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Quantum Electronics and Laser Science Conference

Spin dynamics in an antiferromagnetic spin-1 condensate

Adam T. Black, Lincoln D. Turner, E. Gómez, Sebastian Jung, Paul D. Lett

Published May 1, 2007• 0 citations
Publisher

Abstract

We observe coherent spin dynamics and measure ground state populations in an antiferromagnetic spin-1 Bose-Einstein condensate. At a critical value of the quadratic Zeeman shift, the oscillations display a resonance in oscillation period.
DOI
10.1109/qels.2007.4431783

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We study experimentally the equilibrium phase diagram of a spin-1 Bose-Einstein condensate with antiferromagnetic interactions, in a regime where spin and spatial degrees of freedom are decoupled. For a given total magnetization mz{m}_{z}mz​, we observe for low magnetic fields an ``antiferromagnetic'' phase where atoms condense in the $m=\ifmmode\pm\else\textpm\fi{}1$ Zeeman states, and occupation of the m=0m=0m=0 state is suppressed. Conversely, for large enough magnetic fields, a phase transition to a ``broken-axisymmetry'' phase takes place: The m=0m=0m=0 component becomes populated and rises sharply above a critical field Bc(mz){B}_{c}({m}_{z})Bc​(mz​). This behavior results from the competition between antiferromagnetic spin-dependent interactions (dominant at low fields) and the quadratic Zeeman energy (dominant at large fields). We compare the measured Bc{B}_{c}Bc​ as well as the global shape of the phase diagram with mean-field theory, and find good quantitative agreement.
We present measurements and a theoretical model for the interplay of spin-dependent interactions and external magnetic fields in atomic spinor condensates. We highlight general features such as quadratic Zeeman dephasing and its influence on coherent spin mixing processes by focusing on a specific coherent superposition state in a F=1F=1F=1 87Rb^{87}\mathrm{Rb}87Rb Bose-Einstein condensate. In particular, we observe the transition from coherent spinor oscillations to the thermal equilibration.
We observe coherent spin oscillations in an antiferromagnetic spin-1 Bose-Einstein condensate of sodium. The variation of the spin oscillations with magnetic field shows a clear signature of nonlinearity, in agreement with theory, which also predicts anharmonic oscillations near a critical magnetic field. Measurements of the magnetic phase diagram agree with predictions made in the approximation of a single spatial mode. The oscillation period yields the best measurement to date of the sodium spin-dependent interaction coefficient, determining that the difference between the sodium spin-dependent s-wave scattering lengths a(f=2) - a(f=0) is 2.47+/-0.27 Bohr radii.
We have experimentally observed the dynamics of an antiferromagnetic sodium Bose-Einstein condensate quenched through a quantum phase transition. Using an off-resonant microwave field coupling the F = 1 and F = 2 atomic hyperfine levels, we rapidly switched the quadratic energy shift q from positive to negative values. At q = 0, the system undergoes a transition from a polar to antiferromagnetic phase. We measured the dynamical evolution of the population in the F = 1, mF = 0 state in the vicinity of this transition point and observed a mixed state of all 3 hyperfine components for q < 0. We also observed the coarsening dynamics of the instability for q < 0, as it nucleated small domains that grew to the axial size of the cloud.
We have experimentally investigated the quench dynamics of antiferromagnetic spinor Bose-Einstein condensates in the vicinity of a zero temperature quantum phase transition at zero quadratic Zeeman shift qqq. The rate of instability shows good agreement with predictions based upon solutions to the Bogoliubov--de Gennes equations. A key feature of this work was removal of magnetic field inhomogeneities, resulting in a steep change in behavior near the transition point. The quadratic Zeeman shift at the transition point was resolved to 250 mHz uncertainty, equivalent to an energy resolution of ${k}_{B}\phantom{\rule{4pt}{0ex}}\ifmmode\times\else\texttimes\fi{}$ (12 pK). A small (2--3 $\ensuremath{\sigma}$) shift of the transition point was observed, from q=0q=0q=0 to q=+650q=+650q=+650 mHz, whose physical mechanism is currently unknown. In this work, we demonstrate a sub-Hz precision measurement of a phase transition in quantum gases. It paves the way toward observing shifts of the transition point due to finite particle number NNN that scale as 1/N1/N1/N, and also to potential Heisenberg limited spectroscopy with antiferromagnetic spinor gases [L.-N. Wu and L. You, Phys. Rev. A 93, 033608 (2016)].
We numerically simulate the dynamics of a spin-2 Bose–Einstein condensate. We find that the initial phase plays an important role in the spin component oscillations. The spin mixing processes can fully cancel out due to quantum interference when taking some initial special phase. In all the spin mixing processes, the total spin is conversed. When the initial population is mainly occupied by a component with the maximal or minimal magnetic quantum number, the oscillations of spin components cannot happen due to the total spin conversation. The presence of quadratic Zeeman energy terms suppresses some spin mixing processes so that the oscillations of spin components are suppressed in some initial spin configuration. However, the linear Zeeman energy terms have no effects on the spin mixing processes.