The focus of this thesis is to investigate and fabricate a platform that can facilitate the enhancement of light-matter interactions. By tightly confining the photons and atoms to the same region of space, the probability of interaction is drastically increased as compared to free space interactions. Specifically, we focus on forming an optical cavity (or resonator) incorporated into a hollow-core photonic crystal fiber (HCPCF) using two distinct types of reflective mirrors along the axis of the fiber while still permitting atoms to be loaded into the region of high field confinement. \n \nOne means of pursuing this goal that we explored was to propose and numerically simulate two methods for implementing Bragg gratings in a HCPCF. These two methods leave the hollow-core unobstructed and are both based on controlled selective injection of photosensitive polymers into the photonic-crystal region of the hollow-core fiber, followed by interference photolithography. We report the results of numerical simulations for the hollow core fiber with Bragg gratings formed by the two methods. We find that a reflectivity of > 99.99% should be achievable from such fiber-integrated mirrors. Such a device could support high cooperativity and strong coupling regimes to be achieved. \n \nWe also demonstrate a fiber-integrated Fabry-Pérot cavity formed by attaching a pair of dielectric metasurfaces to the ends of a hollow-core photonic-crystal fiber segment. The metasurfaces consist of perforated membranes designed as photonic-crystal slabs that act as planar mirrors but can potentially allow injection of gases through their holes into the hollow core of the fiber. We have so far observed cavities with finesse of 11 and Q-factors of ~ 4.5 × 10^5, but much higher values should be achievable with improved fabrication procedures. We expect this device to enable the advancement of new fiber lasers, enhanced gas spectroscopy, and studies of fundamental light-matter interactions and nonlinear optics. These mirrors can be designed to be polarization dichroic — transparent for one polarization and reflective for another. This unique property can be exploited to allow for all signals to be directed along the high optical depth axis of the cavity and may provide a excellent platform for applications such as optical switching. \n \nFinally, we develop a novel protocol for a single photon all-optical transistor and how it may be implemented in the above mentioned fiber cavity systems. This unique scheme utilizes a far off-resonant vacuum cavity mode to stimulate a Raman absorption process of a source photon which may be switched off by the insertion of a single gate photon into the cavity mode. Relatively high switching contrasts and ratios for the source photon transmission can be obtained in our system.
The focus of this thesis is to investigate and fabricate a platform that can facilitate the enhancement of light-matter interactions. By tightly confining the photons and atoms to the same region of space, the probability of interaction is drastically increased as compared to free space interactions. Specifically, we focus on forming an optical cavity (or resonator) incorporated into a hollow-core photonic crystal fiber (HCPCF) using two distinct types of reflective mirrors along the axis of the fiber while still permitting atoms to be loaded into the region of high field confinement. \n \nOne means of pursuing this goal that we explored was to propose and numerically simulate two methods for implementing Bragg gratings in a HCPCF. These two methods leave the hollow-core unobstructed and are both based on controlled selective injection of photosensitive polymers into the photonic-crystal region of the hollow-core fiber, followed by interference photolithography. We report the results of numerical simulations for the hollow core fiber with Bragg gratings formed by the two methods. We find that a reflectivity of > 99.99% should be achievable from such fiber-integrated mirrors. Such a device could support high cooperativity and strong coupling regimes to be achieved. \n \nWe also demonstrate a fiber-integrated Fabry-Pérot cavity formed by attaching a pair of dielectric metasurfaces to the ends of a hollow-core photonic-crystal fiber segment. The metasurfaces consist of perforated membranes designed as photonic-crystal slabs that act as planar mirrors but can potentially allow injection of gases through their holes into the hollow core of the fiber. We have so far observed cavities with finesse of 11 and Q-factors of ~ 4.5 × 10^5, but much higher values should be achievable with improved fabrication procedures. We expect this device to enable the advancement of new fiber lasers, enhanced gas spectroscopy, and studies of fundamental light-matter interactions and nonlinear optics. These mirrors can be designed to be polarization dichroic — transparent for one polarization and reflective for another. This unique property can be exploited to allow for all signals to be directed along the high optical depth axis of the cavity and may provide a excellent platform for applications such as optical switching. \n \nFinally, we develop a novel protocol for a single photon all-optical transistor and how it may be implemented in the above mentioned fiber cavity systems. This unique scheme utilizes a far off-resonant vacuum cavity mode to stimulate a Raman absorption process of a source photon which may be switched off by the insertion of a single gate photon into the cavity mode. Relatively high switching contrasts and ratios for the source photon transmission can be obtained in our system.
