Quantum Optics
It becomes increasingly difficult to detect long-wavelength single photons because of thermal fluctuations in the background. This can pose problems for single-photon detection for fields such as astronomy and nuclear magnetic resonance imaging. Gely et al. used a superconducting qubit, initially developed for circuit quantum electrodynamics (cQED) and quantum information processing for microwaves, to directly observe the quantization of radio-frequency electromagnetic fields stored in a photonic microresonator. They were then able to manipulate the quantum state of the radio-frequency field, forming one- and two-photon Fock states within the microresonator, and analyze how the system interacts dynamically with its environment. The cQED approach could be used for fundamental studies in quantum thermodynamics and also find practical application in imaging.
Science , this issue p. [1072][1]
[1]: /lookup/doi/10.1126/science.aaw3101
Quantum Optics
It becomes increasingly difficult to detect long-wavelength single photons because of thermal fluctuations in the background. This can pose problems for single-photon detection for fields such as astronomy and nuclear magnetic resonance imaging. Gely et al. used a superconducting qubit, initially developed for circuit quantum electrodynamics (cQED) and quantum information processing for microwaves, to directly observe the quantization of radio-frequency electromagnetic fields stored in a photonic microresonator. They were then able to manipulate the quantum state of the radio-frequency field, forming one- and two-photon Fock states within the microresonator, and analyze how the system interacts dynamically with its environment. The cQED approach could be used for fundamental studies in quantum thermodynamics and also find practical application in imaging.
Detecting weak radio-frequency electromagnetic fields plays a crucial role in a wide range of fields, from radio astronomy to nuclear magnetic resonance imaging. In quantum optics, the ultimate limit of a weak field is a single photon. Detecting and manipulating single photons at megahertz frequencies presents a challenge because, even at cryogenic temperatures, thermal fluctuations are appreciable. Using a gigahertz superconducting qubit, we observed the quantization of a megahertz radio-frequency resonator, cooled it to the ground state, and stabilized Fock states. Releasing the resonator from our control, we observed its rethermalization with nanosecond resolution. Extending circuit quantum electrodynamics to the megahertz regime, we have enabled the exploration of thermodynamics at the quantum scale and allowed interfacing quantum circuits with megahertz systems such as spin systems or macroscopic mechanical oscillators.
Circuit quantum electrodynamics is a currently very active field of research. Since the discoveries that an artificial spin, the so-called qubit, can be implemented using a superconducting non-linear circuit and can coherently interact with the electromagnetic field at the single-photon level, it has gathered strong interest for its potential for quantum computing but also for its ability to create, manipulate and detect microwave states with an exquisite precision. This manuscript describes three experiments harnessing and building on the tools and concepts developed for circuit quantum electrodynamics to couple microwave fields to other fundamental entities, namely phonons and electron spins. In a first experiment, we show the coherent coupling of superconducting to surface acoustic wave phonons. It demonstrates that acoustic waves can be used to carry quantum information and distribute entanglement. We then explore the coupling of superconducting circuits to electronic spins, and its potential for sensing and quantum information storage. The second experiment concentrates at building a high-sensitivity spectrometer able to detect spins in picoliter sized samples, targeting samples from chemical or biological origins. The third experiment is about implementing a quantum memory using a spin ensemble possessing second-long coherence. We namely explore the potential of circuit-enhanced radiation cooling to polarize the spin ensemble and enhance the efficiency of the quantum memory storage.
In this PhD thesis, we will present the theoretical and experimental work that led to the realization of a radio-frequency circuit quantum electrodynamics system (RFcQED). In chapter 2, we provide a detailed derivation of the Hamiltonian of circuit QED formulated in the context of the Rabi model, and extract expressions for the cross-Kerr interaction. The resulting requirements for the coupling rate in RFcQED are discussed, one of them being the need to dramatically increase the coupling rate compared to typical circuit QED device. In chapter 3 we cover two experimental approaches to increasing the coupling in a circuit QED system, one making use of a high impedance resonator, the second utilizing a large coupling capacitor. In chapter 4, we combine these two approaches to implement RFcQED. Through strong dispersive coupling, we could measure individual photons in a megahertz resonator, demonstrate quantum control by cooling the resonator to the ground state or preparing Fock states, and finally observe with nanosecond resolution the re-thermalization of these states. In chapter 5 we present QuCAT or Quantum Circuit Analyzer Tool in Python, a software package that can be used for the design of circuit QED systems such as the one presented in this thesis. In chapter 6 we discuss how certain interplays between general relativity and quantum mechanics cannot be described using our current laws of physics. In particular, we show how radio-frequency mechanical oscillators are perfect candidates to perform experiments in this regime. In chapter 7 we present the prospects for coupling such mechanical oscillator to weakly anharmonic superconducting circuits such as the transmon qubit or RFcQED systems.
