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arXiv:cond-mat/0604065

Quantum Dots: Coulomb Blockade, Mesoscopic Fluctuations, and Qubit Decoherence

Serguei Vorojtsov

Published Apr 4, 2006• 0 citations
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Abstract

In this thesis I find an analytic expression for the conductance of a single electron transistor in the regime when temperature, level spacing, and charging energy of an island are all of the same order. I also study the correction to the spacing between Coulomb blockade peaks due to finite dot-lead tunnel couplings. I find analytic expressions for both correction to the spacing averaged over mesoscopic fluctuations and the rms of the correction fluctuations. In the second part of the thesis I discuss the feasibility of quantum dot based spin- and charge-qubits. Firstly, I study the effect of mesoscopic fluctuations on the magnitude of errors that can occur in exchange operations on quantum dot spin-qubits. Mid-size double quantum dots, with an odd number of electrons in the range of a few tens in each dot, are investigated through the constant interaction model using realistic parameters. It is found that the number of independent parameters per dot that one should tune depends on the configuration and ranges from one to four. Then, I study decoherence of a quantum dot charge qubit due to coupling to piezoelectric acoustic phonons in the Born-Markov approximation. After including appropriate form factors, I find that phonon decoherence rates are one to two orders of magnitude weaker than was previously predicted. My results suggest that mechanisms other than phonon decoherence play a more significant role in current experimental setups.

