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Italian National Conference on Photonic Technologies (Fotonica)

Fourier transform spectroscopy: a tool for quantum optics studies

Gian Giuseppe Bentini, M. Chiarini, Agostino Desalvo

Published Jan 1, 2018• 0 citations
Publisher

Abstract

Most of the experimental interferometric setup are based on the Mach-Zehnder geometry. Usually in the experimental configurations the photons travel in air, at a speed v independent of λ. An integrated optics approach appears necessary both for practical applications and because it can be useful for fundamental optics studies because the transmitted photons are in a spatial coherent state. We exploited a hybrid setup integrating optical fibres and monolithic optical waveguides to implement an asymmetric nonlinear Mach-Zehnder Interferometer (ANLI). One arm of the interferometer was equipped with a single mode Er:LiNbO3 waveguide, acting as nonlinear component whereas the other arm was an undoped LiNbO3 single mode waveguide, used to obtain a phase shift through the application of a voltage ramp. We injected in the ANLI a 980 nm laser radiation to collect interferograms that could be ascribed exclusively to the pump photons, as all frequency conversion events are localized only in one arm of the interferometer. The Fourier Transform analysis of the experimental data allowed us to perform a n Interaction-Free Quantum Optics experiment. This is a novel approach that can be used because in quantum mechanics the wave functions of a state, expressed in terms of two conjugate variables, are Fourier Transform pairs. In fact, operating in the Fourier Transform time-frequency space-domain, we recovered the spectral composition, in the wavenumber space-domain, of the photons generated by the excitation of an Er3+ doped crystal placed in one arm of the interferometer.

