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arXiv:1410.1938 · Physical Review A

Precise measurements on a quantum phase transition in antiferromagnetic spinor Bose-Einstein condensates

Anshuman Vinit, Chandra Raman

Published Jan 23, 2017• 23 citations
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Abstract

We have experimentally investigated the quench dynamics of antiferromagnetic spinor Bose-Einstein condensates in the vicinity of a zero temperature quantum phase transition at zero quadratic Zeeman shift $q$. The rate of instability shows good agreement with predictions based upon solutions to the Bogoliubov--de Gennes equations. A key feature of this work was removal of magnetic field inhomogeneities, resulting in a steep change in behavior near the transition point. The quadratic Zeeman shift at the transition point was resolved to 250 mHz uncertainty, equivalent to an energy resolution of ${k}_{B}\phantom{\rule{4pt}{0ex}}\ifmmode\times\else\texttimes\fi{}$ (12 pK). A small (2--3 $\ensuremath{\sigma}$) shift of the transition point was observed, from $q=0$ to $q=+650$ mHz, whose physical mechanism is currently unknown. In this work, we demonstrate a sub-Hz precision measurement of a phase transition in quantum gases. It paves the way toward observing shifts of the transition point due to finite particle number $N$ that scale as $1/N$, and also to potential Heisenberg limited spectroscopy with antiferromagnetic spinor gases [L.-N. Wu and L. You, Phys. Rev. A 93, 033608 (2016)].

