There is currently a worldwide effort towards the realisation of large-scale quantum computers that exploit quantum phenomena for information processing. While these computing systems could potentially redefine the technological landscape, harnessing quantum effects is challenging due to their inherently fragile nature and the experimentally demanding environments in which they arise. In order for quantum computation to be viable it is first necessary to demonstrate the operation of two-level quantum systems (qubits) which have long coherence times, can be quickly read out, and can be controlled with high fidelity. Focusing on these key requirements, this thesis presents four experiments towards scalable solid state quantum computing using gate-defined quantum dot devices based on gallium arsenide (GaAs) heterostructures. The first experiment investigates a phonon emission process that limits the charge coherence in GaAs and potentially complicates the microwave control of multi-qubit devices. We show that this microwave analogy to Raman spectroscopy can provide a means of detecting the unique phonon spectral density created by a nanoscale device. Experimental results are compared to a theoretical model based on a non-Markovian master equation and approaches to suppressing electron-phonon coupling are discussed. The second experiment demonstrates a technique involving in-situ gate electrodes coupled to lumped-element resonators to provide high-bandwidth dispersive read-out of the state of a double quantum dot. We characterise the charge sensitivity of this method in the few-electron regime and benchmark its performance against quantum point contact charge sensors. The third experiment implements a low-loss, chip-level frequency multiplexing scheme for the readout of scaled-up spin qubit arrays. Dispersive gate-sensing is realised in combination with charge detection based on two radio frequency quantum point contacts to perform multiplexed readout of a double quantum dot in the few-electron regime. Demonstration of a 10-channel multiplexing device is achieved and limitations in scaling spin qubit readout to large numbers using multiplexed channels discussed. The final experiment ties previously presented results together by realising a micro-architecture for controlling and reading out qubits during the execution of a quantum algorithm. The basic principles of this architecture are demonstrated via the manipulation of a semiconductor qubit using control pulses that are cryogenically routed using a high-electron mobility transistor switching matrix controlled by a field programmable gate array. Finally, several technical results are also presented including the development of printed circuit board solutions to allow the high-frequency measurement of nanoscale devices at cryogenic temperatures and the design of on-chip interconnects used to suppress electromagnetic crosstalk in high-density spin qubit device architectures.
There is currently a worldwide effort towards the realisation of large-scale quantum computers that exploit quantum phenomena for information processing. While these computing systems could potentially redefine the technological landscape, harnessing quantum effects is challenging due to their inherently fragile nature and the experimentally demanding environments in which they arise. In order for quantum computation to be viable it is first necessary to demonstrate the operation of two-level quantum systems (qubits) which have long coherence times, can be quickly read out, and can be controlled with high fidelity. Focusing on these key requirements, this thesis presents four experiments towards scalable solid state quantum computing using gate-defined quantum dot devices based on gallium arsenide (GaAs) heterostructures. The first experiment investigates a phonon emission process that limits the charge coherence in GaAs and potentially complicates the microwave control of multi-qubit devices. We show that this microwave analogy to Raman spectroscopy can provide a means of detecting the unique phonon spectral density created by a nanoscale device. Experimental results are compared to a theoretical model based on a non-Markovian master equation and approaches to suppressing electron-phonon coupling are discussed. The second experiment demonstrates a technique involving in-situ gate electrodes coupled to lumped-element resonators to provide high-bandwidth dispersive read-out of the state of a double quantum dot. We characterise the charge sensitivity of this method in the few-electron regime and benchmark its performance against quantum point contact charge sensors. The third experiment implements a low-loss, chip-level frequency multiplexing scheme for the readout of scaled-up spin qubit arrays. Dispersive gate-sensing is realised in combination with charge detection based on two radio frequency quantum point contacts to perform multiplexed readout of a double quantum dot in the few-electron regime. Demonstration of a 10-channel multiplexing device is achieved and limitations in scaling spin qubit readout to large numbers using multiplexed channels discussed. The final experiment ties previously presented results together by realising a micro-architecture for controlling and reading out qubits during the execution of a quantum algorithm. The basic principles of this architecture are demonstrated via the manipulation of a semiconductor qubit using control pulses that are cryogenically routed using a high-electron mobility transistor switching matrix controlled by a field programmable gate array. Finally, several technical results are also presented including the development of printed circuit board solutions to allow the high-frequency measurement of nanoscale devices at cryogenic temperatures and the design of on-chip interconnects used to suppress electromagnetic crosstalk in high-density spin qubit device architectures.