DOI
10.1049/cp.2018.1628

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Most of the experimental interferometric setup are based on the Mach-Zehnder geometry. Usually in the experimental configurations the photons travel in air, at a speed v independent of λ. An integrated optics approach appears necessary both for practical applications and because it can be useful for fundamental optics studies because the transmitted photons are in a spatial coherent state. We exploited a hybrid setup integrating optical fibres and monolithic optical waveguides to implement an asymmetric nonlinear Mach-Zehnder Interferometer (ANLI). One arm of the interferometer was equipped with a single mode Er:LiNbO3 waveguide, acting as nonlinear component whereas the other arm was an undoped LiNbO3 single mode waveguide, used to obtain a phase shift through the application of a voltage ramp. We injected in the ANLI a 980 nm laser radiation to collect interferograms that could be ascribed exclusively to the pump photons, as all frequency conversion events are localized only in one arm of the interferometer. The Fourier Transform analysis of the experimental data allowed us to perform a n Interaction-Free Quantum Optics experiment. This is a novel approach that can be used because in quantum mechanics the wave functions of a state, expressed in terms of two conjugate variables, are Fourier Transform pairs. In fact, operating in the Fourier Transform time-frequency space-domain, we recovered the spectral composition, in the wavenumber space-domain, of the photons generated by the excitation of an Er3+ doped crystal placed in one arm of the interferometer.
Quantum optics has become a key field of development for investigations of quantum physics principles, leading to novel quantum technologies. In this view Integrated Optics allows implementing complex quantum circuits that can give rise to significant outcomes, difficult to reach using traditional approaches based on discrete components. In this framework, a non-linear Mach-Zehnder Interferometer (MZI) was implemented by using two commercial 50:50 directional fibre couplers. One of the MZI arms was equipped with a single mode Er:LiNbO3 optical waveguide, acting as non-linear component whereas the other MZI arm was provided with an undoped LiNbO3 single mode optical waveguide, used to obtain a phase shift through the application of a controlled voltage ramp. The injection in the MZI of a 980nm wavelength laser radiation allowed to collect structured interferogrammes, that could be ascribed exclusively to the pump photons, as all frequency conversion events are localized only in one arm of the Interferometer. The Fourier Transform elaboration of such interferogrammes, produces multiple peak spectra that tightly match the typical transition spectrograms of Er:LiNbO3 when excited by a 980nm radiation. Thus it is possible to perform a spectrometry of the noninterfering converted photons only by using the interfering pump photons. In this work, the experimental apparatus and the most interesting results, obtained in different experimental conditions, are described. Finally, a possible interpretation is outlined.
One of the main challenges in quantum computing is implementing algorithms within quantum optical free-space and integrated circuits. This research focuses on the quantum addition algorithm, derived from the Deutsch-Jozsa algorithm, to advance quantum computing using optical technologies. The developed quantum optical integrated circuit is built on a hybrid substrate with interconnected components on a silicon dioxide base. Qubits and their states are arranged according to the requirements of each quantum algorithm. In the Fourier transform section, qubits act as propagation modes within silicon waveguides, with emitted photons representing the Fourier transform after traveling a distance of π/2. The phase-shifting section consists of two parts: one shifts the phase of incoming photons by π, while the other modulates this shift based on the quantum full adder algorithm. The first employs a photonic crystal for short phase shifts, which are adjusted via impurities in the silicon substrate and controlled by an electro-optic circuit. Additionally, single-mode waveguides made of silicon dioxide and air serve as qubits. By coupling photon amplitudes, a comparator circuit is triggered based on the generated output. Through these integrations, the sum of two quantum numbers can be represented at the output. This underscores the importance of designing and simulating a full adder within quantum optical integrated circuits to address the complexities inherent in quantum computing.
Abstract Quantum interferometry based on induced-coherence phenomena has demonstrated the possibility of undetected-photon measurements. Perturbation in the optical path of probe photons can be detected by interference signals generated by quantum mechanically correlated twin photons propagating through a different path, possibly at a different wavelength. To the best of our knowledge, this work demonstrates for the first time a hybrid-type induced-coherence interferometer that incorporates a Mach–Zehnder-type interferometer for near-visible photons and a Michelson-type interferometer for infrared (IR) photons, based on double-pass-pumped spontaneous parametric down-conversion. This configuration enables IR optical measurements via the detection of near-visible photons and provides methods for optimizing the quality of measurements by identifying photon pairs of different origins. We theoretically identify that the induced-coherence interference visibility is approximately the same as the heralding efficiency between twin photons along the relevant spatial modes, and experimentally maximize the visibility by setting up a common reference spatial mode for IR photons. Applications to both time-domain and frequency-domain quantum optical induced-coherence tomography for three-dimensional test structures are demonstrated. The results prove the feasibility of practical undetected-photon sensing and imaging techniques based on the presented structure.
We show several quantum-sensing experimental realizations dedicated to the qualification of optical-material key-properties, such as chromatic dispersion and refractive index variations. More specifically, the material under test (typically, an optical fibre or a nonlinear crystal) is introduced in one of the two arms or in the loop of interferometric devices, mainly in Mach-Zehnder and Sagnac configurations. Probing such devices using peculiar quantum, or quantum-mimicking, photonic states creates material-under-test-dependent relative-phase differences that are imprinted on the established coherent superposition. Here, the employed photonic states exhibit specific modal structures, in the frequency and/or spatial domains, that exploit or mimic quantum entanglement, providing access to the relative phases and to the optical properties under investigation. Associated measurement results show unprecedented precision and/or accuracy, reduced overhead, and otherwise unreachable stability and repeatability. Such quantum interferometric methods pave the way to redefining the very way optical materials are characterized, finding repercussion in various fields ranging from fundamental optics to industry-grade developments.
We propose and demonstrate a method for measuring the joint spectrum of photon pairs via Fourier spectroscopy. The biphoton spectral intensity is computed from a two-dimensional interferogram of coincidence counts. The method has been implemented for a type-I downconversion source using a pair of common-path Mach-Zehnder interferometers based on Soleil compensators. The experimental results agree well with calculated frequency correlations that take into account the effects of coupling into single-mode fibers. The Fourier method is advantageous over scanning spectrometry when detectors exhibit high dark count rates leading to dominant additive noise.