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Quantum Sensing and Nano Electronics and Photonics

Entanglement-enabled qualification of optical-material properties

Romain Dalidet, Anthony Martin, Grégory Sauder, Laurent Labonté, Sébastien Tanzilli

Published Mar 21, 2025• 0 citations
Publisher

Abstract

We show several quantum-sensing experimental realizations dedicated to the qualification of optical-material key-properties, such as chromatic dispersion and refractive index variations. More specifically, the material under test (typically, an optical fibre or a nonlinear crystal) is introduced in one of the two arms or in the loop of interferometric devices, mainly in Mach-Zehnder and Sagnac configurations. Probing such devices using peculiar quantum, or quantum-mimicking, photonic states creates material-under-test-dependent relative-phase differences that are imprinted on the established coherent superposition. Here, the employed photonic states exhibit specific modal structures, in the frequency and/or spatial domains, that exploit or mimic quantum entanglement, providing access to the relative phases and to the optical properties under investigation. Associated measurement results show unprecedented precision and/or accuracy, reduced overhead, and otherwise unreachable stability and repeatability. Such quantum interferometric methods pave the way to redefining the very way optical materials are characterized, finding repercussion in various fields ranging from fundamental optics to industry-grade developments.

DOI
10.1117/12.3038907

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We show several quantum-sensing experimental realizations dedicated to the qualification of optical-material key-properties, such as chromatic dispersion and refractive index variations. More specifically, the material under test (typically, an optical fibre or a nonlinear crystal) is introduced in one of the two arms or in the loop of interferometric devices, mainly in Mach-Zehnder and Sagnac configurations. Probing such devices using peculiar quantum, or quantum-mimicking, photonic states creates material-under-test-dependent relative-phase differences that are imprinted on the established coherent superposition. Here, the employed photonic states exhibit specific modal structures, in the frequency and/or spatial domains, that exploit or mimic quantum entanglement, providing access to the relative phases and to the optical properties under investigation. Associated measurement results show unprecedented precision and/or accuracy, reduced overhead, and otherwise unreachable stability and repeatability. Such quantum interferometric methods pave the way to redefining the very way optical materials are characterized, finding repercussion in various fields ranging from fundamental optics to industry-grade developments.
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Optical phase measurements play a key role in the detection of macroscopic parameters such as position, velocity, and displacement. They also permit to qualify the microscopic properties of photonic waveguides such as polarization mode dispersion, refractive index difference, and chromatic dispersion. In the quest for ever-better measurement performance and relevance, we report a quantum nonlinear interferometer based on a Sagnac configuration allowing precise, accurate, self-stabilized, and reproductible optical phase measurement. The potential of this system is demonstrated through the measurement of second-order dispersion, namely, chromatic dispersion of a commercial dispersion-shifted fiber at telecommunication wavelength. We demonstrate a precision of 0.007 % , surpassing state-of-the-art measurements by more than one order of magnitude. Additionally, the accuracy of the second-order dispersion value is determined through the measurement of the third-order dispersion, showing a quadratic error as low as 5%. Our system promises the development of photonic-based sensors enabling the measurements of optical-material properties in a user-friendly manner.
White-light interferometry is one of today's most precise tools for determining the properties of optical materials. Its achievable precision and accuracy are typically limited by systematic errors due to a high number of interdependent data-fitting parameters. Here, we introduce spectrally resolved quantum white-light interferometry as a novel tool for optical property measurements, notably, chromatic dispersion in optical fibres. By exploiting both spectral and photon-number correlations of energy-time entangled photon pairs, the number of fitting parameters is significantly reduced, which eliminates systematic errors and leads to an absolute determination of the material parameter. By comparing the quantum method to state-of-the-art approaches, we demonstrate the quantum advantage of 2.4 times better measurement precision, despite requiring 62 times fewer photons. The improved results are due to conceptual advantages enabled by quantum optics, which are likely to define new standards in experimental methods for characterising optical materials.
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Infrared (IR) spectroscopy and imaging are important tools in metrology, including material analysis, sensing and characterization. Although conventional methods of IR metrology are available, they face challenges related to the high cost and low efficiency of IR light sources and photodetectors. These challenges can be addressed by circumventing the need for IR-range components using tools and techniques of quantum optics. In this thesis, we describe a technique for IR measurements, which requires using only accessible light sources and detectors operating in the visible range. Our technique is based on the nonlinear interference of correlated photon pairs generated via spontaneous parametric down conversion (SPDC). In SPDC, a photon from the pump laser generates a pair of correlated photons within a nonlinear crystal. One photon of the pair can be generated in the visible range, and the other in the IR range. Two identical nonlinear crystals pumped by the same laser form the nonlinear interferometer, where interference of the visible SPDC photons can be observed. The interference pattern of the visible photons depends on amplitudes and phases of the IR photons, which are used to probe the properties of the medium under study. Hence, by observing the interference of the visible photons we infer the IR properties of the media, without direct measurements of IR light. We applied the nonlinear interference method to realize the IR spectroscopy, IR optical coherence tomography (OCT), IR imaging and IR polarimetry. In the IR spectroscopy experiment, we simultaneously and independently measured both refractive index and absorption coefficient of various samples in the IR range, while only detecting photons in the visible range. In IR OCT and IR imaging schemes, we measured the reflectivity of the interfaces of the sample, performed 3D raster and wide field imaging through opaque (in the visible range) materials. In the IR polarimetry, we measured the birefringence of the samples. We studied glass, organic polymer, Silicon and CO2 gas, but our method can be applied to a broad variety of samples. Our method is widely tunable and has high precision and accuracy over mid-IR wavelengths. This work paves the way for further practical adoption of the method in the field of IR metrology, without the need for IR grade detectors and sources.