DOI
10.48550/arxiv.cond-mat/0604065

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In this thesis I find an analytic expression for the conductance of a single electron transistor in the regime when temperature, level spacing, and charging energy of an island are all of the same order. I also study the correction to the spacing between Coulomb blockade peaks due to finite dot-lead tunnel couplings. I find analytic expressions for both correction to the spacing averaged over mesoscopic fluctuations and the rms of the correction fluctuations. In the second part of the thesis I discuss the feasibility of quantum dot based spin- and charge-qubits. Firstly, I study the effect of mesoscopic fluctuations on the magnitude of errors that can occur in exchange operations on quantum dot spin-qubits. Mid-size double quantum dots, with an odd number of electrons in the range of a few tens in each dot, are investigated through the constant interaction model using realistic parameters. It is found that the number of independent parameters per dot that one should tune depends on the configuration and ranges from one to four. Then, I study decoherence of a quantum dot charge qubit due to coupling to piezoelectric acoustic phonons in the Born-Markov approximation. After including appropriate form factors, I find that phonon decoherence rates are one to two orders of magnitude weaker than was previously predicted. My results suggest that mechanisms other than phonon decoherence play a more significant role in current experimental setups.
In this dissertation we discuss decoherence in charge qubits formed by multiple lateral quantum dots in the framework of the spin-boson model and the Born-Markov approximation. We consider the intrinsic decoherence caused by the coupling to bulk phonon modes and electromagnetic environmental fluctuations. In the case of decoherence caused by phonon coupling, two distinct quantum dot configurations are studied and proposed as setups that mitigate its nocive effects : (i) Three quantum dots in a ring geometry with one excess electron in total and (ii) arrays of quantum dots where the computational basis states form multipole charge configurations. For the three-dot qubit, we demonstrate the possibility of performing one- and two-qubit operations by solely tuning gate voltages. Compared to a previous proposal involving a linear three-dot spin qubit, the three-dot charge qubit allows for less overhead on two-qubit operations. For small interdot tunnel amplitudes, the three-dot qubits have Q factors much higher than those obtained for double-dot systems. The high-multipole dot configurations also show a substantial decrease in decoherence at low operation frequencies when compared to the double-dot qubit. We also discuss decoherence due to electromagnetic fluctuations in charge qubits formed by two lateral quantum dots. We use effective circuit models to evaluate correlations of voltage fluctuations in the qubit setup. These correlations allows us to estimate energy (T1) and phase (T2) relaxation times of the the qubit system. We also discuss the dependence the quality factor Q shows with respect to parameters of the setup, such as temperature and capacitive coupling between the electrodes.
The spin of an electron confined into a lateral semiconductor quantum dot has been proposed as a possible physical realization of a qubit. While the spin has the advantage of large decoherence times, operations with more than one qubit will necessarily involve orbital degrees of freedom, namely, charge, which is much more prone to decoherence. There are also alternative quantum dot qubit proposals that are entirely based on charge. We have used a realistic model to quantify the limitations imposed by acoustic phonons on the operation of quantum dot-based qubits. Our treatment includes essential aspects of the setup geometry, wave function profile and materials characteristics. The time dependence of the qubit density matrix is the presence of a phonon bath solved within the Born-Markov approximation. We find that the inclusion of geometric form factors makes the phonon-induced decoherence rates in double dot charge qubits nearly one order of magnitude lower than estimates previously in the literature. Moreover, our theoretical prediction for the quality factor of coherent charge oscillations based on phonon decoherence are higher than the values recently observed experimentally. This allows us to conclude that phonons are not the primary source of decoherence in double quantum dot qubits.
We describe time-dependent single-electron transport through quantum dots in the Coulomb blockade regime. Coherent dynamics of a single charge qubit in a double quantum dot is discussed with full one-qubit manipulation. Strength of decoherence is controlled with the applied voltage, but uncontrolled decoherence arises from electron–phonon coupling and background fluctuations. Then energy-relaxation dynamics is discussed for orbital and spin degree of freedom in a quantum dot. The electron–phonon interaction and spin–orbit coupling can be investigated as the dissipation problem. Finally, charge detection measurement is presented for statistical analysis of single-electron tunnelling transitions and for a sensitive qubit read-out device.
We study the effect of mesoscopic fluctuations on the magnitude of errors that can occur in exchange operations on quantum dot spin qubits. Midsize double quantum dots, with an odd number of electrons in the range of a few tens in each dot, are investigated through the constant interaction model using realistic parameters. It is found that the constraint of having short pulses and small errors implies keeping accurate control, at the few percent level, of several electrode voltages. In practice, the number of independent parameters per dot that one should tune depends on the configuration and ranges from one to four.
The major contribution to decoherence of a double quantum dot or a Josephson-junction charge qubit comes from the electrostatic coupling to fluctuating background charges hybridized with the conduction electrons in the reservoir. However, estimations according to previously developed theories show that finding a sufficient number of effective fluctuators in a realistic experimental layout is quite improbable. We show that this paradox is resolved by allowing for a short-range Coulomb interaction of the fluctuators with the electrons in the reservoir. This dramatically enhances both the number of effective fluctuators and their contribution to decoherence, resulting in the most dangerous decoherence mechanism for charge qubits.
Electron spins confined in quantum dots (QDs) are among the leading contenders for implementing quantum information processing. In this Thesis we address two of the most significant technological challenges towards developing a scalable quantum information processor based on spins in quantum dots: (i) decoherence of the electronic spin qubit due to the surrounding nuclear spin bath, and (ii) long-range spin-spin coupling between remote qubits. To this end, we develop novel strategies that turn the unavoidable coupling to the solid-state environment (in particular, nuclear spins and phonons) into a valuable asset rather than a liability. In the first part of this Thesis, we investigate electron transport through single and double QDs, with the aim of harnessing the (dissipative) coupling to the electronic degrees of freedom for the creation of coherence in both the transient and steady-state behaviour of the ambient nuclear spins. First, we theoretically show that intriguing features of coherent many-body physics can be observed in electron transport through a single QD. To this end, we first develop a master-equation-based formalism for electron transport in the Coulomb-blockade regime assisted by hyperfine (HF) interaction with the nuclear spin ensemble in the QD. This general tool is then used to study the leakage current through a single QD in a transport setting. When starting from an initially uncorrelated, highly polarized state, the nuclear system experiences a strong correlation buildup, due to the collective nature of the coupling to the central electron spin. We demonstrate that this results in a sudden intensity burst in the electronic tunneling current emitted from the QD system, which exceeds the maximal current of a corresponding classical system by several orders of magnitude. This gives rise to the new paradigm of electronic superradiance. Second, building upon the insight that the nuclear spin dynamics are governed by collective interactions giving rise to coherent effects such as superradiance, we propose a scheme for the deterministic generation of steady-state entanglement between the two nuclear spin ensembles in an electrically defined double quantum dot. Because of quantum interference in the collective coupling to the electronic degrees of freedom, the nuclear system is actively driven into a two-mode squeezedlike target state. The entanglement buildup is accompanied by a self-polarization of the nuclear spins towards large Overhauser field gradients. Moreover, the feedback between the electronic and nuclear dynamics is shown to lead to intriguing effects such as multistability and criticality in the steady-state solutions. In the second part of this Thesis, our focus turns towards the realization of long-range spin-spin coupling between remote qubits. We propose a universal, on-chip quantum transducer based on surface acoustic waves in piezo-active materials. Because of the intrinsic piezoelectric (and/or magnetostrictive) properties of the material, our approach provides a universal platform capable of coherently linking a broad array of qubits, including quantum dots, trapped ions, nitrogen-vacancy centers or superconducting qubits. The quantized modes of surface acoustic waves lie in the gigahertz range, can be strongly confined close to the surface in phononic cavities and guided in acoustic waveguides. We show that this type of surface acoustic excitations can be utilized efficiently as a quantum bus, serving as an on-chip, mechanical cavity-QED equivalent of microwave photons and enabling long-range coupling of a wide range of qubits. In summary, this thesis provides contributions towards developing a scalable quantum information processor based on spins in quantum dots in two different aspects. The first part is dedicated to a deeper understanding of the nuclear spin dynamics in quantum dots. In the second part we put forward a novel sound-based strategy to realize long-range spin-spin coupling between remote qubits. This completes a broad picture of spin-based quantum information processing which integrates different perspectives, ranging from the single-qubit level to a broader quantum network level.