Quantum Electronics

Optical pumping of ultracold thulium atoms to a lower level of the clock transition and study of their depolarisation

E.S. Fedorova, Dmitry O. Tregubov, Artem A. Golovizin, Gulnara A. Vishnyakova, D. Mishin, Daniil I. Provorchenko, Ksenia Yu. Khabarova, В. Н. Сорокин, N. Kolachevsky

Published May 8, 2019• 7 citations

Publisher

Abstract

Abstract The atomic energy levels corresponding to states with the zero projection of the total angular momentum have a weak sensitivity to certain sources of shifts and, therefore, are widely used in precision spectroscopy. The optical pumping of ultracold thulium atoms to the ground state level with the zero projection of the total angular momentum is described. The population dynamics of this state due to magnetic dipole − dipole interaction in an external magnetic field is studied.

DOI: 10.1070/qel16998

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Quantum Electronics

Optical pumping of ultracold thulium atoms to a lower level of the clock transition and study of their depolarisation

E.S. Fedorova, Dmitry O. Tregubov, Artem A. Golovizin, Gulnara A. Vishnyakova, D. Mishin, Daniil I. Provorchenko, Ksenia Yu. Khabarova, В. Н. Сорокин, N. Kolachevsky

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Publisher

Abstract

DOI: 10.1070/qel16998

Related papers

Measurement of absolute frequencies of transitions in thulium atoms

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K. O. Babichev, Daniil I. Provorchenko, D. Mishin +3 more

The deterministic excitation of thulium atoms from the ground vibrational state of the optical lattice potential to the first and second vibrational levels with efficiencies of 40 and 24%, respectively, has been demonstrated. The purity of the prepared vibrational states is at least 93 and 95% in the former and latter cases, respectively, and is limited by both the purity of the initial state and the non-resonant excitation of the clock transition carrier frequency. The obtained high efficiency and quality of the preparation of atoms in a given vibrational level make it possible to characterize and control the frequency shift of the clock transition due to the interaction of thulium atoms with the field of the optical lattice, which is necessary to achieve an uncertainty of 10–17 for the thulium optical clock.The deterministic excitation of thulium atoms from the ground vibrational state of the optical lattice potential to the first and second vibrational levels with efficiencies of 40 and 24%, respectively, has been demonstrated. The purity of the prepared vibrational states is at least 93 and 95% in the former and latter cases, respectively, and is limited by both the purity of the initial state and the non-resonant excitation of the clock transition carrier frequency. The obtained high efficiency and quality of the preparation of atoms in a given vibrational level make it possible to characterize and control the frequency shift of the clock transition due to the interaction of thulium atoms with the field of the optical lattice, which is necessary to achieve an uncertainty of 10–17 for the thulium optical clock.

Journal of Experimental and Theoretical Physics LettersMay 1, 20251 citation

Clock transition at

1.14 \mu \mathrm{m}

in neutral thulium is a promising candidate for compact and robust transportable optical clock due to its extremely low sensitivity to external electric and magnetic fields. Cold Tm atoms are now used in optical lattice clocks, quantum simulators and for the study of Bose-Einstein condensation and cold collision physics. In this work, we discuss experimentally measured absolute frequencies of the two transitions at 410.6 nm and 530.7 nm, used for laser cooling of thulium atoms, transition at 418.8 nm used for optical pumping and clock transition at 1140 nm. Using accurate laser spectroscopy in an ensemble of cold thulium atoms, we measured frequencies of these transitions using an optical frequency comb, which was referenced to an active hydrogen maser. Transition frequencies were measured with an uncertainty at one tenth of their natural linewidth, which is sufficient for cooling and pumping of thulium atoms. The uncertainty of the clock transition frequency is 30 Hz, which was limited by the maser frequency calibration with GNSS. Our results can find application in existing experiments with cold thulium atoms and especially in new projects.

{4f}^{13}{(}^{2}{F}_{7/2}^{o}{)6s}^{2}

, which indicates that the transition between the inner shells is weakly perturbed by surrounding helium atoms. The pressure dependence of the emission wavelength suggests that the symmetry of helium atoms distributed around a thulium atom in the solid phase is similar to that in the liquid phase. The emission intensity was stable and large in the solid phase since thulium atoms were trapped at a density of 10

{}^{10}

--10

{}^{11}

atoms/cm

{}^{3}

. The lifetime of the excited state was measured to be $7.09\ifmmode\pm\else\textpm\fi{}0.04$ $\ensuremath{\mu}$s, which was longer than that of the

{4f}^{12}{(}^{3}{H}_{6}{)5d}_{5/2}{6s}^{2}

{(6,5/2)}_{7/2}

state of free thulium atoms. The excited state is expected to be a mixed state of the

{4f}^{12}{5d6s}^{2}

and

{4f}^{13}6s6p

configurations. The metastable state

{4f}^{13}{(}^{2}{F}_{5/2}^{o}{)6s}^{2}

is populated by a radiative transition from this excited state and relaxes to the ground state through a magnetic dipole transition. The lifetime of the metastable state of a neutral thulium atom was measured to be $75\ifmmode\pm\else\textpm\fi{}3$ ms.