Quantum mechanics allows for the processing of information in entirely new ways, surpassing the computational limits set by classical physics. Termed `quantum information processing', scaling this scheme relies on simultaneously increasing the number of qubits -- the fundamental unit of quantum computation -- whilst reducing their error rates. With this comes a variety of challenges, including the ability to readout the quantum state of large numbers of qubits, as well as to control their evolution in order to mitigate errors. This thesis aims to address these challenges by developing techniques for the readout and control of quantum systems. The first series of experiments focuses on the readout of GaAs/AlGaAs semiconductor quantum systems, primarily relating to the technique of dispersive gate sensing (DGS). DGS is used to probe electron transmission in an open system, a quantum point contact, demonstrating an ability to resolve characteristic features of a one-dimensional ballistic channel in the limit where transport is not possible. DGS is also used to observe anomalous signals in the potential landscape of quantum-dot defining gate electrodes. A technique for time domain multiplexing is also presented, which allows for readout resources, in the form of microwave components, to be shared between multiple qubits, increasing the capacity of a single readout line. The second series of experiments validates control techniques using trapped 171Yb+ ions. Classical error models are engineered using high-bandwidth IQ modulation of the microwave source used to drive qubit rotations. Reductions in the coherent lifetime of the quantum system are shown to match well with quantitative models. This segues in to developing techniques to understand and suppress noise in the system. This is achieved using the filter-transfer function approach, which casts arbitrary quantum control operations on qubits as noise spectral filters.
Quantum mechanics allows for the processing of information in entirely new ways, surpassing the computational limits set by classical physics. Termed `quantum information processing', scaling this scheme relies on simultaneously increasing the number of qubits -- the fundamental unit of quantum computation -- whilst reducing their error rates. With this comes a variety of challenges, including the ability to readout the quantum state of large numbers of qubits, as well as to control their evolution in order to mitigate errors. This thesis aims to address these challenges by developing techniques for the readout and control of quantum systems. The first series of experiments focuses on the readout of GaAs/AlGaAs semiconductor quantum systems, primarily relating to the technique of dispersive gate sensing (DGS). DGS is used to probe electron transmission in an open system, a quantum point contact, demonstrating an ability to resolve characteristic features of a one-dimensional ballistic channel in the limit where transport is not possible. DGS is also used to observe anomalous signals in the potential landscape of quantum-dot defining gate electrodes. A technique for time domain multiplexing is also presented, which allows for readout resources, in the form of microwave components, to be shared between multiple qubits, increasing the capacity of a single readout line. The second series of experiments validates control techniques using trapped 171Yb+ ions. Classical error models are engineered using high-bandwidth IQ modulation of the microwave source used to drive qubit rotations. Reductions in the coherent lifetime of the quantum system are shown to match well with quantitative models. This segues in to developing techniques to understand and suppress noise in the system. This is achieved using the filter-transfer function approach, which casts arbitrary quantum control operations on qubits as noise spectral filters.
There is currently a worldwide effort towards the realisation of large-scale quantum computers that exploit quantum phenomena for information processing. While these computing systems could potentially redefine the technological landscape, harnessing quantum effects is challenging due to their inherently fragile nature and the experimentally demanding environments in which they arise. In order for quantum computation to be viable it is first necessary to demonstrate the operation of two-level quantum systems (qubits) which have long coherence times, can be quickly read out, and can be controlled with high fidelity. Focusing on these key requirements, this thesis presents four experiments towards scalable solid state quantum computing using gate-defined quantum dot devices based on gallium arsenide (GaAs) heterostructures. The first experiment investigates a phonon emission process that limits the charge coherence in GaAs and potentially complicates the microwave control of multi-qubit devices. We show that this microwave analogy to Raman spectroscopy can provide a means of detecting the unique phonon spectral density created by a nanoscale device. Experimental results are compared to a theoretical model based on a non-Markovian master equation and approaches to suppressing electron-phonon coupling are discussed. The second experiment demonstrates a technique involving in-situ gate electrodes coupled to lumped-element resonators to provide high-bandwidth dispersive read-out of the state of a double quantum dot. We characterise the charge sensitivity of this method in the few-electron regime and benchmark its performance against quantum point contact charge sensors. The third experiment implements a low-loss, chip-level frequency multiplexing scheme for the readout of scaled-up spin qubit arrays. Dispersive gate-sensing is realised in combination with charge detection based on two radio frequency quantum point contacts to perform multiplexed readout of a double quantum dot in the few-electron regime. Demonstration of a 10-channel multiplexing device is achieved and limitations in scaling spin qubit readout to large numbers using multiplexed channels discussed. The final experiment ties previously presented results together by realising a micro-architecture for controlling and reading out qubits during the execution of a quantum algorithm. The basic principles of this architecture are demonstrated via the manipulation of a semiconductor qubit using control pulses that are cryogenically routed using a high-electron mobility transistor switching matrix controlled by a field programmable gate array. Finally, several technical results are also presented including the development of printed circuit board solutions to allow the high-frequency measurement of nanoscale devices at cryogenic temperatures and the design of on-chip interconnects used to suppress electromagnetic crosstalk in high-density spin qubit device architectures.
