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Single photons from a trapped-ion cavity-QED system

Thomas Walker

Published Mar 18, 2021• 0 citations
OpenAlex

Abstract

Quantum networking is an established and growing field of research, with applications in many other fields of quantum technology, as well as fundamental research in quantum mechanics. A quantum network consists of multiple quantum devices that can interchange quantum information or be entangled with each other. Trapped ions coupled to optical cavities are among the most promising platforms in quantum technology broadly and networking specifically, with the ability to initialise and store quantum states in the ions and, via the cavity, transfer those states onto photons, which can interact with distant systems. This thesis describes two experiments using an ion trap with integrated high finesse optical cavity as a source of single photons. In the first, the photons were converted to a standard telecommunications wavelength through quantum frequency conversion and transmitted over 10 km of optical fibre. The attenuation experienced by the photons in optical fibre without frequency conversion would make transmission over such a long distance impractical. The converted photons were shown to maintain their nonclassical statistics, meaning such a system could be used to create quantum networks over long distances. A novel scheme for producing single photons from the ion-cavity system was demonstrated. This scheme significantly reduces the impact of decoherence in the system compared to commonly used schemes through selection of the initial state of the ion. This scheme may be directly applied to ion-photon entanglement and would lead to improved fidelity in ion-ion entanglement or state transfer. Both experiments represent significant steps towards the building of quantum networks based on ions coupled to optical cavities. They lay the groundwork for future experiments using the same system to entangle ions with photons and eventually with ions in other traps.

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Experiments in quantum optics are motivated by fundamental questions about the quantum mechanical description of matter and light as well as by applications in quantum technologies such as quantum information processing. Exploiting the quantum character of both matter and light has turned out to be extremely rewarding for novel technological applications in the emerging fields of quantum communication and computation. Here we consider the implementation of quantum information technology with trapped ions and single photons, focusing on two key issues: the entanglement of distant atoms and the controlled interaction of a single photon with a single atom. This thesis describes the construction of a double ion trap apparatus including the necessary frequency-stabilized laser systems, and first experiments to investigate the generation of distant atomic entanglement, the implementation of a simple quantum network and controlled single-atom single-photon interaction. The experimental setup comprises two ion traps at a distance of one meter, which are independent but identical in construction. We introduce novel realizations of a photoionization method for calcium atoms, a laser frequency stabilization scheme and a radio frequency pulse sequencer. Linear Paul traps are used to load individual or strings of calcium ions. High-numerical aperture objectives mounted on sub-micrometer positioning systems allow us to address and manipulate a single ion with strongly focused light fields and collect the emitted fluorescence photons from a large solid angle. With these bidirectional single-atom single-photon interfaces the essential building blocks of a quantum network with atoms and photons are available. One of the main objectives we pursue with the double-trap apparatus is the generation of entanglement between ions in different traps, which is one of the key tasks in a quantum network. We compare single- and two-photon schemes for probabilistic entanglement creation and analyze how the performance of the schemes depends on photon detection efficiency. As a first step towards the experimental realization of such schemes we measure the second order correlation function of fluorescence photons emitted from two distant trapped ions. We observe high-contrast quantum (Hong-Ou-Mandel) interference, proving the indistinguishability of photons emitted from different ions, which is a prerequisite for the considered entanglement schemes. To investigate the interaction of single photons and a single atom in free space we combine the ion trap apparatus with a tunable, narrowband spontaneous parametric down-conversion source. The high-numerical aperture objectives allow us to efficiently couple bandwidth-tunable photons to a single trapped ion. Such atom-photon interaction at the single-particle level is the most fundamental process in quantum optics and lies literally at the focus of many experimental implementations of quantum information processing protocols and of studies of the (quantum) limits of matter -light interaction, which were so far restricted to weak coherent light fields. Here we observe individual atomic absorption events of one photon of an entangled pair by employing a quantum jump detection scheme. To characterize and control the interaction process we modify the spectral properties of the down conversion photons and perform single-photon spectroscopy of a single ion. To go beyond experiments with cohe rent fields we study temporal correlations between the absorption of photons from the spontaneous parametric down conversion source by a single ion and the detection of the corresponding partner photon. For the applied scheme we observe promising indications that the quantum correlations of photons produced in spontaneous parametric down conversion are preserved in the resonant interaction with a single atom. The implementation of more efficient atom-light coupling and entanglement transfer schemes with our apparatus is outlined.