Quantum entanglement and superposition, in addition to revealing interesting physics in their own right, can be harnessed as computational resources in a machine, enabling a range of algorithms for classically intractable problems. In recent years, experiments with small numbers of qubits have been demonstrated in a range of solid-state systems, but this is far from the numbers required to realise a useful quantum computer. In addition to the qubits themselves, quantum operation requires a host of classical electronics for control and readout, and current techniques used in few-qubit systems are not scalable. This thesis presents a series of techniques for control and readout of solid-state qubits, working towards scalability by integrating classical control with the quantum technology. Two techniques for reducing the footprint associated with readout of gallium arsenide spin qubits are demonstrated. Gate electrodes, used to define the quantum dot, are also shown to be sensitive state detectors. These gate-sensors, and the more conventional Quantum Point Contacts, are then multiplexed in the frequency domain, where three-channel qubit readout and ten-channel QPC readout are demonstrated. Two types of superconducting devices are also explored. The loss in superconducting coplanar waveguide resonators is measured, and a suppression of coupling to the parasitic electromagnetic environment is demonstrated. The thesis also details software for the simulation of Josephson-junction based circuits including features beyond what is available in commercial products. Finally, an architecture for managing control of a scalable machine is proposed where classical components are distributed throughout a cryostat and cryogenic switches route control pulses to the appropriate qubits. A simple implementation of the architecture is demonstrated that incorporates a double quantum dot, a gallium arsenide switch matrix, frequency multiplexed readout, and cryogenic classical computation.
Quantum computing promises to deliver uniquely powerful information processing machines by exploiting the quantum phenomena of superposition and entanglement. In solid-state systems, there has been significant progress in the isolation and control of the fundamental units needed to build such machines, known as qubits. However, scaling-up the number of qubits to the point where sophisticated algorithms can be performed presents considerable experimental challenges. In particular, it is becoming increasingly apparent that a new class of tools will be required to interface between fragile quantum systems, and the classical readout and control hardware of the outside world. This thesis presents experimental investigations towards the development of a scalable readout architecture for semiconductor qubit platforms. Fast readout of a GaAs-AlGaAs double quantum dot in the few-electron regime is first demonstrated via an embedded dispersive gate sensor (DGS), alleviating the burden of requiring separate charge sensors for every qubit. The sensitivity and bandwidth of this technique are extracted and benchmarked against well-established readout methods. Dispersive gate sensing of quantum point contacts (QPCs) is then presented, probing charge rearrangement within the local electrostatic environment of quasi one-dimensional channels. A low-loss, lumped-element, LC resonant circuit is also implemented for frequency multiplexed readout. The second set of experiments concern the design and characterisation of miniaturised, on-chip circulators based on the quantum Hall effect, and the quantum anomalous Hall effect. Microwaves are first capacitively coupled into edge magnetoplasmon modes in a mesoscopic GaAs-AlGaAs droplet. Non-reciprocal forward transmission comparable to off-the-shelf components is observed, which is accounted for within an interferometric picture. This circulator design is then extended to thin films of the three-dimensional topological insulator, Cr-doped (Bi,Sb)2Te3, wherein similar non-reciprocity is demonstrated in the absence of an external magnetic field.
Quantum mechanics allows for the processing of information in entirely new ways, surpassing the computational limits set by classical physics. Termed `quantum information processing', scaling this scheme relies on simultaneously increasing the number of qubits -- the fundamental unit of quantum computation -- whilst reducing their error rates. With this comes a variety of challenges, including the ability to readout the quantum state of large numbers of qubits, as well as to control their evolution in order to mitigate errors. This thesis aims to address these challenges by developing techniques for the readout and control of quantum systems. The first series of experiments focuses on the readout of GaAs/AlGaAs semiconductor quantum systems, primarily relating to the technique of dispersive gate sensing (DGS). DGS is used to probe electron transmission in an open system, a quantum point contact, demonstrating an ability to resolve characteristic features of a one-dimensional ballistic channel in the limit where transport is not possible. DGS is also used to observe anomalous signals in the potential landscape of quantum-dot defining gate electrodes. A technique for time domain multiplexing is also presented, which allows for readout resources, in the form of microwave components, to be shared between multiple qubits, increasing the capacity of a single readout line. The second series of experiments validates control techniques using trapped 171Yb+ ions. Classical error models are engineered using high-bandwidth IQ modulation of the microwave source used to drive qubit rotations. Reductions in the coherent lifetime of the quantum system are shown to match well with quantitative models. This segues in to developing techniques to understand and suppress noise in the system. This is achieved using the filter-transfer function approach, which casts arbitrary quantum control operations on qubits as noise spectral filters.
