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Laser-cooled Atomic Ensembles in Hollow Optical Fibers

Sai Sreesh Venuturumilli

Published May 6, 2021• 0 citations
OpenAlex

Abstract

This thesis explores hollow-core fibres as a platform for quantum optics experiments with laser-cooled atomic ensembles. The non-diffracting, tightly-confined guided modes of these fibers grant us a ~µm-wide one-dimensional space to study atom-light interactions. In order to describe on-going experiments, simulations are carried out to understand atomic motion into the hollow fibers. Following which, a preliminary case study of a quantum optics experiment to convert wavelengths of single photons with Cs atomic ensembles inside the hollow fiber is presented. Lastly, basic optical properties of photonic crystal membranes are briefly explored. These can form novel cavities when appended to hollow fibers.

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•Jan 1, 2020•0 citations
This thesis explores hollow-core fibres as a platform for quantum optics experiments with laser-cooled atomic ensembles. The non-diffracting, tightly-confined guided modes of these fibers grant us a ~µm-wide one-dimensional space to study atom-light interactions. In order to describe on-going experiments, simulations are carried out to understand atomic motion into the hollow fibers. Following which, a preliminary case study of a quantum optics experiment to convert wavelengths of single photons with Cs atomic ensembles inside the hollow fiber is presented. Lastly, basic optical properties of photonic crystal membranes are briefly explored. These can form novel cavities when appended to hollow fibers.
Our goal is to study quantum optical phenomena in a strong nonlinear optical system. For this purpose, we create a hollow-core photonic-crystal (HCPC) fiber-based platform that confines photons and atomic ensembles together. This enables strong light-matter interactions which are crucial for implementing optical nonlinearities at single-photon levels [1]. We use an optical dipole trap at cesium's magic wavelength to guide laser cooled cesium atoms into and inside the fiber core. This approach will allow us to perform experiments with the dipole trap continuously on as opposed to the previously reported fiber-loading systems [2,3] in which the dipole trap was rapidly amplitude-modulated to avoid the effect from the spatially dependent AC Stark shift. In this system, we perform experiments on electromagnetically induced transparency (EIT) and demonstrate slow light and all optical switch. We also aim to observe large cross-phase modulation (XPM) using a three-level ladder scheme [4,5]. Lastly, the approaches to integrate a cavity into HCPCFs to increase light-matter interactions, thus the optical nonlinearities, will be described.
In this thesis, I am intending to understand the cooperative effect of an ensemble of quantum emitters, which constitutes the preliminary elements of our current experimental investigations towards realization of an ultra-narrow linewidth superriant laser. In the first part of the thesis, I investigate the basics of the theory of superradiance (SR), which includes the full derivation of the Hamiltonian and the Lindblad equation for an ensemble of two-level atoms in both free-space and a single-mode waveguide. In addition, I construct the simulations for observing the transition from single-atom uncorrelated spontaneous emission to superradiance in various physical settings, as well as a simulation for the understanding of the cooperative effects of an ensemble of two-level atoms inside an optical cavity. Then, in the second part of the thesis, I introduce the experimental progress we have been making to observe SR with an ensemble of laser-cooled Cs atoms inside a hollow-core photonic crystal fiber (HCPCF). In our experiment, the Cs atoms, initially cooled using a magneto-optical trap (MOT), are guided and confined inside a short piece of HCPCF with a magic-wavelength dipole trap. Currently we have successfully implemented a novel detection methods for studying superradiance.
Cold atoms trapped and guided in hollow-core photonic crystal fibers provide a scalable diffraction-free setting for atom–light interactions for quantum technologies. However, due to the mismatch of the depth and spatial extension of the trapping potential from free space to the fiber, the number of cold atoms in the fiber is mainly determined by the loading process from free space to waveguide confinement. Here, we provide a numerical study of the loading dynamics of cold atoms into a hollow-core photonic crystal fiber. We use the Monte Carlo method to simulate the trajectories of an ensemble of cold atoms from free space trapping potential to optical potential inside a hollow-core fiber and calculate the temperature, loading efficiency, and geometry of the ensemble. We also study the noise sources that cause heating and a loss of atoms during the process. Our result could be used to design and optimize the loading process of cold atoms into a hollow-core fiber for cold atom experiments.
Recent demonstrations of light-matter interactions with atoms and molecules confined to hollow waveguides offer great promise for ultralow-light-level applications. The use of waveguides allows for tight optical confinement over interaction lengths much greater than what could be achieved in bulk geometries. However, the combination of strong atom-photon interactions and nonuniformity of guided light modes gives rise to spectroscopic features that must be understood in order to take full advantage of the properties of such systems. We use light-induced atomic desorption to generate an optically dense Rb vapor at room temperature inside a hollow-core photonic band-gap fiber. Saturable-absorption spectroscopy and passive slow-light experiments reveal large ac Stark shifts, power broadening, and transit-time broadening, that are present in this system even at nanowatt powers.
Coherent manipulation and interaction between atoms and light are the core ingredients in modern quantum science and technology. Various applications such as quantum computation, quantum memories and quantum sensors which are promising in future technologies, are currently under exploration. However, due to the diffraction nature of light, miniaturizing quantum systems involving atom-light interactions has been highly limited. To avoid diffraction, I load cold atoms into a hollow-core fiber (HCF) and demonstrate four major experiments inside the fiber: inertia-sensitive Mach-Zehnder atom interferometer, long-lived quantum spin coherence, light storage and creation of an array of Schr\"odinger cat states. In this thesis, I show the theoretical framework of each experiment and demonstrate experimentally a cold atoms quantum laboratory realized a HCF. Cold 85Rb^{85}\text{Rb}85Rb atoms of temperature ∼\sim∼\SI{6}{\micro\kelvin} are loaded into a Kagome type photonic crystal hollow-core fiber (HCF) through an optical trapping beam coupled into the HCF. I first demonstrate an inertia-sensitive Mach-Zehnder atom interferometer using two counter-propagating Raman beams. However, the short quantum spin coherence time of ∼\sim∼\SI{100}{\micro\second} due to the differential AC stark shift from the trapping beam is a major obstacle to reaching high sensitivity of the optically trapped atom interferometer inside the HCF. By introducing a vector light shift from the dipole trap to cancel the differential scalar light shift, the quantum spin coherence time is increased to hundreds of milliseconds. The long quantum spin coherence time opens up possibilities for various quantum experiments in HCF. Here, I demonstrate light storage using atoms as the storage medium in the HCF. A maximum storage efficiency of \SI{3}{\percent} and storage time of over \SI{20}{\milli\second} is shown in this thesis. With the implementation of dynamical decoupling, the storage time is improved to ∼\sim∼\SI{100}{\milli\second}. Moreover, I create a 1D array of Schr\"odinger cats states in facilitated by an optical lattice in the HCF and study its potential for applications in quantum sensing and quantum simulation in HCF. Both odd and even cat states are validated and their coherence properties are studied. This thesis realized the state-of-the-art quantum experiments that are miniaturized into a HCF. The results signify a promise in future quantum sciences and technologies with compact fiber-based devices.