Quantum computing promises to deliver uniquely powerful information processing machines by exploiting the quantum phenomena of superposition and entanglement. In solid-state systems, there has been significant progress in the isolation and control of the fundamental units needed to build such machines, known as qubits. However, scaling-up the number of qubits to the point where sophisticated algorithms can be performed presents considerable experimental challenges. In particular, it is becoming increasingly apparent that a new class of tools will be required to interface between fragile quantum systems, and the classical readout and control hardware of the outside world. This thesis presents experimental investigations towards the development of a scalable readout architecture for semiconductor qubit platforms. Fast readout of a GaAs-AlGaAs double quantum dot in the few-electron regime is first demonstrated via an embedded dispersive gate sensor (DGS), alleviating the burden of requiring separate charge sensors for every qubit. The sensitivity and bandwidth of this technique are extracted and benchmarked against well-established readout methods. Dispersive gate sensing of quantum point contacts (QPCs) is then presented, probing charge rearrangement within the local electrostatic environment of quasi one-dimensional channels. A low-loss, lumped-element, LC resonant circuit is also implemented for frequency multiplexed readout. The second set of experiments concern the design and characterisation of miniaturised, on-chip circulators based on the quantum Hall effect, and the quantum anomalous Hall effect. Microwaves are first capacitively coupled into edge magnetoplasmon modes in a mesoscopic GaAs-AlGaAs droplet. Non-reciprocal forward transmission comparable to off-the-shelf components is observed, which is accounted for within an interferometric picture. This circulator design is then extended to thin films of the three-dimensional topological insulator, Cr-doped (Bi,Sb)2Te3, wherein similar non-reciprocity is demonstrated in the absence of an external magnetic field.
Quantum entanglement and superposition, in addition to revealing interesting physics in their own right, can be harnessed as computational resources in a machine, enabling a range of algorithms for classically intractable problems. In recent years, experiments with small numbers of qubits have been demonstrated in a range of solid-state systems, but this is far from the numbers required to realise a useful quantum computer. In addition to the qubits themselves, quantum operation requires a host of classical electronics for control and readout, and current techniques used in few-qubit systems are not scalable. This thesis presents a series of techniques for control and readout of solid-state qubits, working towards scalability by integrating classical control with the quantum technology. Two techniques for reducing the footprint associated with readout of gallium arsenide spin qubits are demonstrated. Gate electrodes, used to define the quantum dot, are also shown to be sensitive state detectors. These gate-sensors, and the more conventional Quantum Point Contacts, are then multiplexed in the frequency domain, where three-channel qubit readout and ten-channel QPC readout are demonstrated. Two types of superconducting devices are also explored. The loss in superconducting coplanar waveguide resonators is measured, and a suppression of coupling to the parasitic electromagnetic environment is demonstrated. The thesis also details software for the simulation of Josephson-junction based circuits including features beyond what is available in commercial products. Finally, an architecture for managing control of a scalable machine is proposed where classical components are distributed throughout a cryostat and cryogenic switches route control pulses to the appropriate qubits. A simple implementation of the architecture is demonstrated that incorporates a double quantum dot, a gallium arsenide switch matrix, frequency multiplexed readout, and cryogenic classical computation.
