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Physical Review Applied

Enhancement of the Signal-to-Noise Ratio of an Atomic Magnetometer by 10 dB

Guzhi Bao, Shuhe Wu, Shuqi Liu, Wenfeng Huang, Ziran Li, L. Q. Chen, Chun-Hua Yuan, Weiping Zhang

Published May 28, 2019• 9 citations
Publisher

Abstract

Nonlinear magneto-optical rotation (NMOR) is a sensitive technique for measuring magnetic fields, though the polarization self-rotation (PSR) effect is a fundamental source of excess quantum noise that limits its sensitivity. This study uses a phase shifter to solve the limitation due to the PSR effect. Implementation of the phase shifter improves the signal-to-noise ratio up to 10 dB in the range of Earth's magnetic field. This approach should be useful for high-sensitivity magnetic field measurements in a geomagnetic environment.

DOI
10.1103/physrevapplied.11.054075

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Nonlinear magneto-optical rotation (NMOR) is a sensitive technique for measuring magnetic fields, though the polarization self-rotation (PSR) effect is a fundamental source of excess quantum noise that limits its sensitivity. This study uses a phase shifter to solve the limitation due to the PSR effect. Implementation of the phase shifter improves the signal-to-noise ratio up to 10 dB in the range of Earth's magnetic field. This approach should be useful for high-sensitivity magnetic field measurements in a geomagnetic environment.
The detection of nonlinear magneto-optical rotation (NMOR) of polarized light through alkali atomic vapor is a highly sensitive technique for measuring magnetic fields. We demonstrate that when using frequency modulated light to excite the NMOR resonance, it is possible to cause the system to self-oscillate. The NMOR signal is not a simple replica of the sine wave modulation of the light, but rather contains many higher harmonics of the modulation frequency, and we implement two ways of processing the signal to recover the fundamental modulation frequency in the feedback loop and induce self-oscillation. Self-oscillation simplifies and reduces the power consumption of the electronics required to operate a magnetometer, making the NMOR technique attractive for commercialized magnetic sensors.
We experimentally demonstrate that a squeezed probe optical field can improve the sensitivity of magnetic field measurements based on nonlinear magneto-optical rotation (NMOR) with an amplitude-modulated pump when compared to a coherent probe field under identical conditions. To realize an all-atomic magnetometer prototype, we utilize a nonlinear atomic interaction, known as polarization self-rotation, to produce a squeezed probe field. An independent pump field, amplitude-modulated at the Larmor frequency of the bias magnetic field, allows us to extend the range of most sensitive NMOR measurements to sub-Gauss magnetic fields. While the overall sensitivity of the magnetometer is rather low ( > 250 p T / H z ), we clearly observe a 15 % sensitivity improvement when the squeezed probe is used. Our observations confirm the recently reported quantum enhancement in a modulated atomic magnetometer [ Phys. Rev. Lett. 127 , 193601 ( 2021 ) PRLTAO 0031-9007 10.1103/PhysRevLett.127.193601 ].
A self-oscillating magnetometer based on nonlinear magneto-optical rotation using amplitude-modulated pump light and unmodulated probe light (AM-NMOR) in 87Rb has been constructed and tested towards a goal of airborne detection of magnetic anomalies. In AM-NMOR, stroboscopic optical pumping via amplitude modulation of the pump beam creates alignment of the ground electronic state of the rubidium atoms. The Larmor precession causes an ac rotation of the polarization of a separate probe beam; the polarization rotation frequency provides a measure of the magnetic field. An anti-relaxation coating on the walls of the atomic vapor cell results in a long lifetime of 56 ms for the alignment, which enables precise measurement of the precession frequency. Light is delivered to the magnetometer by polarization-maintaining optical fibers. Tests of the sensitivity include directly measuring the beat frequency between the magnetometer and a commercial instrument and measurements of Earth's field under magnetically quiet conditions, indicating a sensitivity of at least 5 pT/νHz. Rotating the sensor indicates a heading error of less than 1 nT, limited in part by residual magnetism of the sensor.
Optical pumping in an alkali metal vapour produces long-standing coherences of ground state Zeeman sub-levels. These coherences produce large nonlinear magneto-optic rotation (NMOR). Techniques using optical coherences for sensitive magnetometry have been in vogue for a long time. However, the sensitivity achieved has been three orders of magnitude lower than that of a SQUID magnetometer. The NMOR technique has yielded signals having a very narrow width of a few micro-Gauss. In principle, it has been demonstrated that with NMOR magnetometers one can obtain a sensitivity matching, or better than the sensitivity of a Squid magnetometer. There are still many problems to be resolved before these magnetometers can be put to use in geomagnetic and biological applications, where small magnetic fields need to be measured.
Precise magnetometry is vital in numerous scientific and technological applications. At the forefront of sensitivity, optical atomic magnetometry, particularly techniques utilizing nonlinear magneto-optical rotation (NMOR), enables ultraprecise measurements across a broad field range. Despite their potential, these techniques reportedly lose sensitivity in higher magnetic fields, which is attributed to the alignment-to-orientation conversion (AOC) process. In our study, we utilized light with continuously rotating linear polarization to avoid the AOC, which produced robust optical signals and achieving high magnetometric sensitivity over a dynamic range nearly three times greater than Earth's magnetic field. We demonstrated that employing rotating polarization surpasses other NMOR techniques that use modulated light. Our findings also indicate that the previously observed signal deterioration was not due to the AOC, suggesting an alternative cause for this decline.
The nonlinear magneto-optical rotation (NMOR) effect has prolific applications ranging from precision mapping of Earth's magnetic field to biomagnetic sensing. Studies on collisional spin relaxation effects have led to ultrahigh magnetic field sensitivities using a single-beam Λ scheme with state-of-the-art magnetic shielding/compensation techniques. However, the NMOR effect in this widely used single-beam Λ scheme is peculiarly small, requiring complex radio-frequency phase-locking protocols. We show the presence of a previously unknown energy symmetry-based nonlinear propagation blockade and demonstrate an optical inelastic wave-mixing NMOR technique that breaks this NMOR blockade, resulting in an NMOR optical signal-to-noise ratio (SNR) enhancement of more than two orders of magnitude never before seen with the single-beam Λ scheme. The large SNR enhancement was achieved simultaneously with a nearly two orders of magnitude reduction in laser power while preserving the magnetic resonance linewidth. This new method may open a myriad of applications ranging from biomagnetic imaging to precision measurement of the magnetic properties of subatomic particles.