Nonlinear superconducting circuits are a leading candidate to implement quantum information tasks beyond the reach of classical processors. One such task, quantum simulation, involves using a controllable quantum system to study the dynamics of another. In this thesis, we present a series of experiments using small systems of superconducting circuits to perform various quantum tasks relevant to quantum simulation.In the first experiment, we design and build a circuit comprising three transmon qubits whose dynamics mirror those of interacting bosonic particles on a lattice, described by the Bose-Hubbard Hamiltonian. We verify the predictions of the Bose-Hubbard model for this system spectroscopically and then use time-domain measurements to study the decoherence processes affecting the qubits. Using a Raman process, we engineer artificial decay dynamics in the system which allow us to prepare and stabilize otherwise inaccessible states of the transmon array.The second experimental demonstration concerns topological quantum matter. Certain quantum systems are characterized by quantities known as topological invariants, which are robust to local perturbations. These topological invariants are challenging to measure in naturally-occurring systems. We engineer an artificial system, comprising a transmon qubit coupled to a high-Q cavity, capable of undergoing a protocol known as the quantum walk, which also exhibits topological invariants. By using particular non-classical state of the cavity, we modify the quantum walk protocol to make the topological invariant directly accessible.Finally, we implement a hybrid quantum-classical algorithm—known as the variational quantum eigensolver—in a two-transmon quantum processor. As a proof of principle demonstration, we compute the ground-state and low-lying excited state energies of the hydrogen molecule as a function of nuclear separation. We show that an extension of the basic algorithm, known as the quantum subspace expansion, allows for the mitigation of errors caused by decoherence processes affecting the quantum processor.
Nonlinear superconducting circuits are a leading candidate to implement quantum information tasks beyond the reach of classical processors. One such task, quantum simulation, involves using a controllable quantum system to study the dynamics of another. In this thesis, we present a series of experiments using small systems of superconducting circuits to perform various quantum tasks relevant to quantum simulation.In the first experiment, we design and build a circuit comprising three transmon qubits whose dynamics mirror those of interacting bosonic particles on a lattice, described by the Bose-Hubbard Hamiltonian. We verify the predictions of the Bose-Hubbard model for this system spectroscopically and then use time-domain measurements to study the decoherence processes affecting the qubits. Using a Raman process, we engineer artificial decay dynamics in the system which allow us to prepare and stabilize otherwise inaccessible states of the transmon array.The second experimental demonstration concerns topological quantum matter. Certain quantum systems are characterized by quantities known as topological invariants, which are robust to local perturbations. These topological invariants are challenging to measure in naturally-occurring systems. We engineer an artificial system, comprising a transmon qubit coupled to a high-Q cavity, capable of undergoing a protocol known as the quantum walk, which also exhibits topological invariants. By using particular non-classical state of the cavity, we modify the quantum walk protocol to make the topological invariant directly accessible.Finally, we implement a hybrid quantum-classical algorithm—known as the variational quantum eigensolver—in a two-transmon quantum processor. As a proof of principle demonstration, we compute the ground-state and low-lying excited state energies of the hydrogen molecule as a function of nuclear separation. We show that an extension of the basic algorithm, known as the quantum subspace expansion, allows for the mitigation of errors caused by decoherence processes affecting the quantum processor.
This thesis explores nonlinear couplings in superconducting circuits with the purpose of achieving quantum control over the elementary excitations of light and motion. It consists mainly of three research themes. The first theme concerns the experimental realisation of a tuneable coupling scheme, giving rise to different interactions with adjustable ratios, between two transmon qubits. The tuneable capabilities of the device together with its versatile geometry and high coherence make it an interesting building block for analog quantum simulators of certain classes of complex problems. The second theme concerns two theoretical proposals for controlling mechanical resonators using transmon qubits. In the first part we analyse an electromechanical circuit architecture giving rise to tuneable three-body interactions between two qubits and a mechanical beam. Several protocols are performed numerically demonstrating ground-state cooling and the creation of mechanical quantum states, such as single-phonon and multi-phonon superposition states as well as qubit-phonon entanglement. Additionally, schemes for generating arbitrary quantum states are explored. The second part relies on the same concept for coupling a mechanical resonator to a transmon qubit and explores the qubit-resonator system in the ultrastrong coupling regime, where the optomechanical coupling approaches or even exceeds the mechanical frequency. We find that for certain coupling strengths ground-state cooling is possible and devise a protocol for generating macroscopic quantum superposition states, known as “Shrödinger cats”, on the mechanical resonator. Finally, the third research theme presented in the thesis concerns an experiment where a cold superconducting qubit is employed to readout and control a thermally populated radio-frequency resonator coupled via a strong dispersive coupling. By means of reservoir engineering, ground-state cooling as well as stabilisation of Fock states in the resonator are demonstrated reaching a new operating regime for circuit quantum electrodynamics.