For several decades it has been appreciated that quantum computers hold incredible promise to perform calculations intractable to classical computation. However, this promise has be slow to realize. Dozens of quantum systems are currently being investigated for use in quantum information processing - none of which have yet demonstrated algorithms involving more than a handful of qubits and it remains unclear which, if any, of these systems will ultimately compose a scalable, robust quantum information processing architecture. In this thesis we employ analytical, optimal and algebraic control techniques to evaluate various quantum systems for their potential use in quantum information processing. In doing so, we have additionally identified several novel characterization procedures capable of probing both the coherent and incoherent dynamics of quantum systems. The first part of this thesis discusses work motivated by attempts to utilize donor qubits in silicon as quantum bits. We first propose a measurement of the state of a single donor electron spin using two-dimensional electron gas of a field-effect transistor and electrically detected magnetic resonance. We analyze the potential sensitivity of this measurement and show that it is a quantum nondemolition measurement of an electron-encoded state. We then present the first of two novel qubit characterization procedures. We consider the problem of rapidly characterizing a large number of similarly prepared qubits using techniques from optimal experiment design. All qubits are assumed to evolve according to the same physical processes, though the Hamiltonian parameters may vary from device to device - an inevitability in solid state qubits. We use the Cram\\'er-Rao bound on the variance of a point estimator to construct the optimal series of experiments to estimate these free parameters, and present a complete analysis of the optimal experimental configuration. Though applied to dipole- and exchange-coupled qubits, this technique is widely applicable to other systems. The second part of the thesis discusses the role that control can play in measuring and mitigating noise in qubit systems. Our first result describes a method for quickly simulating the effects of arbitrary markovian noise on qubit systems through the use of a numerically optimized, multi-state Markovian fluctuator. This ability to rapidly simulate the noisy qubit evolution allows us to compute control sequences capable of maximally decoupling the qubit from the noise source. We then introduce the second characterization procedure of the these, showing that a single measurable and controllable qubit may act as a spectrometer of dephasing noise. We show that the formalism of dynamical decoupling can be used to estimate the short-time correlation function of the noise source, while long time correlations may be estimated by a very simple series of free evolution experiments. This technique is applicable to the wide range of physical implementations which suffer from dephasing noise.The final part of this thesis demonstrates that trapped neutral atoms may be utilized for the robust simulation of complex systems exhibiting a topological phase. We present a method to simulate the toric code Hamiltonian stroboscopically, and demonstrate that our technique preserves the ground state degeneracy . Furthermore, we introduce a dissipative mechanism allowing for thermalization of the system to a finite temperature or direct cooling to the ground state manifold.
In the last decade, quantum information processing has transformed from a field of mostly academic research to an applied engineering subfield with many commercial companies announcing strategies to achieve quantum advantage and construct a useful universal quantum computer. Continuing efforts to improve qubit lifetime, control techniques, materials and fabrication methods together with exploring ways to scale up the architecture have culminated in the recent achievement of quantum supremacy using a programmable superconducting processor -- a major milestone in quantum computing en route to useful devices. Marking the point when for the first time a quantum processor can outperform the best classical supercomputer, it heralds a new era in computer science, technology and information processing.One of the key developments enabling this transition to happen is the ability to exert more precise control over quantum bits and the ability to detect and mitigate control errors and imperfections. In this thesis, ways to efficiently control superconducting qubits are explored from the experimental viewpoint.We introduce a state-of-the-art experimental machinery enabling one to perform one- and two-qubit gates focusing on the technical aspect and outlining some guidelines for its efficient operation. We describe the software stack from the time alignment of control pulses and triggers to the data processing organisation. We then bring in the standard qubit manipulation and readout methods and proceed to describe some of the more advanced optimal control and calibration techniques.The described toolbox together with some newly developed advances such as multi-level single-shot readout are applied to a practical problem of generating high-quality random numbers. Following the recent advances in the field, we certify our generator based on the Kochen-Specker theorem utilizing contextuality of quantum mechanics as an underlying resource of randomness. Our implementation based on the solid-state circuit quantum electrodynamics (QED) platform and the new certification scheme allows us to greatly enhance the bit rate of certified quantum random number generators (QRNGs) and approach the requirements for real-world applications.Addressing some of the control and state preparation errors, we develop a set of techniques to use a qubit as an in situ probe of distortions of its control lines and its effective temperature. Considering a qubit simultaneously driven by a longitudinal and a transverse MW-drives under certain resonant conditions, we show that in the rotating dressed-state picture (second rotating frame) one can get information about both the amplitude and the phase of the drive signals. This allows us to employ a qubit as an on-chip vector network analyzer and precisely measure the transfer functions of its control lines. As no other method with comparable frequency domain coverage exists, we verify our technique by cancelling out the distortions and increasing the fidelity of entangling two-qubit CPHASE gate.Finally, we show that the decay of the correlations between two sequential measurements of a quantum bit is a manifestation of its nonzero effective temperature. We use it to develop a precise method of evaluating the qubits population allowing for virtually unlimited suppression of absolute errors. We realize the method and demonstrate its applicability to the calibration of a quantum processor and evaluation of active reset techniques. As the actual mechanism of the increased excited-state population is currently unknown, we use our method's precision to show the qubit’s coupling to two separate independent thermal baths. We also introduce the ‘temperature spectroscopy’ as a tool to acquire more information about the qubits spurious excitation sources.
