This dissertation describes research to coherently control quantum states of superconducting devices. In the first project, the state of an 8 GHz 3D superconducting Al cavity at 20mK was manipulated to add a quantum of excitation. Preparing a harmonic resonator in a state with a well-defined number of excitations (Fock states) is not possible using one external classical drive. I generated Fock states by transferring a single excitation from a 5.5 GHz transmon qubit to a cavity using Stimulated Raman Adiabatic Passage (STIRAP). I also extended the STIRAP technique to put the cavity in higher Fock states, superpositions of Fock states, and Bell states between the qubit and the cavity. Master-equation simulations of the system’s density matrix were in good agreement with the data, and I obtained estimated fidelities of 89%, 68% and 43% for the first three Fock states, respectively. The second project involved implementing an entangling gate between two Al/AlOx/Al transmon qubits that were mounted in an Al cavity and cooled to 20mK. Pertinent system frequencies were as follows: one qubit was at 6.0 GHz, the other qubit at 6.8 GHz, the cavity at 7.7 GHz, and the qubit-qubit dispersive shift was -1MHz. By applying a specially-shaped pulse of duration tg = 907ns, I implemented a generalized CNOT gate using an all-microwave technique known as Speeding up Waveforms by Inducing Phases to Harmful Transitions (SWIPHT). Using quantum process tomography, I found that the gate fidelity was 80%–82%, close to the 87% fidelity expected from decoherence in the transmons during the gate time. Details of the device fabrication, device characterization, measurement techniques, and extensive modeling of device behavior are presented, along with chi-matrix characterization of single-qubit gates and SWIPHT gates.
This dissertation describes research to coherently control quantum states of superconducting devices. In the first project, the state of an 8 GHz 3D superconducting Al cavity at 20mK was manipulated to add a quantum of excitation. Preparing a harmonic resonator in a state with a well-defined number of excitations (Fock states) is not possible using one external classical drive. I generated Fock states by transferring a single excitation from a 5.5 GHz transmon qubit to a cavity using Stimulated Raman Adiabatic Passage (STIRAP). I also extended the STIRAP technique to put the cavity in higher Fock states, superpositions of Fock states, and Bell states between the qubit and the cavity. Master-equation simulations of the system’s density matrix were in good agreement with the data, and I obtained estimated fidelities of 89%, 68% and 43% for the first three Fock states, respectively. The second project involved implementing an entangling gate between two Al/AlOx/Al transmon qubits that were mounted in an Al cavity and cooled to 20mK. Pertinent system frequencies were as follows: one qubit was at 6.0 GHz, the other qubit at 6.8 GHz, the cavity at 7.7 GHz, and the qubit-qubit dispersive shift was -1MHz. By applying a specially-shaped pulse of duration tg = 907ns, I implemented a generalized CNOT gate using an all-microwave technique known as Speeding up Waveforms by Inducing Phases to Harmful Transitions (SWIPHT). Using quantum process tomography, I found that the gate fidelity was 80%–82%, close to the 87% fidelity expected from decoherence in the transmons during the gate time. Details of the device fabrication, device characterization, measurement techniques, and extensive modeling of device behavior are presented, along with chi-matrix characterization of single-qubit gates and SWIPHT gates.