Our goal is to study quantum optical phenomena in a strong nonlinear optical system. For this purpose, we create a hollow-core photonic-crystal (HCPC) fiber-based platform that confines photons and atomic ensembles together. This enables strong light-matter interactions which are crucial for implementing optical nonlinearities at single-photon levels [1]. We use an optical dipole trap at cesium's magic wavelength to guide laser cooled cesium atoms into and inside the fiber core. This approach will allow us to perform experiments with the dipole trap continuously on as opposed to the previously reported fiber-loading systems [2,3] in which the dipole trap was rapidly amplitude-modulated to avoid the effect from the spatially dependent AC Stark shift. In this system, we perform experiments on electromagnetically induced transparency (EIT) and demonstrate slow light and all optical switch. We also aim to observe large cross-phase modulation (XPM) using a three-level ladder scheme [4,5]. Lastly, the approaches to integrate a cavity into HCPCFs to increase light-matter interactions, thus the optical nonlinearities, will be described.
Non-classical states of light, such as squeezed states, enable a wide variety of scientific and engineering applications in optical communication, precision measurements and quantum computing. Therefore, engineering non-classical states of light in different systems for different purposes is interesting and appealing. Non-classical states of light, particularly squeezed states, can be generated from light in a coherent state or vacuum state by using certain optical nonlinear interactions. To efficiently introduce such optical nonlinear interactions, a high nonlinear coefficient of the medium and high intensity of light in the medium are the key factors, where the hollow core photonic crystal fibers filled with atomic vapor shows their great benefits. In this thesis, we report on our approach to apply hollow core photonic crystal fibers (HCPCFs) with the goal to generate squeezed states using strong optical nonlinearities of atomic vapor. In a HCPCF, light with high intensity has a well confined mode over long distances along the fiber. To apply the HCPCF in squeezed state generation, we experimentally investigated unexpected noise properties of the HCPCF and determined the parameter range to reduce excess noise from the fiber. Furthermore, we have filled the hollow core of a piece of HCPCF with rubidium vapor, which provides a high nonlinearity when the confined light is on resonance with the rubidium dipole transition. Fundamentally, our planned approach relies on self induced transparency (SIT), which offers high nonlinearity and absorption-free propagation at the same time. We have theoretically investigated SIT solitons in rubidium vapor to analyze the required parameters to achieve SIT solitons in our rubidium filled HCPCF. The experimental and theoretical approach presented in this thesis suggests an efficient method for generating squeezed light.
This thesis explores hollow-core fibres as a platform for quantum optics experiments with laser-cooled atomic ensembles. The non-diffracting, tightly-confined guided modes of these fibers grant us a ~µm-wide one-dimensional space to study atom-light interactions. In order to describe on-going experiments, simulations are carried out to understand atomic motion into the hollow fibers. Following which, a preliminary case study of a quantum optics experiment to convert wavelengths of single photons with Cs atomic ensembles inside the hollow fiber is presented. Lastly, basic optical properties of photonic crystal membranes are briefly explored. These can form novel cavities when appended to hollow fibers.
