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Stability limitations in optical frequency standards.

Paul Taylor

Published Sep 1, 1999• 0 citations
OpenAlex

Abstract

The limiting effects to the stability of optical frequency standards has been assessed. The stability of such a standard depends critically on the spectral width of the atomic absorber. The limiting stability is explored in the absence decoherence (interrogation time limited) and in the more realistic case where optical decoherence and radiative decay are present. The role of motional decoherence in an ion trap system is also discussed. (author)

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Philosophical Transactions of the Royal Society A Mathematical Physical and Engineering Sciences•Sep 19, 2011•29 citations
The limiting effects to the stability of optical frequency standards has been assessed. The stability of such a standard depends critically on the spectral width of the atomic absorber. The limiting stability is explored in the absence decoherence (interrogation time limited) and in the more realistic case where optical decoherence and radiative decay are present. The role of motional decoherence in an ion trap system is also discussed. (author)
Optical atomic clocks have been rapidly developing in recent decades, resulting in major improvements in both precision and accuracy. As a result, they have become instrumental in multiple areas of applied and fundamental research. Despite all atomic frequency references having more than two energy-levels, the commonly used model for evaluating their ultimate limits assumes a two-level atom. This leads to frequency interrogation protocols and theoretical stability bounds that are suboptimal for a true multi-level atom. The most fundamental stability bound assumes two noise sources - quantum projection noise and spontaneous decay from the excited state. In this work, we analyze a model that includes these noise types and is generalized beyond the two-level assumption, where spontaneous decay can branch to more than a single ground state. This model allows for detection and exclusion of atomic frequency interrogations in which the atom decayed, leading to a frequency stability improvement of up to ≈4.5 dB\approx 4.5 \text{ dB}≈4.5 dB compared with the two-level model. Furthermore, we identify an even greater stability enhancement of ≈5.4 dB\approx 5.4 \text{ dB}≈5.4 dB for frequency comparisons between atoms in an odd parity Bell state. These enhancements are particularly relevant for the numerous trapped-ion optical clock species that operate close to lifetime-limited stability. We calculate new stability limits for those cases and provide a detailed experimental protocol for frequency interrogation with an 27Al+^{27}\text{Al}^{+}27Al+ optical ion clock.
Active optical frequency standards provide interesting alternatives to their passive counterparts. Particularly, such a clock alone continuously generates highly stable narrow-line laser radiation. Thus, a local oscillator is not required to keep the optical phase during a dead time between interrogations as in passive clocks, but only to boost the active clock's low output power to practically usable levels with the current state of technology. Here we investigate the spectral properties and the stability of active clocks, including homogeneous and inhomogeneous broadening effects. We find that for short averaging times the stability is limited by photon shot noise from the limited emitted laser power and at long averaging times by phase diffusion of the laser output. Operational parameters for best long-term stability were identified. Using realistic numbers for an active clock with 87Sr^{87}\mathrm{Sr}87Sr, we find that optimized stability of ${\ensuremath{\sigma}}_{y}(\ensuremath{\tau})\ensuremath{\approx}4\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}18}/\sqrt{\ensuremath{\tau}[\mathrm{s}]}$ is achievable.
We consider various approaches to the creation of a high-stability active optical frequency standard, where the atomic ensemble itself produces a highly stable and accurate frequency signal. The short-time frequency stability of such standards may overcome the stability of lasers stabilized to macroscopic cavities which are used as local oscillators in the modern optical frequency standard systems. The main idea is to create a “superradiant” laser operating deep in the bad cavity regime, where the decay rate of the cavity field significantly exceeds the decoherence rate of the lasing transition. Two main approaches towards the realization of an active optical frequency standard have been proposed already: the optical lattice laser, and the atomic beam laser. We consider these and some alternative approaches, and discuss the parameters for atomic ensembles necessary to attain the metrology relevant level of short-time frequency stability, and various effects and main challenges critical for practical implementations.
An optical clock or frequency standard based on the interrogation of an atomic transition in the optical domain, operates at ~1014Hz is capable of providing orders of magnitude better accuracy than the present primary standard of frequency or time operating in the microwave range. Optical transitions of an ions, confined within a radio frequency ion trap and laser cooled to ~mK temperature, provides better long term stability since they are free from Coulomb and intra-atomic interactions. Optical frequency standards have been realized with several ions, e.g.,199Hg+,171Yb+,115In+,88Sr+,40Ca+,27Al+and among those171Y+has multiple ultra-narrow optical transitions suitable for serving as frequency standards [1-2].
A fundamental limit to the stability of a single-ion optical frequency standard is set by quantum noise in the measurement of the internal state of the ion. We discuss how the interrogation sequence and the processing of the atomic resonance signal can be optimized in order to obtain the highest possible stability under realistic experimental conditions. A servo algorithm is presented that stabilizes a laser frequency to the single-ion signal and that eliminates errors due to laser frequency drift. Numerical simulations of the servo characteristics are compared to experimental data from a frequency comparison of two single-ion standards based on a transition at 688 THz in 171 Yb + . Experimentally, an instability σ y (100 s) = 9 × 10 −16 is obtained in the frequency difference between both standards.
Experimental techniques of laser cooling and trapping, along with other cooling techniques, have produced gaseous samples of atoms so cold that they are, for many practical purposes, in the quantum ground state of their centre-of-mass motion. Such low velocities have virtually eliminated effects such as Doppler shifts, relativistic time dilation and observation-time broadening that previously limited the performance of atomic frequency standards. Today, the best laser-cooled, caesium atomic fountain, microwave frequency standards realize the International System of Units (SI) definition of the second to a relative accuracy of ≈3×10(-16). Optical frequency standards, which do not realize the SI second, have even better performance: cold neutral atoms trapped in optical lattices now yield relative systematic uncertainties of ≈1×10(-16), whereas cold-trapped ions have systematic uncertainties of 9×10(-18). We will discuss the current limitations in the performance of neutral atom atomic frequency standards and prospects for the future.