Superconducting devices as quantum bits (qubits) are one of the most promising candidates for implementing a practical quantum computer. Over the last decade, quantum coherence times of superconducting qubits have been continuously improved. Operating qubits in noise insensitive points, eliminating the participation of the lossy materials, and better isolation from environment increased the decoherence times from nanoseconds to tens of microseconds. One recent approach on the qubit design is to shunt the Josephson junctions with large capacitors to reduce the sensitivity to noise and to redistribute the stored electromagnetic energy in a well-engineered area. This approach was first applied on charge qubits and later adopted to other types of superconducting qubits. \n \nIn this thesis, we present the design and the characterization of a three-Josephson junction superconducting circuit with three large shunt capacitors. We present experiments on decoherence in the circuit used as a qubit. The qubit relaxation time T₁ is reaching as high as 47 μs and the spin-echo dephasing time T₂ = 9.4 μs. In addition, we present spectroscopy experiments and decoherence characterization in the qutrit subspace formed by the lowest three energy levels. The spectroscopy data is in excellent agreement with the complete circuit model based on the system capacitance matrix. At the flux symmetry point, the circuit has a large anharmonicity, defined as the difference between the 1-2 and 0-1 transition frequencies, approaching 2π × 3.7 GHz, which is enabling fast single qubit operations. We performed randomized benchmarking with the qubit gates with a duration of 1.62 ns and an average gate fidelity of 99.9%. \n \nMoreover, we present experiments with multi-level control in qutrit subspace, formed by the lowest three energy levels. We demonstrate a single step experimental implementation of a generalized Walsh-Hadamard gate. We use a decomposition of the quantum gate into two unitary operations, one implemented by an off-diagonal Hamiltonian and the other implemented by a diagonal Hamiltonian. The off-diagonal Hamiltonian is obtained by the simultaneous driving of the transitions between levels 0-1, 1-2, and 0-2, with the latter being a two-photon process. The diagonal Hamiltonian is effectively implemented by appropriately shifting the phases of adjacent pulses. The gate is characterized using tomography process and the average fidelity exceeds 90%, in good agreement with numerical simulations that take into account the multi-level structure of the system.
Superconducting transmon qubits comprise one of the most promising platforms for quantum information processing due to their long coherence times and to their scalability into larger qubit networks. However, their weakly anharmonic spectrum leads to spectral crowding in multiqubit systems, making it challenging to implement fast, high-fidelity gates while avoiding leakage errors. To address this challenge, we use a protocol for speeding up waveforms by inducing phases to harmful transitions (SWIPHT) [S. E. Economou and E. Barnes, Phys. Rev. B 91, 161405(R) (2015)], which yields smooth, simple microwave pulses designed to suppress leakage without sacrificing gate speed through spectral selectivity. Here, we determine the parameter regimes in which SWIPHT is effective and demonstrate that in these regimes, it systematically produces two-qubit gate fidelities for cavity-coupled transmons in the range 99.6%--99.9% with gate times as fast as 23 ns. Our results are obtained from full numerical simulations that include current experimental levels of relaxation and dephasing. These high fidelities persist over a wide range of system parameters that encompass many current experimental setups and are insensitive to small parameter variations and pulse imperfections.
Logic gates in superconducting quantum processors are implemented through precisely shaped microwave pulses, whose durations are constrained by both device coherence and the multilevel structure of artificial atoms. While single-qubit fidelities above 0.999 are routinely achieved, the physical execution time of these gates remains a major bottleneck for deep quantum circuits. Here we examine single-qubit control across adiabatic [where the rotating-wave approximation (RWA) is valid], intermediate, and diabatic driving regimes using both an ideal two-level model and a realistic weakly anharmonic transmon Hamiltonian. By sweeping pulse durations and drive strengths over experimentally relevant ranges, we compare performance trade-offs and identify the conditions under which ultrashort gates remain viable. Our simulations uncover a quantitative speed-limit mechanism intrinsic to weakly anharmonic superconducting qubits: leakage to higher levels rises sharply once the peak Rabi rate exceeds a fixed fraction of the anharmonicity. Across all pulse shapes and driving regimes studied, we find a consistent numerical threshold at Ω max /|Δ|≈0.15−0.20, where Ω max denotes the peak drive (Rabi) amplitude and Δ is the transmon anharmonicity. Beyond this ratio, gate fidelity deteriorates regardless of waveform engineering. This boundary, obtained from full multilevel time-domain simulations spanning adiabatic, intermediate, and diabatic regimes, constitutes a previously unreported characterization of the fundamental leakage barrier in transmon devices. Our results, therefore, provide the first unified quantitative map linking pulse duration, driving strength, and anharmonicity, establishing why realistic superconducting qubits cannot sustain picosecond-scale gates despite ideal two-level predictions, and offering a practical benchmark for next-generation architectures seeking shorter, high-fidelity control.
