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Collective and optical phenomena in equilibrium and nonequilibrium interacting quantum systems

Eduardo Carlo Mascarenhas Moraes

Published Nov 13, 2014• 0 citations
OpenAlex

Abstract

In this thesis we study collective, emergent and optical properties of interacting quantum systems both in equilibrium and nonequilibrium situations from a microscopic modelling. This orientation steams from both the fact there is a profound need to design, characterise and set up control strategies for realistic systems in which quantum technologies could be conceived and the interest to grasp and identify fundamental principles for the emergence of macroscopic behaviour. The thesis is divided into three parts: I Optical and Collective Phenomena; II Equilibrium many-body systems and III Nonequilibrium many-body systems. Part I includes four complementary contributions to the optics emerging from the collective behaviour of microscopic quantum systems. In part II (Equilibrium many-body systems) of the thesis I have addressed the physics of quantum phase transitions from the perspective of nonequilibrium thermodynamics. We have shown that such an approach captures the essential features of finite order transitions that have a strong connection to thermodynamical and energetic figures of merit, but does not capture infinite order transitions that are of a much more subtle nature. Motivated by these exotic infinite order transitions we have looked at quantum phases and phase transitions through an informational and operational perspective based on pure state conversions restricted by local operations. In the third and last part (Nonequilibrium many-body systems) of the thesis I have laid out a project on the closed evolution of quantum spin chains focussing on the emergent nonequilibrium laws that depart from equilibrium physics.