DOI
10.1103/physreva.95.011603

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This thesis discusses non-equilibrium phenomena in antiferromagnetic spinor quantum gases. We investigate, both experimentally and theoretically, the quench dynamics of antiferromagnetic spinor Bose-Einstein condensates in the vicinity of a zero temperature quantum phase transition. A microwave dressing field was used as a novel tool to access the polar to antiferrmagnetic quantum phase transition at the quadratic Zeeman shift, q=0. By performing instantaneous quenches across the phase transition,a dynamical instability was induced in the atomic cloud. This lead to pair formation and rapid amplification of spin +/-1 atoms through spin-mixing collisions. The spatial ordering kinetics in the vicinity of the phase transition was quantified by performing the local spin measurement. The coarsening dynamics was observed for the instability for q < 0, as it nucleated small domains that grew to the axial size of the cloud. Rich nonequilibrium behavior was observed in the form of growth and decay of both nematic and magnetic spin waves, following the quench. The spatiotemporal evolution was characterized through two particle correlations between atoms in each pair of spin states, which revealed dramatic differences between the dynamics of the spin correlations and those of the spin populations. \nFinally, we demonstrate the remarkable influence of linear Zeeman term on non-equilibrium dynamics of spinor Bose-Einstein condensates. We show that contrary to prior understanding magnetic field gradient actually suppresses the tendency of spin 0 state to separate into spin +/-1 state. This reconciles the Bogoliubov discrepancies and leads to a dramatic sharpening of the transition point, resulting in a resolution at the 1 Hz level. Our results point to the use of dynamics, rather than equilibrium quantities for high precision measurements of phase transitions in quantum gases.
We have experimentally observed the dynamics of an antiferromagnetic sodium Bose-Einstein condensate quenched through a quantum phase transition. Using an off-resonant microwave field coupling the F = 1 and F = 2 atomic hyperfine levels, we rapidly switched the quadratic energy shift q from positive to negative values. At q = 0, the system undergoes a transition from a polar to antiferromagnetic phase. We measured the dynamical evolution of the population in the F = 1, mF = 0 state in the vicinity of this transition point and observed a mixed state of all 3 hyperfine components for q < 0. We also observed the coarsening dynamics of the instability for q < 0, as it nucleated small domains that grew to the axial size of the cloud.
Spinor Bose-Einstein condensates under external magnetic fields exhibit well-characterized spin domains of its ground state due to spin-dependent interactions. At low temperatures, collision-induced spin-mixing instabilities may promote the condensate to dwell into metastable states occurring near the phase boundaries. In this paper, we study theoretically the metastable spin-phase diagram of a spin-1 antiferromagnetic Bose-Einstein condensate at zero and finite temperatures. The approach makes use of Hartree-Fock theory and exploits the symmetry of the Hamiltonian and of the order parameters yielding a closed system of transcendental equations for the free energy, fully avoiding the use of self-consistency methods. Our results are consistent with recent experiments and allow us to explain qualitatively the different types of observed quench dynamics. In addition, we found that similar phenomena should occur in antiferromagnetic spinor condensates with a sudden change in the temperature. It is shown also that the increase in temperature induces a traceable shift of the ferromagnetic-polar transition boundary, behavior previously not noted by self-consistent mean-field calculations.
We study the equilibrium and dynamical properties of a ferromagnetic spinor atomic Bose-Einstein condensate. In the vicinity of the critical point for a continuous quantum phase transition, universal behaviors are observed both in the equilibrium state and in the dynamics when the quadratic Zeeman shift is swept linearly. Three distinct dynamical regions are identified for different sweeping time scales ($\ensuremath{\tau}$) when compared to the time scale ${\ensuremath{\tau}}_{\mathrm{KZ}}\ensuremath{\sim}{N}^{(1+\ensuremath{\nu}z)/\ensuremath{\nu}d}$ decided by external driving in a system with finite size NNN ($\ensuremath{\nu},z$ are critical exponents and ddd the dimensionality). They are manifested by the excitation probability P\mathcal{P}P and the excess heat density Q\mathcal{Q}Q. The adiabatic region of $\mathcal{P}\ensuremath{\sim}\mathcal{Q}\ensuremath{\sim}{\ensuremath{\tau}}^{\ensuremath{-}2}$ follows from the adiabatic perturbation theory when $\ensuremath{\tau}>{\ensuremath{\tau}}_{\mathrm{KZ}}$, while the nonadiabatic universal region of $\mathcal{P}\ensuremath{\sim}\mathcal{Q}\ensuremath{\sim}{\ensuremath{\tau}}^{\ensuremath{-}1}$ in the thermodynamic limit is described by the Kibble-Zurek mechanism when ${\ensuremath{\tau}}_{\mathrm{KZ}}>\ensuremath{\tau}>$ the time scale given by initial gap. The Kibble-Zurek scaling hypothesis is augmented with finite-size scaling in the latter region and several experimentally falsifiable features for the finite system we consider are predicted. The region of the fastest sweeping is found to be nonuniversal and far from equilibrium, with P\mathcal{P}P and Q\mathcal{Q}Q essentially being constants independent of $\ensuremath{\tau}$.
We observe multistep condensation of sodium atoms with spin F=1, where the different Zeeman components m_{F}=0,±1 condense sequentially as the temperature decreases. The precise sequence changes drastically depending on the magnetization m_{z} and on the quadratic Zeeman energy q (QZE) in an applied magnetic field. For large QZE, the overall structure of the phase diagram is the same as for an ideal spin-1 gas, although the precise locations of the phase boundaries are significantly shifted by interactions. For small QZE, antiferromagnetic interactions qualitatively change the phase diagram with respect to the ideal case, leading, for instance, to condensation in m_{F}=±1, a phenomenon that cannot occur for an ideal gas with q>0.
We study experimentally the equilibrium phase diagram of a spin-1 Bose-Einstein condensate with antiferromagnetic interactions, in a regime where spin and spatial degrees of freedom are decoupled. For a given total magnetization mz{m}_{z}mz​, we observe for low magnetic fields an ``antiferromagnetic'' phase where atoms condense in the $m=\ifmmode\pm\else\textpm\fi{}1$ Zeeman states, and occupation of the m=0m=0m=0 state is suppressed. Conversely, for large enough magnetic fields, a phase transition to a ``broken-axisymmetry'' phase takes place: The m=0m=0m=0 component becomes populated and rises sharply above a critical field Bc(mz){B}_{c}({m}_{z})Bc​(mz​). This behavior results from the competition between antiferromagnetic spin-dependent interactions (dominant at low fields) and the quadratic Zeeman energy (dominant at large fields). We compare the measured Bc{B}_{c}Bc​ as well as the global shape of the phase diagram with mean-field theory, and find good quantitative agreement.