Superconducting qubits are a promising technology for building a scalable quantum computer. An important architecture employed in the field is called Circuit Quantum Electrodynamics (circuit QED), where such qubits are combined with high quality microwave cavities to study the interaction between artificial atoms and single microwave photons. The ultra-strong coupling achieved in these systems allows for control and readout of the quantum state of qubits to perform quantum information processing. The work on circuit QED performed in this thesis consisted of realizing an experimental setup for qubit experiments in a new laboratory, investigating the coherence and decay of higher energy levels of superconducting transmon qubits and finally demonstrating a novel coaxial form of circuit QED. Designing and building a 3D circuit QED setup involved the following main accomplishments: producing high quality 3D cavities; designing and installing the cryogenic microwave setup as well as the room temperature amplification and data acquisition circuitry; successfully developing a recipe for the fabrication of Josephson junctions; controlling and measuring superconducting 3D transmon qubits at 10mK. Several qubits were fully characterised and have shown coherence times of several microseconds and relaxation times up to 25μs. Superconducting qubits in fact possess higher energy levels that can provide significant computational advantages in quantum information applications. In experiments performed at MIT, preparation and control of the five lowest states of a transmon qubit was demonstrated, followed by an investigation of the phase coherence and decay dynamics of these higher energy levels. The decay was found to proceed mainly sequentially with relaxation times in excess of 20μs for all transitions. A direct measurement of the charge dispersion of these levels was performed to explore their characteristics of dephasing. This experiment was also reproduced on a 3D transmon fabricated and measured in Oxford, where due to a higher effective qubit temperature a multi-level decay model including thermal excitations was developed to explain the observed relaxation dynamics. Finally, a coaxial transmon, which we name the coaxmon, is presented and measured with a coaxial LC readout resonator and input/output coupling ports placed inline along the third dimension. This novel coaxial circuit QED architecture holds great promise for developing a scalable planar grid of qubits to build a quantum computer.
Quantum information processing holds the promise of a paradigm shift in computational power for specific problem classes. While contemporary quantum processors operate in the Noisy Intermediate-Scale Quantum (NISQ) regime and remain highly susceptible to errors, ongoing experimental efforts on these near-term devices are crucial for advancing the underlying technology. Among the various hardware implementations, superconducting quantum circuits stand out as one of the most robust architectures for scalable quantum technologies. Nevertheless, the primary bottleneck in these systems is the fragility of quantum information: interactions with the environment inevitably perturb the quantum states, a phenomenon known as decoherence. This rapid loss of stored information imposes a fundamental limit on the time available to reliably execute computations on these devices. Within this context, this thesis focuses on the comprehensive experimental characterization of a planar chip featuring isolated, fixed-frequency superconducting transmon qubits. The measurements were conducted in a cryogenic environment, relying on a dilution refrigerator to maintain the device at millikelvin temperatures. To probe the quantum system under these conditions, custom measurement scripts were developed to operate state-of-the-art microwave control electronics (Keysight Quantum Control System), establishing full control over pulse generation, signal acquisition, and digital demodulation. The experimental workflow systematically mapped the physical properties of the device through a progressive series of characterization steps. Initial spectroscopic techniques probed the coupled resonator-qubit system, identifying its fundamental transition frequencies and relevant energy scales. Building upon these frequency-domain measurements, coherent control was achieved by calibrating resonant microwave pulses to drive single-qubit rotations, enabling the reliable preparation of the qubit in excited or coherent superposition states. Finally, specific time-domain protocols were implemented to evaluate the operational limits of the device. By executing standard pulse sequences, the characteristic decoherence metrics of the system, namely the longitudinal energy relaxation time (T1) and the inhomogeneous dephasing time (T2*), were successfully extracted, providing a quantitative assessment of the qubit's overall performance and establishing a baseline for future implementations of more advanced quantum control protocols.
Superconducting qubits are artificial atoms whose spectra and interactions can be engineered through appropriate circuit design, a versatility that can be exploited for quantum simulation. We theoretically investigate a linear array of capacitively coupled transmons, effectively described by a Bose-Hubbard Hamiltonian with attractive interaction. We revisit the discrete-soliton nature of the lowest-energy band of the spectrum, and identify spatially localized quantum solitons. The solitonic character of these states is revealed through their time evolution, which displays a quantum interference pattern, or quantum walk, highlighting their composite nature. We discuss protocols for preparing spatially localized quantum solitons that are compatible with current state-of-the-art tunable-transmon circuits. Our results demonstrate that superconducting circuits provide a promising and experimentally accessible platform for the investigation of quantum soliton physics.
