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Quantum Correlations and Temperature Fluctuations in Nanoscale Systems

Fredrik Brange

Published Apr 1, 2019• 0 citations
OpenAlex

Abstract

This thesis addresses two different topics related to the physics of nanoscale systems. The first topic concerns quantum correlations and entanglement between electrons in solid-state systems, with a focus on how to generate electronic orbital entanglement on a sub-decoherence time scale and how to achieve experimentally more feasible entanglement detection schemes. The second topic concerns heat transport and temperature fluctuations in nanoscale systems, with a focus on how to utilize temperature fluctuations for calorimetric detection of single particles. The thesis comprises five papers.In Paper I, we propose a quantum dot system to generate and detect, using cotunneling processes, orbitally entangled pairs of electrons on a sub-decoherence time scale.In Paper II, we investigate, by applying an entanglement witness, the minimal number of zero-frequency current cross-correlation measurements needed to detect bipartite entanglement between two flying qubits.In Paper III, we consider energy and temperature fluctuations, and the influence of charging effects, in a metallic island tunnel coupled to a normal metallic lead, the so-called single electron box.In Paper IV, we investigate nanoscale quantum calorimetry and propose a setup consisting of a metallic island and a superconducting lead to realize a nanoscale calorimeter that may probe the energies of tunneling electrons.In Paper V, we investigate photon transport statistics of a microwave cavity, including the short-time statistics of single photon emissions and the long-time statistics of heat transport through the cavity.

