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arXiv:2203.00429

Colliding-probe bi-atomic magnetometers via energy circulation: Breaking symmetry-enforced magneto-optical rotation blockade

Lu Deng

Published Feb 25, 2022• 0 citations
arXivHTMLPDF

Abstract

We have developed an inelastic wave scattering based colliding-probe bi-atomic magnetometer theory. We show a propagation growth blockade in single probe based magnetic field sensing schemes, revealing the root cause of strong suppression of nonlinear magneto-optical rotation effect (NMORE) in single probe based atomic magnetometers. We further show, both experimentally and theoretically, a colliding probe bi-atomic magnetometer that lifts this NMORE blockade. The directional energy circulation in this new atomic magnetometry technique results in more than two orders of magnitude increase in NMORE signal as well as greater than 6dB increase of magnetic field detection sensitivity. The new technique may have broad applications in photon gates and switching operations.

DOI
10.48550/arxiv.2203.00429

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We have developed an inelastic wave scattering based colliding-probe bi-atomic magnetometer theory. We show a propagation growth blockade in single probe based magnetic field sensing schemes, revealing the root cause of strong suppression of nonlinear magneto-optical rotation effect (NMORE) in single probe based atomic magnetometers. We further show, both experimentally and theoretically, a colliding probe bi-atomic magnetometer that lifts this NMORE blockade. The directional energy circulation in this new atomic magnetometry technique results in more than two orders of magnitude increase in NMORE signal as well as greater than 6dB increase of magnetic field detection sensitivity. The new technique may have broad applications in photon gates and switching operations.
We show theoretically the presence of an optical field polarization rotation blocking mechanism in single-probe-based magnetic field sensing schemes, revealing the root cause for extremely small nonlinear magneto-optical rotation (NMOR) signal in single-probe-based atomic magnetometers. We present a colliding-probe atomic magnetometer theory, analytically describing the principle of the first nonlinear-optical atomic magnetometer. This new atomic magnetometry technique breaks the NMOR blockade in single-probe atomic magnetometers, enabling an energy circulation that results in larger than 20-dB enhancement in NMOR signal as well as better than 6-dB improvement of magnetic field detection sensitivity. Remarkably, all experimental observations reported to date can be qualitatively well-explained using this colliding-probe atomic magnetometry theory without numerical computations. This colliding-probe atomic magnetometry technique may have broad applications in scientific and technological fields ranging from micro-Tesla magnetic resonance imaging to cosmic particle detection.
The nonlinear magneto-optical rotation (NMOR) effect has prolific applications ranging from precision mapping of Earth's magnetic field to biomagnetic sensing. Studies on collisional spin relaxation effects have led to ultrahigh magnetic field sensitivities using a single-beam Λ scheme with state-of-the-art magnetic shielding/compensation techniques. However, the NMOR effect in this widely used single-beam Λ scheme is peculiarly small, requiring complex radio-frequency phase-locking protocols. We show the presence of a previously unknown energy symmetry-based nonlinear propagation blockade and demonstrate an optical inelastic wave-mixing NMOR technique that breaks this NMOR blockade, resulting in an NMOR optical signal-to-noise ratio (SNR) enhancement of more than two orders of magnitude never before seen with the single-beam Λ scheme. The large SNR enhancement was achieved simultaneously with a nearly two orders of magnitude reduction in laser power while preserving the magnetic resonance linewidth. This new method may open a myriad of applications ranging from biomagnetic imaging to precision measurement of the magnetic properties of subatomic particles.
The nonlinear magneto-optical effect has significantly impacted modern society with prolific applications ranging from precision mapping of the Earth's magnetic field to bio-magnetic sensing. Pioneering works on collisional spin-exchange effects have led to ultra-high magnetic field detection sensitivities at the level of fT/HzfT/\sqrt{Hz}fT/Hz​ using a single linearly-polarized probe light field. Here we demonstrate a nonlinear Zeeman-coherence parametric wave-mixing optical-atomic magnetometer using room temperature rubidium vapor that results in more than a three-order-of-magnitude optical signal-to-noise ratio (SNR) enhancement for extremely weak magnetic field sensing. This unprecedented enhancement was achieved with nearly a two-order-of-magnitude reduction in laser power while preserving the sensitivity of the widely-used single-probe beam optical-atomic magnetometry method. This new method opens a myriad of applications ranging from bio-magnetic imaging to precision measurement of the magnetic properties of subatomic particles.