Fiber optical parametric oscillators are being busily investigated as sources of classical light, but are comparatively neglected as potential quantum light sources. Squeezed light is a crucial resource for emerging quantum technologies for computing, communications, and measurement. The direct generation of squeezed light inside optical fiber is of particular interest due to minimal material loss, desirable mode properties and compatibility with long-distance optical networks. Here, we describe a novel all-fiber continuous-wave optical parametric oscillator developed with the aim of generating squeezed light. Our device is based on a 10 cm Fabry-Perot cavity formed by two high-reflectivity fiber Bragg gratings written directly into a single section of photonic crystal fiber. This enables low-loss optical feedback and strongly resonance-enhanced four-wave mixing, with a cavity finesse of up to 400. We observe resonance-enhanced four-wave mixing in these devices, demonstrating a step towards their application as quantum light sources.
This dissertation explores the integration and interfacing of a variety of photonic devices with optical waveguides, aiming to minimize the optical losses and physical footprint of such systems. The specific investigations include interfacing solid-core and hollow-core optical fibers, development of a monolithic single-photon source based on a quantum dot embedded in a semiconductor nanowire aligned with a single-mode fiber, a proposal for a waveguide-integrated power limiter that can protect detectors in a quantum key distribution (QKD) network, and integrating superconducting-nanowire single photon detectors (SNSPD) with laser-written waveguides. \n \nHollow-core photonic-crystal fibers (HCPCFs), which can allow simultaneous tight confinement of both photons and atoms in their hollow core, offer a platform for enhancing interactions between light and atomic ensembles. However, interfacing HCPCFs with conventional solid core (SC) fibers presents a unique set of challenges including significant losses in the joint region due to partial melting and deformation of the photonic crystal during the conventional arc-fusion splicing process. We address this issue with a lithographically defined, vacuum-compatible on-chip structure acting as a mechanical splicer that allows efficient injection of light from a SC fiber to a HCPCF and vice versa, with maximum observed light injection efficiency from a single-mode SC fiber into a HCPCF of 90%. \n \nSingle photon sources (SPS) are often required in photonic quantum information applications. Among various candidates, quantum dots (QD) embedded in tapered semiconductor nanowires have demonstrated excellent progress so far to realize a SPS. However, the overall collection efficiency of the emitted photon into a single mode fiber remains as one of the major challenges, mainly due to loss in the intermediate optical components. We design a complete scheme for high efficiency light coupling from such quantum dot to a single mode fiber. We optimize the geometry of the tapered nanowire to achieve a low numerical aperture Gaussian output mode profile from the wire tip and use a lithographically defined structure to align the SMF collecting the emitted photons. A graded-index multimode fiber acting as a lens is spliced on the SMF end for high efficiency coupling of light from the nanowire into the fiber. \n \nExtremely sensitive photonic devices are often used in quantum optics applications for detection and manipulation of signals with very low power. To prevent malfunction or even damage to these sensitive devices by excess incident power, we propose an optical power limiter based on a pair of cavities integrated with optical waveguides. Such power limiter can be used to protect sensitive electro-optical devices and prevent certain types of attacks on QKD systems. \n \nLastly, a 2D photonic lattice formed by laser-written waveguides in bulk glass can be used as an analogue quantum simulator. We explore the integration of SNSPDs with laser-written waveguides with the goal of making this platform fully on-chip.
Cold atoms trapped and guided in hollow-core photonic crystal fibers provide a scalable diffraction-free setting for atom–light interactions for quantum technologies. However, due to the mismatch of the depth and spatial extension of the trapping potential from free space to the fiber, the number of cold atoms in the fiber is mainly determined by the loading process from free space to waveguide confinement. Here, we provide a numerical study of the loading dynamics of cold atoms into a hollow-core photonic crystal fiber. We use the Monte Carlo method to simulate the trajectories of an ensemble of cold atoms from free space trapping potential to optical potential inside a hollow-core fiber and calculate the temperature, loading efficiency, and geometry of the ensemble. We also study the noise sources that cause heating and a loss of atoms during the process. Our result could be used to design and optimize the loading process of cold atoms into a hollow-core fiber for cold atom experiments.