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In this thesis we study collective, emergent and optical properties of interacting quantum systems both in equilibrium and nonequilibrium situations from a microscopic modelling. This orientation steams from both the fact there is a profound need to design, characterise and set up control strategies for realistic systems in which quantum technologies could be conceived and the interest to grasp and identify fundamental principles for the emergence of macroscopic behaviour. The thesis is divided into three parts: I Optical and Collective Phenomena; II Equilibrium many-body systems and III Nonequilibrium many-body systems. Part I includes four complementary contributions to the optics emerging from the collective behaviour of microscopic quantum systems. In part II (Equilibrium many-body systems) of the thesis I have addressed the physics of quantum phase transitions from the perspective of nonequilibrium thermodynamics. We have shown that such an approach captures the essential features of finite order transitions that have a strong connection to thermodynamical and energetic figures of merit, but does not capture infinite order transitions that are of a much more subtle nature. Motivated by these exotic infinite order transitions we have looked at quantum phases and phase transitions through an informational and operational perspective based on pure state conversions restricted by local operations. In the third and last part (Nonequilibrium many-body systems) of the thesis I have laid out a project on the closed evolution of quantum spin chains focussing on the emergent nonequilibrium laws that depart from equilibrium physics.
This thesis contributes to the field of nonequilibrium phenomena in many-body quantum systems. The properties of systems driven out of equilibrium are studied from three different perspectives: dynamics, thermodynamics, and dynamical phase transitions. The real-time dynamics of quenched quantum systems is studied on the basis of explicit examples of strongly-correlated many-body systems such as the Kondo model, the Luttinger liquid, and the anisotropic Heisenberg chain. The thermodynamic point of view is addressed in terms of the nonequilibrium work fluctuation theorems. In particular, it is shown that work distribution functions and thus also the Crooks relation can be measured in optical spectra of the x-ray edge type. The central aspect of this thesis is the definition of a dynamical phase transition for closed quantum many-body systems that is then analyzed in detail for the one-dimensional transverse field Ising model. In the end the properties of periodically driven quantum systems is discussed for different models such as the Kondo model, resonant level model, and the Luttinger liquid.
This thesis investigates quantum-many body systems out of equilibrium in a variety of physically relevant and intriguing settings. It provides an overview of the recent developments in this field and based on the author’s recent review illuminates many interesting connections and summarises open questions. In this general framework, the various results of the author are embedded. While they often rely on advanced mathematics, great care is taken to present them in an intuitive way and most technical material is discussed separately in appendices. In the context of equilibration, work created as part of this thesis is able to capture the Gaussification of correlated initial states for a large class of free models. This allows to significantly extend equilibration results of free models, which are of crucial importance, as they provide reasonable relaxation time scales and immediately connect to our physical intuition in terms of ballistic spreading. Building on two surprising connections between static and dynamic features of Hamiltonians, which in general are hard to obtain, the results of this thesis further greatly contribute to the recent debate on the true nature of quantum many- body localisation. For those interacting models, we derive the localised structure of eigenstates from a dynamical suppression of information propagation on the low-energy sector. Further, we show how a non-degenerate spectrum, indicating the presence of interactions, and the existence of an approximately local constant of motion are sufficient to show information propagation, if arbitrary energies are allowed. In the context of quantum phase transitions, we continue such connections between static and dynamic features. We specifically investigate the Mott-superfluid transition of the Bose-Hubbard model and ask to what extent it has a universal dynamical signature. In a joint experimental, numerical and analytical effort, complex behaviour of these dynamics is uncovered, thus challenging the common believe that the Kibble-Zurek mechanism is sufficient to fully capture such transitions. We embed such experimental investigation in the recent debate on quantum simulators, which give the exciting perspective of solving notoriously and even provably hard problems efficiently in the laboratory. For such devices, we argue that the final read-out of the results is an important out- standing problem to be solved. We approach this issue in the case of a continuous quantum field, in which the notion of reconstructing the quantum state is even conceptually unclear. Based on tensor network methods, we demonstrate that in an experiment of ultra-cold atoms in a continuous setup, states can nevertheless efficiently be obtained. Thus, this thesis constitutes not only an important review of the field of quantum many-body systems out of equilibrium, but, using advanced mathematical and numerical tools, has significantly contributed to our understanding of various important out- standing questions in interacting many-body systems.
Technological and scientific advances have given rise to an era in which coherent quantum-mechanical phenomena can be probed and experimentally-realised over unprecedented timescales in condensed matter physics. In turn, scientific interest in non-equilibrium dynamics and irreversibility signatures of thermodynamics has taken place in recent decades, particularly in relation to cold-atom platforms and thermoelectric devices. In this PhD thesis I summarise some of the most important results obtained over the duration of my PhD, on the topic of thermodynamics involving interacting many-body quantum systems. The topics of discussion encompass three main themes: spin/particle transport in non-integrable systems, explorations in eigenstate thermalisation and finite-temperature transport in autonomous thermal machines. By questioning the effect of local integrability-breaking perturbations, I describe the subtle effects that may rise from conservation laws and their connection to linear response transport using microscopic models. Then, I describe thermalisation in the context of the eigenstate thermalisation hypothesis and its consequence to multipartite entanglement and high-order correlation functions. Finally, motivated by the necessity of describing quantum thermal machines in the finite-temperature regime, I introduce a novel tensor-network based method to investigate thermodynamic properties of autonomous machines that employ interacting many-body systems as working media.
Many-body systems constructed of quantum-optical building blocks can now be realized in experimental platforms ranging from exciton-polariton fluids to ultracold Rydberg gases, establishing a fascinating interface between traditional many-body physics and the driven-dissipative, nonequilibrium setting of cavity QED. At this interface, the standard techniques and intuitions of both fields are called into question, obscuring issues as fundamental as the role of fluctuations, dimensionality, and symmetry on the nature of collective behavior and phase transitions. Here, we study the driven-dissipative Bose-Hubbard model, a minimal description of numerous atomic, optical, and solid-state systems in which particle loss is countered by coherent driving. Despite being a lattice version of optical bistability, a foundational and patently nonequilibrium model of cavity QED, the steady state possesses an emergent equilibrium description in terms of a classical Ising model. We establish this picture by making new connections between traditional techniques from many-body physics (functional integrals) and quantum optics (the system-size expansion). To lowest order in a controlled expansion---organized around the experimentally relevant limit of weak interactions---the full quantum dynamics reduces to nonequilibrium Langevin equations, which support a phase transition described by model A of the Hohenberg-Halperin classification. Numerical simulations of the Langevin equations corroborate this picture, revealing that canonical behavior associated with the Ising model manifests readily in simple experimental observables.
One of the distinguishing achievements of physics has been the ability to describe the Universe based upon underlying microscopic principles. When there are many participating objects being governed by these microscopic principles, the resultant behavior often harbors emergent collective phenomena that may not be obviously related to the microscopic description. Phase transitions, quantum or classical, are a canonical example of such many-body phenomena that are understood in equilibrium through a framework of thermodynamic constraints, statistical ensembles, and a growth of system-wide correlations at the transition. However, a new class of quantum phase transitions has recently emerged for non-equilibrium systems with behavior that is not captured by this traditional framework. In the case of isolated quantum systems, these transitions occur among excited eigenstates and requires knowledge of the structure of these individual eigenstates in the quantum system. Understanding what drives such a phase transition requires a deeper microscopic knowledge of the role of correlations at the transition. \nThe use of ultracold atoms in optical lattices has paved the way for faithfully realizing quantum phase transitions. In particular, the advent of the quantum gas microscope realized an experimental platform that is highly controllable and provides microscopic access to the many-bodied wave functions. All experiments presented in this thesis use such a quantum gas microscope architecture where a quantum degenerate gas of Rb is used to probe the behavior of non-equilibrium quantum systems in one spatial dimension.\nThis thesis briefly discusses some studies of entanglement in equilibrium quantum phase transitions near the ground state of the system. In the first experiment, we directly measure the second-order R\\'enyi entanglement entropy that develops as a Bose-Hubbard system transitions from a Mott insulator to a superfluid. This is followed by a study of entanglement growth at the transition in the transverse Ising model. \nThese studies progress to the investigation of two particular non-equilibrium quantum phases and their transition into one another: quantum thermalization and many-body localization. We investigate the development of entanglement entropy that mimics thermodynamic entropy for an isolated quantum system which locally thermalizes under its own unitary dynamics. We then investigate the only known robust exception to this thermalizing behavior by studying the onset of many-body localization due to disorder. We observe the breakdown of thermalization in this phase and the logarithmically slow growth of entanglement throughout the system, which identifies the localized system to be an interacting one. Lastly, we investigate the role of correlations in the critical dynamics that emerge at high-orders where the system transitions from thermalizing behavior to many-body localization.
This thesis addresses different aspects of the dynamics of isolated quantum many-body systems far from equilibrium, ranging from transient phenomena at short times to questions about relaxation and equilibration at late times. The first part deals with nonequilibrium critical phenomena. Dynamical quantum phase transitions are characterized in a two-dimensional spin system by studying the distribution of Fisher zeros in the complex time plane. Moreover, a new topologically driven transition in the nonequilibrium steady state of quenched Chern insulators is investigated, resulting in the identification of universal nonanalytic behavior of the Hall conductance as a function of the quench parameter. The second part of the thesis comprises a study of transient dynamics of the transverse-field Ising model in two and three dimensions based on a perturbative derivation of classical networks to encode the time-evolved wave function; this construction is also applicable to represent the state as an artificial neural network. In the last part of the thesis a possible definition of the irreversibility of quantum many-body dynamics is introduced, which is based on the echo dynamics of observables under imperfect effective time reversal. Echo dynamics is studied in generic and integrable quantum systems as well as in the semiclassical limit. The relation to out-of-time-order correlators is explored, which were recently introduced to probe the quantum butterfly effect.