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Science Advances

Symmetry-breaking inelastic wave-mixing atomic magnetometry

Feng Lei Zhou, Chengjie Zhu, E. W. Hagley, L. Deng

Published Dec 1, 2017• 23 citations
Publisher

Abstract

The nonlinear magneto-optical rotation (NMOR) effect has prolific applications ranging from precision mapping of Earth's magnetic field to biomagnetic sensing. Studies on collisional spin relaxation effects have led to ultrahigh magnetic field sensitivities using a single-beam Λ scheme with state-of-the-art magnetic shielding/compensation techniques. However, the NMOR effect in this widely used single-beam Λ scheme is peculiarly small, requiring complex radio-frequency phase-locking protocols. We show the presence of a previously unknown energy symmetry-based nonlinear propagation blockade and demonstrate an optical inelastic wave-mixing NMOR technique that breaks this NMOR blockade, resulting in an NMOR optical signal-to-noise ratio (SNR) enhancement of more than two orders of magnitude never before seen with the single-beam Λ scheme. The large SNR enhancement was achieved simultaneously with a nearly two orders of magnitude reduction in laser power while preserving the magnetic resonance linewidth. This new method may open a myriad of applications ranging from biomagnetic imaging to precision measurement of the magnetic properties of subatomic particles.

DOI
10.1126/sciadv.1700422

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The nonlinear magneto-optical rotation (NMOR) effect has prolific applications ranging from precision mapping of Earth's magnetic field to biomagnetic sensing. Studies on collisional spin relaxation effects have led to ultrahigh magnetic field sensitivities using a single-beam Λ scheme with state-of-the-art magnetic shielding/compensation techniques. However, the NMOR effect in this widely used single-beam Λ scheme is peculiarly small, requiring complex radio-frequency phase-locking protocols. We show the presence of a previously unknown energy symmetry-based nonlinear propagation blockade and demonstrate an optical inelastic wave-mixing NMOR technique that breaks this NMOR blockade, resulting in an NMOR optical signal-to-noise ratio (SNR) enhancement of more than two orders of magnitude never before seen with the single-beam Λ scheme. The large SNR enhancement was achieved simultaneously with a nearly two orders of magnitude reduction in laser power while preserving the magnetic resonance linewidth. This new method may open a myriad of applications ranging from biomagnetic imaging to precision measurement of the magnetic properties of subatomic particles.
The nonlinear magneto-optical effect has significantly impacted modern society with prolific applications ranging from precision mapping of the Earth's magnetic field to bio-magnetic sensing. Pioneering works on collisional spin-exchange effects have led to ultra-high magnetic field detection sensitivities at the level of fT/HzfT/\sqrt{Hz}fT/Hz​ using a single linearly-polarized probe light field. Here we demonstrate a nonlinear Zeeman-coherence parametric wave-mixing optical-atomic magnetometer using room temperature rubidium vapor that results in more than a three-order-of-magnitude optical signal-to-noise ratio (SNR) enhancement for extremely weak magnetic field sensing. This unprecedented enhancement was achieved with nearly a two-order-of-magnitude reduction in laser power while preserving the sensitivity of the widely-used single-probe beam optical-atomic magnetometry method. This new method opens a myriad of applications ranging from bio-magnetic imaging to precision measurement of the magnetic properties of subatomic particles.
We show theoretically the presence of an optical field polarization rotation blocking mechanism in single-probe-based magnetic field sensing schemes, revealing the root cause for extremely small nonlinear magneto-optical rotation (NMOR) signal in single-probe-based atomic magnetometers. We present a colliding-probe atomic magnetometer theory, analytically describing the principle of the first nonlinear-optical atomic magnetometer. This new atomic magnetometry technique breaks the NMOR blockade in single-probe atomic magnetometers, enabling an energy circulation that results in larger than 20-dB enhancement in NMOR signal as well as better than 6-dB improvement of magnetic field detection sensitivity. Remarkably, all experimental observations reported to date can be qualitatively well-explained using this colliding-probe atomic magnetometry theory without numerical computations. This colliding-probe atomic magnetometry technique may have broad applications in scientific and technological fields ranging from micro-Tesla magnetic resonance imaging to cosmic particle detection.
We have developed an inelastic wave scattering based colliding-probe bi-atomic magnetometer theory. We show a propagation growth blockade in single probe based magnetic field sensing schemes, revealing the root cause of strong suppression of nonlinear magneto-optical rotation effect (NMORE) in single probe based atomic magnetometers. We further show, both experimentally and theoretically, a colliding probe bi-atomic magnetometer that lifts this NMORE blockade. The directional energy circulation in this new atomic magnetometry technique results in more than two orders of magnitude increase in NMORE signal as well as greater than 6dB increase of magnetic field detection sensitivity. The new technique may have broad applications in photon gates and switching operations.
We report an optical inelastic-wave-mixing-enhanced atomic magnetometry technique that results in nT-level magnetic field detection at temperatures compatible with the human body without magnetic shielding, zero-field compensation, or high-frequency modulated phase-locking spectroscopy. Using Gaussian magnetic pulses that mimic the transient magnetic field produced by an action potential on a frog's nerve, we demonstrate more than 300,000-fold (550-fold) enhancement of magneto-optical rotation signal power spectral-density (power amplitude) over the conventional single-beam Λ−Λ-Λ−scheme atomic magnetometry method. This new technique may bring possibilities for extremely sensitive magnetic field imaging of biological systems accessible via an optical fiber in clinical environments.
Abstract We demonstrate a dual-beam high-sensitivity room-temperature atomic magnetometer (AM) with a large dynamic range based on a nonlinear magneto-optical rotation (NMOR) enhancing scheme. Using an inelastic wave-mixing laser, we find significant NMOR signal enhancement compared with a single-beam scheme under the same far-detuned operation conditions. This dual-beam scheme is shown to operate well in the regime of lower laser intensity and off-resonance detuning. The best sensitivity achieved is 20 fT/Hz1/2 with a bandwidth of 2 kHz, substantially greater than common spin-exchange relaxation-free AMs. This provides a way to develop low-power, inexpensive miniaturized AMs for wide application.
Nonlinear magneto-optical rotation (NMOR) is a sensitive technique for measuring magnetic fields, though the polarization self-rotation (PSR) effect is a fundamental source of excess quantum noise that limits its sensitivity. This study uses a phase shifter to solve the limitation due to the PSR effect. Implementation of the phase shifter improves the signal-to-noise ratio up to 10 dB in the range of Earth's magnetic field. This approach should be useful for high-sensitivity magnetic field measurements in a geomagnetic environment.