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This thesis addresses two different topics related to the physics of nanoscale systems. The first topic concerns quantum correlations and entanglement between electrons in solid-state systems, with a focus on how to generate electronic orbital entanglement on a sub-decoherence time scale and how to achieve experimentally more feasible entanglement detection schemes. The second topic concerns heat transport and temperature fluctuations in nanoscale systems, with a focus on how to utilize temperature fluctuations for calorimetric detection of single particles. The thesis comprises five papers.In Paper I, we propose a quantum dot system to generate and detect, using cotunneling processes, orbitally entangled pairs of electrons on a sub-decoherence time scale.In Paper II, we investigate, by applying an entanglement witness, the minimal number of zero-frequency current cross-correlation measurements needed to detect bipartite entanglement between two flying qubits.In Paper III, we consider energy and temperature fluctuations, and the influence of charging effects, in a metallic island tunnel coupled to a normal metallic lead, the so-called single electron box.In Paper IV, we investigate nanoscale quantum calorimetry and propose a setup consisting of a metallic island and a superconducting lead to realize a nanoscale calorimeter that may probe the energies of tunneling electrons.In Paper V, we investigate photon transport statistics of a microwave cavity, including the short-time statistics of single photon emissions and the long-time statistics of heat transport through the cavity.
The work contained in this thesis deals with two closely related topics. Papers I-III deal with charge transport statistics in nanoscale devices to investigate the presence of entanglement in the constituent electrons. We identify the contributions of entangled electron pairs to the current cross-correlations as a signature of entanglement. Paper IV treats the electric control of a quantum dot based spin qubit via Electric Dipole Spin Resonance.In Paper I, we present a spin entanglement detection model in a hybrid nanoscale device, with a general entangler connected to a set of quantum dots and anti-collinear ferromagnetic contacts. Our model allows us to study the implications of a non-ideal detector in an entanglement detection scheme.In Paper II, we investigate a scheme for generating and detecting orbitally entangled states in a device consisting of six quantum dots. The underlying process which enables our proposed scheme is sufficiently fast, even for the rapidly decaying quantum coherence of orbital states defined in a solid.In Paper III, we investigate a minimal entanglement detection scheme based on measurements of current cross correlations. We find a significant reduction in the number of measurements required for an entanglement test.In Paper IV, we investigate the optimisation of electrically controlling an electron spin in a gate defined semiconductor quantum dot. Specifically, we study how the shape of the quantum dot together with the direction of an in-plane magnetic field affect the spin relaxation rate and frequency of the induced Rabi oscillations.
In this thesis I find an analytic expression for the conductance of a single electron transistor in the regime when temperature, level spacing, and charging energy of an island are all of the same order. I also study the correction to the spacing between Coulomb blockade peaks due to finite dot-lead tunnel couplings. I find analytic expressions for both correction to the spacing averaged over mesoscopic fluctuations and the rms of the correction fluctuations. In the second part of the thesis I discuss the feasibility of quantum dot based spin- and charge-qubits. Firstly, I study the effect of mesoscopic fluctuations on the magnitude of errors that can occur in exchange operations on quantum dot spin-qubits. Mid-size double quantum dots, with an odd number of electrons in the range of a few tens in each dot, are investigated through the constant interaction model using realistic parameters. It is found that the number of independent parameters per dot that one should tune depends on the configuration and ranges from one to four. Then, I study decoherence of a quantum dot charge qubit due to coupling to piezoelectric acoustic phonons in the Born-Markov approximation. After including appropriate form factors, I find that phonon decoherence rates are one to two orders of magnitude weaker than was previously predicted. My results suggest that mechanisms other than phonon decoherence play a more significant role in current experimental setups.
Mesoscopic physics and nanoelectronics concentrate on systems with dimensions somewhere between atomic and everyday macroscopic scale. Modern technology enables construction of submicron nanostructures where modeling based on classical physics has proven inadequate. It is possible to design electric circuits where dynamics of single electrons and photons are controlled using state-of-the-art experimental methods. For quantitative understanding of these systems it is necessary to resort to a quantum-mechanical description. Quantum phenomena, such as tunneling and a wave-like interference of particles, are essential ingredients of physics in mesoscopic systems. Field of mesoscopic physics contains a rich variety of topics ranging from fundamental condensed matter physics to quantum information processing and possible future technological applications. \n \nThis thesis presents theoretical studies of mesoscopic quantum phenomena in nanostructures and small electronic devices. We have focused on effects of environment fluctuations and investigated connections between fluctuations and transport phenomena. Decoherence in quantum bits (qubits) and quantum state engineering in superconducting circuits are also studied. The theoretical analysis in each case requires an open-system treatment. \n \nEffects of current fluctuations on quantum probe systems have been studied in detail. We have calculated transitions induced by current noise and discussed how these could be used for characterization of fluctuations. We have also shown that electric fluctuations play a key role in radiation and photon heat transport in nanostructures. Motivated by recent advances in mesoscopic electron-photon systems, we have studied a response of a coupled resonator-qubit system, squeezing of quantum fluctuations in small superconducting circuits and investigated decoherence in Josephson flux qubits.
This thesis is concerned with employing the statistics of charge transfer in a conductor as a tool for quantum measurement. The physical systems studied are electronic devices made by nanoscale manufacturing techniques. In this context quantum measurement appears not as a postulate, but as physical process. In this thesis I am considering a quantum system, in particular a qubit or a nanomechanical resonator, interacting with a tunnel junction. The effect of coupling a quantum system to a tunnel junction is twofold: The state of the quantum system will be changed and there will be information about the quantum system in the statistics of charge transfer of the tunnel junction. As the first example a quantum measurement process of a qubit is considered. A common description of the system and charge dynamics is found by introducing a new quantity, the charge specific density matrix. By deriving and solving a Markovian master equation for this quantity the measurement process is analyzed. The measurement is shown to be a dynamical process, where correlations between the initial state of the qubit and the number of charges transferred in the tunnel junction arise on a typical timescale, the measurement time. As another example of a quantum system a nanomechanical oscillator is considered. It is found, that the biased tunnel junction, acting as a non-equilibrium environment to the oscillator, increases the temperature of the oscillator from its thermal equilibrium value. The current in the junction is modulated by the interaction with the oscillator, but the influence vanishes for bias voltages smaller than the oscillator frequency. For an asymmetric junction and non-vanishing oscillator momentum a current is shown to flow through the junction even at zero bias. The current noise spectrum induced by the oscillator in the tunnel junction consists of a noise floor and a peaked structure with peaks at zero frequency, the oscillator frequency and double the oscillator frequency. The peak heights are dependent on the coupling strength between oscillator and junction, the occupation number of the oscillator, the bias voltage and the junction temperature. I show how the peak height can be used as a measure of the oscillator temperature, demonstrating that the noise of a tunnel junction can be used for electronic thermometry of a nanomechanical oscillator.
This thesis is devoted to the study of quantum mechanical effects that arise in systems of reduced dimensionality. Specifically, we investigate coherence and correlation effects in quantum transport models. In the first part, we present a theory of Markovian and non- Markovian current correlations in nanoscopic conductors. The theory is applied to obtain the spectrum of quantum noise and high-order current correlations at finite frequencies in quantum-dot systems. One of the main conclusions is that only the non-Markovian approach contains the physics of vacuum fluctuations. In the second part, we study the coupling of superconducting qubits to optical atomic systems and to cavity resonators. We propose a hybrid quantum system consisting of a flux qubit coupled to NV centers in diamond. We also demonstrate the existence of the so-called Bloch-Siegert shift in the ultra-strong coupling regime between a flux qubit and a LC resonator. Throughout the thesis, we make special emphasis on the study of decoherence effects produced by the distinct dissipative baths to which the various types of qubits presented in this thesis are inevitably coupled.
This thesis is devoted to the study of quantum mechanical effects that arise in systems of reduced dimensionality. Specifically, we investigate coherence and correlation effects in quantum transport models. In the first part, we present a theory of Markovian and non- Markovian current correlations in nanoscopic conductors. The theory is applied to obtain the spectrum of quantum noise and high-order current correlations at finite frequencies in quantum-dot systems. One of the main conclusions is that only the non-Markovian approach contains the physics of vacuum fluctuations. In the second part, we study the coupling of superconducting qubits to optical atomic systems and to cavity resonators. We propose a hybrid quantum system consisting of a flux qubit coupled to NV centers in diamond. We also demonstrate the existence of the so-called Bloch-Siegert shift in the ultra-strong coupling regime between a flux qubit and a LC resonator. Throughout the thesis, we make special emphasis on the study of decoherence effects produced by the distinct dissipative baths to which the various types of qubits presented in this thesis are inevitably coupled.