The discovery of quantum mechanics in the 20th century forms the basis of many of the technologies that define our lives today. The ability to engineer and manipulate individual quantum systems -- even create artificial atoms -- promises a similar revolutionary leap in technology. A quantum technology of particular interest is quantum computing, which has the potential to solve problems that are intractable for classical computers, opening up new domains of computation. Meanwhile, an attractive approach to creating engineered quantum systems is circuit quantum electrodynamics (cQED). Where research initially focused on understanding the physics of cQED devices, focus has shifted to building systems capable of performing useful computations. However, this remains extremely challenging, in part due to the inherently fragile nature of the individual quantum bits, but also due to difficulties in controlling and scaling up these systems. This thesis focuses on the control aspects of building an extensible full-stack quantum computer based on superconducting transmon qubits. We define the demonstration of quantum fault-tolerance as our target application to give focus to our efforts. The QuSurf architecture for a full-stack quantum computer presented in this thesis is designed with this application in mind. We provide a detailed study of the error sources present in this system and give an overview of the relevant characterization techniques. In the second part of this thesis, we address several key challenges in the control of a quantum computer. To realize high-fidelity coherence limited gates, we present a novel tuneup protocol that achieves a tenfold speedup over the state-of-the-art. This is realized by eliminating the need for qubit initialization. We demonstrate this protocol by calibrating single-qubit gates to a coherence limited Clifford fidelity of 99.9% in one minute. Performing repeated parity checks, as is required for quantum error correction, requires reusing qubits quickly after they have been measured. By introducing a numerically optimized depletion pulse we are able to speeds up the depletion of measurement photons in a readout resonator without having to rely on specific symmetry conditions. Using this technique speed up photon depletion by more than six inverse resonator linewidths, reducing the error rate in an emulated ancilla parity check by a factor 75. Flux-pulsing based two-qubit gates are the fastest two-qubit gates. However, they are also very technically demanding. The key challenge in performing these gates is addressing the distortions that control signals experience as they traverse various electrical components. We have developed Cryoscope (short for cryogenic oscilloscope) to characterize and correct these distortions. Cryoscope is an in-situ technique that uses the qubit to sample control pulses of arbitrary shape. Even when correcting distortions to within sim0.1 two-qubit gates are history-dependent due to the long timescale upon which some of these distortions act. We have invented Net-Zero, a new type of flux-pulsing based two-qubit gate, to address this problem. It makes use of a symmetry condition of the transmon to have net-zero integral, making the gate resilient to long-timescale distortions. The gate suppresses leakage out of the computational subspace to 0.1% by making use of leakage interference and has a built-in echo effect that enhances the coherence of the gate, achieving a two-qubit gate fidelity of 99.1%. Custom software is required to perform the physics experiments needed to build and operate a quantum computer. PycQED is an open-source software framework we have developed for this purpose. We discuss the design choices and concepts of PycQED before turning our focus to characterization and calibration. Here we introduced dependency graphs as a useful abstraction and system emulation as an essential development tool for automating the characterization and calibration process. We conclude the thesis by reflecting on the limitations of our architecture and providing an outlook on the grand challenges of building a useful kilo-qubit sized quantum computer. We define these challenges as The Application Problem, The Fabrication Problem, and The Calibration Problem.