Recent experimental work on superconducting transmon qubits in three-dimensional (3D) cavities shows that their coherence times are increased by an order of magnitude compared to their two-dimensional cavity counterparts. However, to take advantage of these coherence times while scaling up the number of qubits it is advantageous to address individual qubits which are all coupled to the same 3D cavity fields. The challenge in controlling this system comes from spectral crowding, where the leakage transition of qubits is close to computational transitions in other qubits. Here, it is shown that fast pulses are possible which address single qubits using two-quadrature control of the pulse envelope, while the derivative removal by adiabatic gate method of Motzoi et al. [Phys. Rev. Lett. 103, 110501 (2009)] alone only gives marginal improvements over the conventional Gaussian pulse shape. On the other hand, a first-order result using the Magnus expansion gives a fast analytical pulse shape which gives a high-fidelity gate for a specific gate time, up to a phase factor on the second qubit. Further numerical analysis corroborates these results and yields to even faster gates, showing that leakage-state anharmonicity does not provide a fundamental quantum speed limit.
Superconducting circuits are one of the leading architectures in quantum computing. To undertake quantum computing one must be able to perform quantum gates; however, two-qubit gates are still limited in fidelity and gate time. The cross-resonance gate is a two-qubit gate that uses direct microwave drives and has seen much success in its implementation; but, there are theoretical indications that it has not yet reached the coherence limited fidelity value and its gate time is still relatively long compared with other quantum gate methods. Quantum optimal control theory is a powerful tool in the design of controls for quantum operations and has shown the capability to improve gate fidelities and reduce gate times. Robust quantum optimal control methodologies have further built on this to develop high fidelity quantum gates that are robust to uncertainties and noise in the system. In this thesis we use robust quantum optimal control theory to achieve these goals for the cross-resonance gate in a variety of superconducting qubit architectures. First, we investigate two superconducting qubits embedded in a common 3D microwave cavity in which the control drive is implemented via the common cavity mode of the cavity. We determine pulse shapes that implement the cross-resonance gate that are robust to uncertainty in the qubit transition frequencies for both a strictly two-level superconducting qubit and a three-level qubit. Second, we look at the cross-resonance gate with direct drives on each qubit, finding the minimal time to perform the cross-resonance gate with pulses that are robust to uncertainty in a measured system parameter for three cases: two three-level qubits with no drive crosstalk, two three-level qubits with some drive crosstalk, and two two-level qubits. Lastly, we report on simulations undertaken towards implementing a robust, high fidelity cross-resonance gate in a novel superconducting quantum device known as the coaxmon.
A possible building block for a scalable quantum computer has recently been demonstrated [Mariantoni et al., Science 334, 61 (2011)]. This architecture consists of superconducting qubits capacitively coupled both to individual memory resonators as well as a common bus. In this work we study a natural primitive entangling gate for this and related resonator-based architectures, which consists of a controlled-${\ensuremath{\sigma}}^{z}$ (cz) operation between a qubit and the bus. The cz gate is implemented with the aid of the noncomputational qubit $|2\ensuremath{\rangle}$ state [Strauch et al., Phys. Rev. Lett. 91, 167005 (2003)]. Assuming phase or transmon qubits with 300 MHz anharmonicity, we show that by using only low frequency qubit-bias control it is possible to implement the qubit-bus cz gate with 99.9 (99.99) fidelity in about 17ns (23ns) with a realistic two-parameter pulse profile, plus two auxiliary z rotations. The fidelity measure we refer to here is a state-averaged intrinsic process fidelity, which does not include any effects of noise or decoherence. These results apply to a multiqubit device that includes strongly coupled memory resonators. We investigate the performance of the qubit-bus cz gate as a function of qubit anharmonicity, identify the dominant intrinsic error mechanism and derive an associated fidelity estimator, quantify the pulse shape sensitivity and precision requirements, simulate qubit-qubit cz gates that are mediated by the bus resonator, and also attempt a global optimization of system parameters including resonator frequencies and couplings. Our results are relevant for a wide range of superconducting hardware designs that incorporate resonators and suggest that it should be possible to demonstrate a 99.9 cz gate with existing transmon qubits, which would constitute an important step towards the development of an error-corrected superconducting quantum computer.