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arXiv:cond-mat/0509083 · Physical Review A

Evolution of a spinor condensate: Coherent dynamics, dephasing, and revivals

Jochen Kronjäger, C. Becker, M. Brinkmann, R. Walser, Patrick Navez, Kai Bongs, K. Sengstock

Published Dec 27, 2005• 93 citations
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Abstract

We present measurements and a theoretical model for the interplay of spin-dependent interactions and external magnetic fields in atomic spinor condensates. We highlight general features such as quadratic Zeeman dephasing and its influence on coherent spin mixing processes by focusing on a specific coherent superposition state in a $F=1$ $^{87}\mathrm{Rb}$ Bose-Einstein condensate. In particular, we observe the transition from coherent spinor oscillations to the thermal equilibration.

DOI
10.1103/physreva.72.063619

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We present measurements and a theoretical model for the interplay of spin-dependent interactions and external magnetic fields in atomic spinor condensates. We highlight general features such as quadratic Zeeman dephasing and its influence on coherent spin mixing processes by focusing on a specific coherent superposition state in a F=1F=1F=1 87Rb^{87}\mathrm{Rb}87Rb Bose-Einstein condensate. In particular, we observe the transition from coherent spinor oscillations to the thermal equilibration.
Bose-Einstein condensation (BEC) is a phenomenon in which identical bosons occupy the same quantum state below a certain critical temperature. A hallmark of BEC is the coherence between particles every particle shares the same quantum wavefunction and phase. This coherence has been demonstrated for the external (motional) degrees of freedom of the atomic condensates by interfering two condensates. In this thesis, the coherence is shown to extend to the internal spin degrees of freedom of a spin-1 Bose gas evidenced by the observed coherent and reversible spin-changing collisions. The observed coherent dynamics are analogous to Josephson oscillations in weakly connected superconductors and represent a type of matter-wave four-wave mixing. Control of the coherent evolution of the system using magnetic fields is also demonstrated. The studies on spinor condensates begin by creating spinor condensates directly using all-optical approaches that were first developed in our laboratory. All-optical formation of Bose-Einstein condensates (BEC) in 1D optical lattice and single focus trap geometries are developed and presented. These techniques offer considerable flexibility and speed compared to magnetic trap approaches, and the trapping potential can be essentially spin-independent and are ideally suited for studying spinor condensates. Using condensates with well-defined initial non-equilibrium spin configuration, spin mixing of F = 1 and F = 2 spinor condensates of rubidium-87 atoms confined in an optical trap is observed. The equilibrium spin configuration in the F = 1 manifold confirms that 87Rb is ferromagnetic. The coherent spinor dynamics are demonstrated by initiating spin mixing deterministically with a non-stationary spin population configuration. Finally, the interplay between the coherent spin mixing and spatial dynamics in spin-1 condensates with ferromagnetic interactions is investigated.
Decoherence and Recurrences in a Large Ferromagnetic F=1F = 1F=1 Spinor Bose-Einstein Condensate
Decoherence with recurrences appear in the dynamics of the one-body density matrix of an F=1F = 1F=1 spinor Bose-Einstein condensate, initially prepared in coherent states, in the presence of an external uniform magnetic field and within the single mode approximation. The phenomenon emerges as a many-body effect of the interplay of the quadratic Zeeman effect, that breaks the rotational symmetry, and the spin-spin interactions. By performing full quantum diagonalizations very accurate time evolution of large condensates are analyzed, leading to heuristic analytic expressions for the time dependence of the density matrix, in the weak and strong interacting regimes. We are able to find accurate analytical expressions for both the decoherence and the recurrence times, in terms of the number of atoms and strength parameters, that show remarkable differences depending on the strength of the spin-spin interactions. We discuss the nature of these limits in the light of the thermodynamic limit.
