Chiral materials possess some unusual properties which make them interesting for useful applications in nanophotonics. In this work, we review the basic techniques used to achieve electromagnetically induced chirality in initially isotropic materials and mention some of their novel operations. Next, we investigate the transmission characteristics of two different multi-level atomic models in which chirality is introduced by magnetoelectric cross coupling of external electromagnetic fields with atomic transitions, leading to quantum coherence. The left-(lcp) and right-circularly polarized (rcp) beams, the two eigenmodes of a chiral medium, are shown to transmit in an anti-symmetric manner with respect to the probe field detuning and control field magnitude variations. This selective transmission of a particular mode at specific detunings may find applications in optical isolation and storage. We further demonstrate that the driving control fields and their effective phase can be used as tuning knobs to manipulate the medium's birefringence and the transmission of the eigenmodes.
Chiral materials possess some unusual properties which make them interesting for useful applications in nanophotonics. In this work, we review the basic techniques used to achieve electromagnetically induced chirality in initially isotropic materials and mention some of their novel operations. Next, we investigate the transmission characteristics of two different multi-level atomic models in which chirality is introduced by magnetoelectric cross coupling of external electromagnetic fields with atomic transitions, leading to quantum coherence. The left-(lcp) and right-circularly polarized (rcp) beams, the two eigenmodes of a chiral medium, are shown to transmit in an anti-symmetric manner with respect to the probe field detuning and control field magnitude variations. This selective transmission of a particular mode at specific detunings may find applications in optical isolation and storage. We further demonstrate that the driving control fields and their effective phase can be used as tuning knobs to manipulate the medium's birefringence and the transmission of the eigenmodes.
Chiral materials possess some unusual properties for which they have attracted tremendous interest in recent research. In this paper, we discuss the interaction of electromagnetic fields with an initially isotropic material, making it anisotropic chiral by inducing magnetoelectric cross coupling. We consider a four-level double Λ -type configuration of an atomic ensemble, which is simultaneously sensitive to relative phase of the applied fields due to its closed-loop nature, providing an extra degree of freedom for controlling the birefringent nature of the medium. We show that the material splits a linearly polarized probe field into left- (LCP) and right-circularly polarized (RCP) components, and their angular divergence can be related to the optical activity of the medium. This leads to efficient modulation of the probe field, which may be helpful in accurate position detection of the transmitted beams and images. Next, we demonstrate that such a medium can be used to couple incident light with surface plasmons (SPs) in two ways: (1) as a prism-like coupler, in either Otto- or Kretschmann-type geometry, where excitation of SPs can be achieved beyond a certain incident angle of the interacting pulse in a plasmonic waveguide placed closed to it; and (2) direct excitation of SPs by a LCP or RCP beam from the chiral medium in a particular slit-type plasmonic waveguide. We find that the coupled modes in the latter case are unidirectional and highly tunable. Further, we show that the birefringent nature of the medium as well as the plasmonic field intensities can be efficiently manipulated with a number of controlling parameters. Our results may find applications in image coding, plasmonic sensors, and bio-photonics.
Birefringence and dichroism in atomic systems are active areas of research. Circular dichroism is typically observed in chiral atoms, molecules (such as DNA), and optically asymmetric materials. These phenomena enable polarization-based selectivity and high-precision measurements with applications in optical systems, biomedical diagnostics, and advanced photonics.Meanwhile, negative refractive index materials offer exotic applications in optics and photonics, including super-resolution imaging, invisibility cloaking, and sub-wavelength imaging. Here, we identify a novel route to achieving birefringence and dichroism in a left-handed system for the first time.We investigate the optical activity of an atomic left-handed medium, analyzing the interaction of left- and right-circularly polarized light with different atomic states while incorporating local field corrections. Notably, our results demonstrate simultaneous left-handedness for both polarization states. Furthermore, we find that electric birefringence and dichroism are significantly enhanced with increasing control field strength, while magnetic birefringence and dichroism can be fully controlled via strong laser coupling.These findings have promising implications for spintronics, image transmission in metamaterials, and the development of optical switches and high-speed data transmission devices, opening new avenues in quantum optics and photonics.