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Trapped ions are a promising platform for local quantum information processing. In order to distribute this quantum information over long distances, we can take advantage of optical cavities, which ofier a coherent interface between matter and light, enabling the transfer of quantum information from stationary qubits such as ions onto photons. We demonstrate such an interface by coupling trapped ions to a cavity and have recently shown that a quantum state can be faithfully transferred from a single ion onto a single photon. In particular, this transfer can be improved by taking advantage of a collective effect between multiple ions, namely, superradiant emission into the cavity. In this proof-of-principle experiment, we tune the phase of a two-ion entangled state between sub- and superradiance. The superradiant coupling is then used to enhance the transfer of quantum information onto a photon from a logical qubit encoded in the two ions. Finally, prospects for linking together distant ions in cavities via a quantum network are discussed. Toward this goal, we outline a fiber-based ion-cavity experiment which allows access to the single-ion strong-coupling regime.

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Single ion coupled to a high-finesse optical fibre cavity for cQED in the strong coupling regime

Ezra Kassa

The research undertaken unites two distinct areas of quantum information processing: single ions stored in radio-frequency traps and single photons in optical fibres. Strings of ions are presently the most successful implementation of quantum computing, with elementary quantum algorithm and quantum simulations realised. The principal challenge in the field is to enhance the quantum processing power by scaling up current devices to larger systems. We pursue one of the most promising strategies: distributed quantum computation in which multiple small-scale ion processors are interlinked by exchanging photonic quantum bits via optical fibres. This requires a coherent quantum interface between ions and photons, mapping ionic to photonic quantum states and vice versa. To maximise fidelity and the success rate of the scheme, the interaction of ions and photons must take place in a microscopic optical cavity with high finesse. To this end, single 40Ca+ were trapped in a radio-frequency ion trap whose trapping electrodes are hollow cylinders. Optical fibres with mirrors machined on the facets are inserted into the electrodes to form a Fabry-Pérot cavity. Because the fibres are shielded by the electrodes the detrimental distortion of the trapping field due to their presence is suppressed and ions can be trapped for several hours. 40Ca+ has a -type energy level scheme wherein the ion is cooled on the 42P1/2 ? 42S1/2 transition and the cavity is tuned to the 42P1/2 ? 32D3/2 transition. This thesis reports the successful coupling of single ions to a high finesse optical fibre based cavity, with coupling strength g = 2p · 4:6 MHz. The cavity has length 367 µm, finesse of 40,000 and linewidth 2k = 2p · 9:4 MHz. In this coupling regime, the enhancement of the ion's emission rate through the Purcell effect was observed. Further, anti-correlation was observed in the emission rates between the P1/2 ? D3/2 and P1/2 ? S1/2 transitions with an effective emission rate suppression of up to 60% in the latter transition. The built system offers greater promises. Once the position in the cavity mode has been optimised we expect to reach the long-sought after strong coupling regime with (g, k, y) = 2p · (12:2; 4:7; 11:2) MHz.

•Jul 12, 2017•1 citation

Toward coherent ion-cavity coupling

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Entanglement is an established resource in quantum information processing, and there is a clear imperative to study many-body systems both in quantum technology applications and for probing fundamental physical laws. Ion trap cavity quantum electrodynamics is a highly promising platform for research. Prerequisites are the controlled coupling of many ions to the cavity field along with the ability to initialize the quantum states and drive coherent transitions between them. A coaxial ion trap and high finesse cavity system has been shown to couple strings of up to five ions to the cavity mode with nearly optimal coupling strength thanks to precise control over their positions in the standing wave and their mutual Coulomb interaction. The predictive power of the theoretical model demonstrates that the scheme can be extended to more ions or to higher coupling regimes. In a separate experiment it has been demonstrated that a quantum state can be initialized, before coherently transferring the population to a qubit state through the cavity interaction. The emission of polarized photons in the cavity mode has been measured, taking the system closer to the generation of cluster states for quantum information research and fundamental studies in many-body entanglement. Building on the aforementioned work, an infrastructure has been put in place for the direct observation of vacuum Rabi oscillations between a single ion and the cavity. In this scheme, the contribution to the dynamics from the dominant incoherent channel is minimized through post-selection of the data. As a quantum system coupled to a reservoir with memory, it will provide experimental constraints on theoretical work in the field of non-Markovian dynamics.

