and points towards a preference for 2D or 3D arrays. On the other hand, the added overhead of compensating crosstalk incurred when targeting atoms inside a 3D volume makes parallel operations on multiple qubits challenging. A 2D geometry, as shown schematically in Fig. 1, may be an optimal choice since qubit control and measurement can be performed with lasers propagating normal to the plane of the array so that individual qubit sites can be addressed independently. With demonstrated array periods of a few micrometers we require a footprint of less than 1 mm2 for 104 qubits. Conceptual picture of a 2D neutral-atom qubit array. a) High-numerical-aperture lenses project several different wavelengths of light for control and measurement of the qubits. Specific choices of optical wavelengths depend on the atomic species. Not shown are optics for initial laser cooling, transport to the array, beam scanning, and imaging for qubit measurement. b) Averaged fluorescence image of 49 atomic qubits on a 2D grid with |
3.8μm| spacing [8]. From a fundamental perspective the prospects for scaling neutral-atom systems are particularly promising due to the exceptionally large ratio between coherent and incoherent coupling rates. Neutral-atom qubits are encoded in hyperfine ground states for which coherence times of the order of 10 s have been demonstrated [10]. This implies a dephasing rate |
γ∼0.1s−1|. The coherent coupling that enables quantum logic operations is switched on by exciting atoms to high-lying Rydberg states with principal quantum number close to 100 [11,12]. Rydberg excited atoms at spacings of a few micrometers in an optical lattice interact coherently with rates |
g>109s−1|. The ratio between desired coherent coupling and residual incoherent dephasing of g/γ ∼ 1010 establishes a figure of merit that is enabling for scalability. To our knowledge only trapped ions can claim a similar g/γ ratio [13], but without a correspondingly direct path towards controlling thousands of qubits in a single processing unit. Although the g/γ ratio is exceptionally favorable for neutral-atom qubits a complete set of universal gate operations has not yet been demonstrated with high fidelity. Single-qubit gates in large 2D and 3D arrays have reached fidelity |
F∼0.999| [8,10]. However, the highest demonstrated fidelity for two-qubit entanglement mediated by Rydberg-state interactions is |
F<0.8| [6,14,15], a value that is well short of the theoretical limit of |
F>0.9999| [16,17]. There is healthy optimism within the research community working with neutral-atom qubits that combining improved laser sources with reduced noise, better cooling to reduce motional dephasing, and control of stray electric fields that perturb Rydberg atoms will lead to substantially improved gate fidelity in the near future. Recent results with better filtering of laser phase noise have already demonstrated remarkable improvement in ground–Rydberg entanglement [18]. The outlook for the next few years appears very promising. We anticipate that with advances in lasers, optical lattices for atom trapping, deterministic rearrangement and loading of atoms in multi-dimensional arrays [19,20], and optics for fast beam scanning it will be possible to increase the number of physical qubits in a single neutral-atom module to at least 104. A challenging yet plausible path to a million-qubit processor can then be contemplated by connecting 100 such modules with atom–photon entanglement channels [21]. Beyond the potential for advancing the state of the art in computation, development of techniques for single-atom control inside large multi-atom arrays will enable other applications of quantum science including metrology and time-keeping. Rydberg interactions that are at the heart of a neutral-atom quantum computer may lead to multi-atom entanglement and Heisenberg scaling of atomic-clock precision [22]. This work was supported by the NSF and ARL CDQI.