Birefringence and dichroism in atomic systems are active areas of research. Circular dichroism is typically observed in chiral atoms, molecules (such as DNA), and optically asymmetric materials. These phenomena enable polarization-based selectivity and high-precision measurements with applications in optical systems, biomedical diagnostics, and advanced photonics. Meanwhile, negative-refractive-index materials offer exotic applications in optics and photonics, including superresolution imaging, invisibility cloaking, and subwavelength imaging. Here we identify a route to achieving birefringence and dichroism in a left-handed system. We investigate the optical activity of an atomic left-handed medium, analyzing the interaction of left- and right-circularly polarized light with different atomic states while incorporating local field corrections. Notably, our results demonstrate simultaneous left-handedness for both polarization states. Furthermore, we find that electric birefringence and dichroism are significantly enhanced with increasing control field strength, while magnetic birefringence and dichroism can be fully controlled via strong laser coupling. These findings have promising implications in fields at the interface of left-handedness and dichroism.
The study investigate control of the optical force and its modification with variation of the driving field’s strength in the system levels of the chiral medium for left and right circular polarized light. In addition to orbital and magnetic and spin quantum numbers of applied fields, significant vector field arrows of optical force in chiral media are examined using spatial coordinates, detuning , Rabi frequency and decay rates. The parameters of the probe and control fields’ detuning along with their decay rates and phases are provided to determine the optical force in chiral medium both for left and right circularly polarized fields. The optical force is a function of orbital, magnetic and spin quantum numbers. Using phase, detuning, and Rabi frequency of the control fields as variables, the minimum value of optical force measure is 0.003pN for probe detuning and spatial coordinate while the maximum value of optical force for normalized detuning and transverse radial coordinate is measured to be 0.2pN. Potential uses of optical force in fundamental optics, molecular physics, optomechanics, material science, nanoscience, quantum physics, radar, waveguide, antennas and optical tweezers technology are demonstrated by the results.
Electromagnetically induced transparency and lasing without inversion are optical manifestations of quantum coherence control. Here we theoretically investigate these effects in a chiral molecule, coherently driven by an optical pump, finding that signal fields can undergo chiroptical absorption quenching or amplification within particular spectral windows at pump intensities as low as ≈ 1kW/cm 2 . Our calculations reveal that molecular chirality has the capacity to dramatically alter quantum coherence phenomena at peculiar wavelength ranges, modulating efficiently circular dichroism depending on the polarisation state of both pump and signal fields and the molecular orientation. We find that, for a given molecular orientation, the dissymmetry factor probed upon right/left-circular polarisation excitation by the signal can get maximised by pump polarisation tuning and the signal direction. By averaging over impinging signal orientations, we find that the orientation-averaged dissymmetry factor can diverge owing to electromagnetically induced transparency producing vanishing averaged absorption cross-sections.
Abstract The absorption coefficients, refractive/group indices, phase shifts and fractional change of birefringence beams through dynamic chiral atomic medium are investigated under the effect of quantum tunnelling. The birefringence of phase indices Δ n = n r ( + ) − n r ( − ) and group indices Δ n g = n g ( + ) − n g ( − ) are controlled and modified through induced dynamic chiral medium by tunnelling effect. The group indices n g ( ± ) = ± 500 and group velocities v g ( ± ) = ± c / 500 are reported with the tunnelling effect. The maximum change in birefringent phase shifts is calculated to 5 microradian with tunnelling frequency at a speed of v = 10 cm/s of the chiral medium in the right circularly polarized (RCP) and left circularly polarized (LCP) beams. A 60% fractional change in the phase shift of RCP and LCP beams are investigated through induced chiral medium when the medium is at rest and when it is moving with the speed of v = 10 cm/s. These results will play an important role in scatterplate phase shifting interferometry.