Quantum computing is predicted to provide unprecedented enhancements in computational power. A quantum computer requires implementation of a well-defined and controlled quantum system of many interconnected qubits, each defined using fragile quantum states. The interest in a spin-based quantum computer in silicon stems from demonstrations of very long spin-coherence times, high-fidelity single spin control and compatibility with industrial mass-fabrication. Industrial scale fabrication of the silicon platform offers a clear route towards a large-scale quantum computer, however, some of the processes and techniques employed in qubit demonstrators are incompatible with a dense and foundry-fabricated architecture. In particular, spin-readout utilises external sensors that require nearly the same footprint as qubit devices. In this thesis, improved readout techniques for silicon quantum devices are presented and routes towards implementation of a scalable and high-sensitivity readout architecture are investigated. Firstly, readout sensitivity of compact gate-based sensors is improved using a high-quality factor resonator and Josephson parametric amplifier that are fabricated separately from quantum dots. Secondly, an integrated transistor-based control circuit is presented using which sequential readout of two quantum dot devices using the same gate-based sensor is achieved. Finally, a large-scale readout architecture based on random-access and frequency multiplexing is introduced. The impact of readout circuit footprint on readout sensitivity is determined, showing routes towards integration of conventional circuits with quantum devices in a dense architecture, and a fault-tolerant architecture based on mediated exchange is introduced, capable of relaxing the limitations on available control circuit footprint per qubit. Demonstrations are based on foundry-fabricated transistors and few-electron quantum dots, showing that industry fabrication is a viable route towards quantum computation at a scale large enough to begin addressing the most challenging computational problems.
Spin qubits in semiconductor quantum circuits have been identified as a compelling platform for large scale quantum computing. Today an ongoing effort of the community is aiming at the scaling of such systems by filling larger and larger arrays. In this context the development of tuning and readout protocols allowing to reduce the inherent complexity of such systems seems to be a necessity.In the first part of my thesis, I demonstrate array partitioning of a linear triple quantum dot defined in a AlGaAs/GaAs heterostructure via a highly tunable interdot tunnel coupling. This allows us to operate independently smaller sections of the array which reduces the number of available charge states for the system and therefore reduces its complexity during the tuning.The second part of my thesis is focused on reducing the hardware overhead necessary to extract information during the readout of the spin qubits. In semiconductor spin qubits, high fidelity read-out is obtained through Pauli spin blockade in a double quantum dot with two electrons probed by a local electrometer. One electron is the qubit, the second is the ancilla and only one bit of information is extracted. To obtain the full two-bit information of the two-electron spin states, more quantum hardware is necessary (either dots, electrometers, or reservoirs).Based on an original protocol, I develop in this thesis a complete single-shot read-out procedure for two-electron spin states in a double quantum dot discriminating between S, T0, T+ and T-. It uses successively three distinct spin-to-charge conversion protocols interleaved with charge configuration measurements. The strategy is based on four novel experimental achievements:First, the control from the GHz to sub-Hz regime of the interdot tunnel coupling at the nanosecond timescale.Second, the separation of the spin-to-charge conversion and the charge read-out in the voltage gate space.Third, the suppression of spin relaxation process during the read-out procedure.Finally, the repetition of three distinct spin-to-charge conversion protocols.The read-out procedure is tested on various initialized populations and implemented in more complex spin manipulation sequences to assess its validity.
Quantum computation has been a major focus of research in the past two decades, with recent experiments demonstrating basic algorithms on small numbers of qubits. A large-scale universal quantum computer would have a profound impact on science and technology, providing a solution to several problems intractable for classical computers. To realise such a machine, today's small experiments must be scaled up, and a system must be built which provides control and measurement of many hundreds of qubits. A device of this scale is challenging: qubits are highly sensitive to their environment, and sophisticated isolation techniques are required to preserve the qubits' fragile states. Solid-state qubits require deep-cryogenic cooling to suppress thermal excitations. Yet current state-of-the-art experiments use room-temperature electronics which are electrically connected to the qubits. This thesis investigates various scalable technologies and techniques which can be used to control quantum systems. With the requirements for semiconductor spin-qubits in mind, several custom electronic systems, to provide quantum control from deep cryogenic temperatures, are designed and measured. A system architecture is proposed for quantum control, providing a scalable approach to executing quantum algorithms on a large number of qubits. Control of a gallium arsenide qubit is demonstrated using a cryogenically operated FPGA driving custom gallium arsenide switches. The cryogenic performance of a commercial FPGA is measured, as the main logic processor in a cryogenic quantum control system, and digital-to-analog converters are analysed during cryogenic operation. Recent work towards a 100-qubit cryogenic control system is shown, including the design of interconnect solutions and multiplexing circuitry. With qubit fidelity over the fault-tolerant threshold for certain error correcting codes, accompanying control platforms will play a key role in the development of a scalable quantum machine.