Nonlinear resonances in alkali metal vapor, which are detected by the magneto-optical rotation of the linear polarization of light, are actively used in quantum magnetometry to fabricate atomic magnetometers. The magneto-optical rotation in most such sensors is due to magnetic birefringence, and rotation angles usually do not exceed tens of milliradians. In this work, an experiment where magneto-optical resonances of linear polarization rotation of a probe wave are due to strong dichroism induced in a medium by a counterpropagating pump wave has been proposed. Both waves are in resonance with the Fg = 2 → Fe = 1 optical transition in the 87Rb D1 line (λ ≈ 795 nm). Experiments have been carried out with a 2-cm-long cylindrical cell filled with a buffer gas, and the maximum rotation angle is ≈390 mrad (22°) at a width of resonance of about 300 nT. The results show that the configuration proposed for the observation of magneto-optical rotation is promising for the fabrication of compact high-sensitivity atomic magnetometers.
Nonlinear resonances in alkali metal vapor, which are detected by the magneto-optical rotation of the linear polarization of light, are actively used in quantum magnetometry to fabricate atomic magnetometers. The magneto-optical rotation in most such sensors is due to magnetic birefringence, and rotation angles usually do not exceed tens of milliradians. In this work, an experiment where magneto-optical resonances of linear polarization rotation of a probe wave are due to strong dichroism induced in a medium by a counterpropagating pump wave has been proposed. Both waves are in resonance with the Fg = 2 → Fe = 1 optical transition in the 87Rb D1 line (λ ≈ 795 nm). Experiments have been carried out with a 2-cm-long cylindrical cell filled with a buffer gas, and the maximum rotation angle is ≈390 mrad (22°) at a width of resonance of about 300 nT. The results show that the configuration proposed for the observation of magneto-optical rotation is promising for the fabrication of compact high-sensitivity atomic magnetometers.
We report a rubidium atomic magnetometer based on pump-probe nonlinear magneto-optical rotation. The rubidium vapor cell is placed in a five-layer magnetic shield with inner coils that can generate uniform magnetic fields along the direction of pump beam, and the cell is also placed in the center of a Helmholtz coil that can generate an oscillating magnetic field perpendicular to the direction of pump beam. The atoms are optically pumped by circularly polarized pump beam along a constant magnetic field in a period of time, then the pump beam is turned off and a /2 pulse of oscillating magnetic field for 87Rb atoms is applied. After the above process, the individual atomic magnetic moments become phase coherent, resulting in a transverse magnetization vector precessing at the Larmor frequency in the magnetic field. The linearly polarized probing beam is perpendicular to the direction of magnetic field, and can be seen as a superposition of the left and right circularly polarized light. Because of the different absorptions and dispersions of the left and right circularly polarized light by rubidium atoms, the polarization direction of probing beam rotates when probing beam passes through rubidium vapor cell. The rotation of the polarization is subsequently converted into an electric signal through a polarizing beam splitter. Finally, the decay signal related to the transverse magnetization vector is measured. The Larmor frequency proportional to magnetic field is obtained by the Fourier transform of the decay signal. The value of magnetic field is calculated from the formula:B=(2/) f, where and f are the gyromagnetic ratio and Larmor frequency, respectively. In order to measure the magnetic field in a wide range, the tracking lock mode is proposed and tested. The atomic magnetometer can track the magnetic field jump of 1000 nT or 10000 nT, indicating that the atomic magnetometer has strong locking ability and can be easily locked after start-up. The main performances in different magnetic fields are tested. The results show that the measurement range of the atomic magnetometer is from 100 nT to 100000 nT, the extreme sensitivity is 0.2 pT/Hz1/2, and the magnetic field resolution is 0.1 pT. The transverse relaxation times of the transverse magnetization vector in different magnetic fields are obtained, and the relaxation time decreases with the increase of the magnetic field. When the measurement range is from 5000 nT to 100000 nT, the magnetic field sampling rate of the atomic magnetometer can be adjusted in a range from 1 Hz to 1000 Hz. The atomic magnetometer in high sampling rate can measure weak alternating magnetic field at low frequency. This paper provides an important reference for developing the atomic magnetometer with large measurement range, high sensitivity and high sampling rate.