•May 22, 2017•0 citations
Quantum networking is an established and growing field of research, with applications in many other fields of quantum technology, as well as fundamental research in quantum mechanics. A quantum network consists of multiple quantum devices that can interchange quantum information or be entangled with each other. Trapped ions coupled to optical cavities are among the most promising platforms in quantum technology broadly and networking specifically, with the ability to initialise and store quantum states in the ions and, via the cavity, transfer those states onto photons, which can interact with distant systems. This thesis describes two experiments using an ion trap with integrated high finesse optical cavity as a source of single photons. In the first, the photons were converted to a standard telecommunications wavelength through quantum frequency conversion and transmitted over 10 km of optical fibre. The attenuation experienced by the photons in optical fibre without frequency conversion would make transmission over such a long distance impractical. The converted photons were shown to maintain their nonclassical statistics, meaning such a system could be used to create quantum networks over long distances. A novel scheme for producing single photons from the ion-cavity system was demonstrated. This scheme significantly reduces the impact of decoherence in the system compared to commonly used schemes through selection of the initial state of the ion. This scheme may be directly applied to ion-photon entanglement and would lead to improved fidelity in ion-ion entanglement or state transfer. Both experiments represent significant steps towards the building of quantum networks based on ions coupled to optical cavities. They lay the groundwork for future experiments using the same system to entangle ions with photons and eventually with ions in other traps.
Experiments in quantum optics are motivated by fundamental questions about the quantum mechanical description of matter and light as well as by applications in quantum technologies such as quantum information processing. Exploiting the quantum character of both matter and light has turned out to be extremely rewarding for novel technological applications in the emerging fields of quantum communication and computation. Here we consider the implementation of quantum information technology with trapped ions and single photons, focusing on two key issues: the entanglement of distant atoms and the controlled interaction of a single photon with a single atom. This thesis describes the construction of a double ion trap apparatus including the necessary frequency-stabilized laser systems, and first experiments to investigate the generation of distant atomic entanglement, the implementation of a simple quantum network and controlled single-atom single-photon interaction. The experimental setup comprises two ion traps at a distance of one meter, which are independent but identical in construction. We introduce novel realizations of a photoionization method for calcium atoms, a laser frequency stabilization scheme and a radio frequency pulse sequencer. Linear Paul traps are used to load individual or strings of calcium ions. High-numerical aperture objectives mounted on sub-micrometer positioning systems allow us to address and manipulate a single ion with strongly focused light fields and collect the emitted fluorescence photons from a large solid angle. With these bidirectional single-atom single-photon interfaces the essential building blocks of a quantum network with atoms and photons are available. One of the main objectives we pursue with the double-trap apparatus is the generation of entanglement between ions in different traps, which is one of the key tasks in a quantum network. We compare single- and two-photon schemes for probabilistic entanglement creation and analyze how the performance of the schemes depends on photon detection efficiency. As a first step towards the experimental realization of such schemes we measure the second order correlation function of fluorescence photons emitted from two distant trapped ions. We observe high-contrast quantum (Hong-Ou-Mandel) interference, proving the indistinguishability of photons emitted from different ions, which is a prerequisite for the considered entanglement schemes. To investigate the interaction of single photons and a single atom in free space we combine the ion trap apparatus with a tunable, narrowband spontaneous parametric down-conversion source. The high-numerical aperture objectives allow us to efficiently couple bandwidth-tunable photons to a single trapped ion. Such atom-photon interaction at the single-particle level is the most fundamental process in quantum optics and lies literally at the focus of many experimental implementations of quantum information processing protocols and of studies of the (quantum) limits of matter -light interaction, which were so far restricted to weak coherent light fields. Here we observe individual atomic absorption events of one photon of an entangled pair by employing a quantum jump detection scheme. To characterize and control the interaction process we modify the spectral properties of the down conversion photons and perform single-photon spectroscopy of a single ion. To go beyond experiments with cohe rent fields we study temporal correlations between the absorption of photons from the spontaneous parametric down conversion source by a single ion and the detection of the corresponding partner photon. For the applied scheme we observe promising indications that the quantum correlations of photons produced in spontaneous parametric down conversion are preserved in the resonant interaction with a single atom. The implementation of more efficient atom-light coupling and entanglement transfer schemes with our apparatus is outlined.
Trapped ions are a promising platform for local quantum information processing. In order to distribute this quantum information over long distances, we can take advantage of optical cavities, which ofier a coherent interface between matter and light, enabling the transfer of quantum information from stationary qubits such as ions onto photons. We demonstrate such an interface by coupling trapped ions to a cavity and have recently shown that a quantum state can be faithfully transferred from a single ion onto a single photon. In particular, this transfer can be improved by taking advantage of a collective effect between multiple ions, namely, superradiant emission into the cavity. In this proof-of-principle experiment, we tune the phase of a two-ion entangled state between sub- and superradiance. The superradiant coupling is then used to enhance the transfer of quantum information onto a photon from a logical qubit encoded in the two ions. Finally, prospects for linking together distant ions in cavities via a quantum network are discussed. Toward this goal, we outline a fiber-based ion-cavity experiment which allows access to the single-ion strong-coupling regime.