This thesis discusses non-equilibrium phenomena in antiferromagnetic spinor quantum gases. We investigate, both experimentally and theoretically, the quench dynamics of antiferromagnetic spinor Bose-Einstein condensates in the vicinity of a zero temperature quantum phase transition. A microwave dressing field was used as a novel tool to access the polar to antiferrmagnetic quantum phase transition at the quadratic Zeeman shift, q=0. By performing instantaneous quenches across the phase transition,a dynamical instability was induced in the atomic cloud. This lead to pair formation and rapid amplification of spin +/-1 atoms through spin-mixing collisions. The spatial ordering kinetics in the vicinity of the phase transition was quantified by performing the local spin measurement. The coarsening dynamics was observed for the instability for q < 0, as it nucleated small domains that grew to the axial size of the cloud. Rich nonequilibrium behavior was observed in the form of growth and decay of both nematic and magnetic spin waves, following the quench. The spatiotemporal evolution was characterized through two particle correlations between atoms in each pair of spin states, which revealed dramatic differences between the dynamics of the spin correlations and those of the spin populations. \nFinally, we demonstrate the remarkable influence of linear Zeeman term on non-equilibrium dynamics of spinor Bose-Einstein condensates. We show that contrary to prior understanding magnetic field gradient actually suppresses the tendency of spin 0 state to separate into spin +/-1 state. This reconciles the Bogoliubov discrepancies and leads to a dramatic sharpening of the transition point, resulting in a resolution at the 1 Hz level. Our results point to the use of dynamics, rather than equilibrium quantities for high precision measurements of phase transitions in quantum gases.
We experimentally investigate and analyze the rich dynamics in F=2F=2F=2 spinor Bose-Einstein condensates of 87Rb^{87}\mathrm{R}\mathrm{b}87Rb. An interplay between mean-field driven spin dynamics and hyperfine-changing losses in addition to interactions with the thermal component is observed. In particular, we measure conversion rates in the range of ${10}^{\ensuremath{-}12}\text{ }\text{ }{\mathrm{c}\mathrm{m}}^{3}\text{ }{\mathrm{s}}^{\ensuremath{-}1}$ for spin-changing collisions within the F=2F=2F=2 manifold and spin-dependent loss rates in the range of ${10}^{\ensuremath{-}13}\text{ }\text{ }{\mathrm{c}\mathrm{m}}^{3}\text{ }{\mathrm{s}}^{\ensuremath{-}1}$ for hyperfine-changing collisions. We observe polar behavior in the F=2F=2F=2 ground state of 87Rb^{87}\mathrm{R}\mathrm{b}87Rb, while we find the F=1F=1F=1 ground state to be ferromagnetic. We further see a magnetization for condensates prepared with nonzero total spin.
Decoherence with recurrences appear in the dynamics of the one-body density matrix of an F=1 spinor Bose–Einstein condensate, initially prepared in coherent states, in the presence of an external uniform magnetic field and within the single mode approximation. The phenomenon emerges as a many-body effect of the interplay of the quadratic Zeeman effect, which breaks the rotational symmetry, and the spin-spin interactions. By performing full quantum diagonalizations, a very accurate time evolution of large condensates is analyzed, leading to heuristic analytic expressions for the time dependence of the one-body density matrix, in the weak and strong interacting regimes, for initial coherent states. We are able to find accurate analytical expressions for both the decoherence and the recurrence times, in terms of the number of atoms and strength parameters, which show remarkable differences depending on the strength of the spin-spin interactions. The features of the stationary states in both regimes are also investigated. We discuss the nature of these limits in light of the thermodynamic limit.
We study the nonequilibrium coherent spin-mixing dynamics in ferromagnetic spin-1 and antiferromagnetic spin-2 thermal gases of ultracold 87Rb^{87}\mathrm{Rb}87Rb atoms. Long-lasting spin population oscillations with magnetic-field-dependent resonances are observed in both cases. Our observations are well reproduced by Boltzmann equations of the Wigner distribution function. Compared to the equation of motion of spinor Bose-Einstein condensates, the only difference here is a factor-of-2 increase in the spin-dependent interaction, which is confirmed directly in the spin-2 case by measuring the relation between the oscillation amplitude and the sample's density.