Quantum computing holds the promise of solving problems that are intractable for classical computers, with applications ranging from optimization and materials simulation to cryptography. It achieves this by leveraging the exponentially scaling dimensionality of the space encoding quantum information and by executing algorithms on quantum registers in superposition states – a feature often referred to as quantum parallelism. However, while encoding information in computational units capable of exploring a continuous set of quantum states enables exponential scaling of computational power with system size, quantum systems are also more susceptible to errors than their classical counterparts. These errors take the form of both control errors, where miscalibration of the control pulses causes coherent errors on the qubit states, as well as incoherent errors due to energy relaxation and dephasing. Scaling quantum systems to run useful algorithms involving hundreds or thousands of logical qubits will require quantum error correction. In this approach, quantum information is redundantly encoded across an entangled state of many physical qubits. This has enabled experimental demonstrations across various platforms – including ion traps, superconducting circuits, and neutral atoms – showing that encoded quantum states can be preserved beyond the coherence times of the constituting physical qubits. However, quantum state preservation is only one component needed for scalable quantum computing. To execute algorithms, it is also necessary to implement quantum gates on and between encoded qubits, in a way that maintains fault tolerance by preserving the ability to correct errors as they occur during the computation. In the first part of this thesis, we demonstrate the implementation of an error-corrected quantum operation that entangles two logical qubits. This is achieved by performing lattice surgery on a distance-three surface code qubit, resulting in a logical Bell state encoded in distance-three repetition codes, which enable the correction of single bit-flip errors. We further introduce techniques to benchmark and characterize the performance of logical operations, including applying the protocol to arbitrary logical input states and performing logical quantum process tomography. Together, these results constitute one of the first realizations of error-corrected lattice surgery in superconducting circuits. While quantum error correction can correct errors provided they occur with sufficiently low frequency, it may fail when many qubits experience errors simultaneously. In the second part of this thesis, we therefore shift focus to a specific error mechanism known to cause correlated errors in superconducting circuits – quasiparticle-induced decoherence. In this case, various forms of energy deposition on the quantum device can break Cooper pairs into quasiparticles, which may subsequently diffuse to the tunnel junction and interact with the qubit state, thereby causing decoherence. In this thesis, we investigate the impact of quasiparticle tunneling on qubit performance, with a focus on infrared-induced quasiparticles. We compare the sensitivity of niobium-based qubits to those made from tantalum – a material that has gained interest in recent years following demonstrations of qubits with improved coherence times based on this material. Using a thermal radiator source, we show that the performance of tantalum qubits may be limited by infrared-induced quasiparticles in typical superconducting circuit experimental setups. By employing both ambient and in-line infrared filters, we investigate the effectiveness of different filtering strategies and develop best practices for engineering cryogenic environments for superconducting quantum processors. The results presented in this thesis contribute to the advancement of quantum computing based on superconducting circuits by implementing and characterizing quantum error-corrected operations, and by investigating quasiparticles as a source of decoherence, along with strategies to improve infrared filtering and signal conditioning in cryogenic environments for future fault-tolerant quantum computing.
Quantum processors based on superconducting circuitry have reached the scale of hundreds of qubits and demonstrated computational capabilities that challenge state-of-the-art classical methods for carefully designed problems. Despite these advances, fundamental questions persist over how to best improve and scale the computational power of this emerging technology. Most transmon-based quantum processors encode information in two-level systems, or qubits, leaving the rich multilevel structure of the transmon largely unexploited. In this thesis, we demonstrate how the capabilities of these devices can be meaningfully extended by harnessing this intrinsic multilevel structure to encode qudits — d-level quantum systems that access a larger and more connected Hilbert space than their qubit counterparts. We begin by demonstrating universal single-qudit operation before turning to microwave-activated entanglement to realize scalable two-qudit gates. We present a high-fidelity, fully entangling two-qutrit CZ gate based on a novel tunable cross-Kerr mechanism. We further explore two-qudit gates that selectively entangle subspaces of the full Hilbert space via two-photon multipartite Raman transitions, employing these operations to generate large entangled states across a transmon array. To address the noisy nature of near-term qudit computation, we introduce and characterize error suppression techniques for qudit circuits, including dynamical decoupling and quantum error mitigation. We then synthesize these directions by exploring simulations of quantum systems that have innate multilevel interactions and are therefore well tailored to qudit operation. First we investigate digital quantum simulations of collective neutrino oscillations and the spin-1 truncated Abelian Higgs model, finding error mitigation methods critical for improving circuit performance. Finally, out of equilibrium --- or Floquet --- spin-1 systems are realized using an array of 15 superconducting qutrits to probe a novel Z3 discrete time crystalline (DTC) phase of matter with intrinsically chiral interactions. This DTC result demonstrates that native qudit hardware provides powerful access to non-equilibrium phases rooted in higher discrete symmetries, opening a route to a broader landscape of dynamical orders beyond the Z2 Ising paradigm.