Trapped atomic ions are ideal single photon emitters with long-lived internal states which can be entangled with emitted photons. Coupling the ion to an optical cavity enables the efficient emission of single photons into a single spatial mode and grants control over their temporal shape. These features are key for quantum information processing and quantum communication. However, the photons emitted by these systems are unsuitable for long-distance transmission due to their wavelengths. Here we report the transmission of single photons from a single ^{40}Ca^{+} ion coupled to an optical cavity over a 10 km optical fiber via frequency conversion from 866 nm to the telecom C band at 1530 nm. We observe nonclassical photon statistics of the direct cavity emission, the converted photons, and the 10 km transmitted photons, as well as the preservation of the photons' temporal shape throughout. This telecommunication-ready system can be a key component for long-distance quantum communication as well as future cloud quantum computation.
The controlled emission and absorption of single photons is an important enabling technology in the fields of quantum communication, cryptography and computing. We have realised a novel single photon source, based on a miniature ‘endcap’ ion trap with integrated optical fibres. To minimise distortion of the trapping field the fibres are tightly integrated and recessed within the two hollow cylindrical rf electrodes of the trap. This allows us to bring the fibres to within approximately 300 µm of the trapped ion. With the fibres in place we are able to collect the ion’s fluorescence using no further optics. In this thesis the ion trap is fully characterised, and the quantum nature of the light demonstrated in the results of a variant on the Hanbury Brown-Twiss photon-correlation experiment. The scheme will ultimately be extended to implement a coherent ion-photon interface through strong coupling cavity-QED. Towards this end, an ultra-high-finesse cavity has been designed and fabricated by laser-machining and coating surfaces with a range of radii of curvature on the end facets of the fibres. To improve the stability and precision manipulation of the cavity in-vacuum, an entirely new trap has been designed and built. Finally, the current status of the fibre cavity and the outlook for the experiment are presented.
The research undertaken unites two distinct areas of quantum information processing: single ions stored in radio-frequency traps and single photons in optical fibres. Strings of ions are presently the most successful implementation of quantum computing, with elementary quantum algorithm and quantum simulations realised. The principal challenge in the field is to enhance the quantum processing power by scaling up current devices to larger systems. We pursue one of the most promising strategies: distributed quantum computation in which multiple small-scale ion processors are interlinked by exchanging photonic quantum bits via optical fibres. This requires a coherent quantum interface between ions and photons, mapping ionic to photonic quantum states and vice versa. To maximise fidelity and the success rate of the scheme, the interaction of ions and photons must take place in a microscopic optical cavity with high finesse. To this end, single 40Ca+ were trapped in a radio-frequency ion trap whose trapping electrodes are hollow cylinders. Optical fibres with mirrors machined on the facets are inserted into the electrodes to form a Fabry-Pérot cavity. Because the fibres are shielded by the electrodes the detrimental distortion of the trapping field due to their presence is suppressed and ions can be trapped for several hours. 40Ca+ has a -type energy level scheme wherein the ion is cooled on the 42P1/2 ? 42S1/2 transition and the cavity is tuned to the 42P1/2 ? 32D3/2 transition. This thesis reports the successful coupling of single ions to a high finesse optical fibre based cavity, with coupling strength g = 2p · 4:6 MHz. The cavity has length 367 µm, finesse of 40,000 and linewidth 2k = 2p · 9:4 MHz. In this coupling regime, the enhancement of the ion's emission rate through the Purcell effect was observed. Further, anti-correlation was observed in the emission rates between the P1/2 ? D3/2 and P1/2 ? S1/2 transitions with an effective emission rate suppression of up to 60% in the latter transition. The built system offers greater promises. Once the position in the cavity mode has been optimised we expect to reach the long-sought after strong coupling regime with (g, k, y) = 2p · (12:2; 4:7; 11:2) MHz.
Entanglement is an established resource in quantum information processing, and there is a clear imperative to study many-body systems both in quantum technology applications and for probing fundamental physical laws. Ion trap cavity quantum electrodynamics is a highly promising platform for research. Prerequisites are the controlled coupling of many ions to the cavity field along with the ability to initialize the quantum states and drive coherent transitions between them. A coaxial ion trap and high finesse cavity system has been shown to couple strings of up to five ions to the cavity mode with nearly optimal coupling strength thanks to precise control over their positions in the standing wave and their mutual Coulomb interaction. The predictive power of the theoretical model demonstrates that the scheme can be extended to more ions or to higher coupling regimes. In a separate experiment it has been demonstrated that a quantum state can be initialized, before coherently transferring the population to a qubit state through the cavity interaction. The emission of polarized photons in the cavity mode has been measured, taking the system closer to the generation of cluster states for quantum information research and fundamental studies in many-body entanglement. Building on the aforementioned work, an infrastructure has been put in place for the direct observation of vacuum Rabi oscillations between a single ion and the cavity. In this scheme, the contribution to the dynamics from the dominant incoherent channel is minimized through post-selection of the data. As a quantum system coupled to a reservoir with memory, it will provide experimental constraints on theoretical work in the field of non-Markovian dynamics.