Superconducting quantum bits (qubits) are a leading candidate towards realizing a processor that is able to outperform existing classical computers at select tasks. One particular qubit architecture, the transmon, boasts long coherence times compared to required gate lengths and flexibility with respect to circuit couplings as these 'artificial atoms' are photolithographically defined. These attributes allow qubits to be leveraged for other tasks as well — such as efficiently detecting itinerant microwave photons. Such a device may prove useful for remote entanglement protocols, quantum optics experiments in the microwave regime, and as a detector for low-mass dark matter.Through a blend of circuit quantum electrodynamics (cQED) and waveguide quantum electrodynamics (wQED) theories, high detector performance was achieved even when the photon arrival time was not known. Utilizing an ensemble (N = 4) of identical transmon absorbers, photon mediated interactions along a common waveguide enable absorbed itinerant photons to be trapped for longer than the inverse of the bandwidth of an individual qubit. This extended trapping time allows for sufficient integration of the dispersively shifted readout resonator to resolve deviations from vacuum with high fidelity.
Using modern micro and nano-fabrication techniques combined with superconducting materials we realize quantum electronic circuits in which we create, store, and manipulate individual microwave photons. The strong interaction of photons with superconducting quantum two-level systems allows us to probe fundamental quantum effects of microwave radiation and also to develop components for applications in quantum technology. Previously we have realized on-demand single photon sources which we have characterized using correlation function measurements [1] and full quantum state tomography [2]. For this purpose we have developed efficient methods to separate the quantum signals of interest from the noise added by the linear amplifiers used for quadrature amplitude detection [3]. We now regularly employ superconducting parametric amplifiers [4] to perform nearly quantum limited detection of propagating electromagnetic fields. These enable us to probe the entanglement which we generate on demand between stationary qubits and microwave photons freely propagating down a transmission line [5]. Using two independent microwave single photon sources, we have recently performed Hong-Ou-Mandel experiments at microwave frequencies [6] and have probed the coherence of two-mode multi-photon states at the out-put of a beam-splitter. The non-local nature of such states may prove to be useful for distributing entanglement in future small-scale quantum networks.
Atoms and photons, two things so different but yet so alike. The former, the building block of matter, something we learn about in school and imagine it as some tiny marbles encircled by other tinier marbles. The latter, an electromagnetic wave, a light particle or an excitation of the electromagnetic field. Quantum mechanics tells us about the properties of these two entities. And even if it sounds, looks and writes counter-intuitive, it has proven right for over a century now. In this work, I elaborate on how we tested the laws of quantum mechanics and how we used them learn more about the tiny building blocks of nature and the fields they use to talk to each other. The atoms we use, are artificial. Superconducting qubits, small electrical circuits with quantized energy levels behave like electrons that transition between different orbitals in an atom. One of the qubits' advantages, is also a big disadvantage. We design the circuits' energy levels and fabricate them in a cleanroom. This allows for arbitrary spaced energy levels but in contrast to real atoms, prevents two superconducting qubits from being alike. Still, this qubit platform is one of the frontrunners for future quantum computing technology and testing fundamental physics due to their scalability. We interface superconducting qubits, which operate in the GHz regime, with microwave photons. We use 3D aluminum cavities as mediators between qubits and photons. The cavities allow for non-destructive readout of the qubit state, they shield the qubits from noise at the qubit frequency and they give us an easy way to frequency-tune these joint systems. We need to operate superconducting qubits and their cavities at millikelvin temperatures in dilution refrigerators. At higher temperatures, superconductivity suffers and even worse, the environment is filled with thermal noise photons. This poses a fundamental limitation on the scalability of superconducting qubit devices. Also connecting multiple devices in different fridges does not work over room temperature links because the microwave photons used for this purpose will be covered in noise and the quantum information they carry, will be unusable. Infrared photons do not suffer from this noise problem since there are close to zero thermal noise photons at their frequencies at room temperature. We cannot simply interface superconducting devices with optical photons due their frequency mismatch and the destructive effect of optical photons on superconductors. Therefore, we use microwave-to-optics transducers that allow to convert microwave photons into optical ones and vice-versa. The transducers that we use are macroscopic electro-optic transducers using the Pockels effect in a disk-shaped Lithium Niobate whispering gallery mode resonator. By using a strong optical pump, photons from the two frequency domains experience a beam-splitter interaction and get converted from one to the other. We measure the generated optical photons using elaborate optical setups, optical heterodyning and single photon detectors to gain knowledge about the qubit state or the converted microwave photons. Bridging the microwave and the optical world allows us to take advantage of both of their strengths but it also requires deep knowledge about both of their working principles. In this work, we describe two experiments that our group conducted to showcase the opportunities that arise from interfacing superconducting qubits with optical photons but also the pitfalls, one may encounter on the way. In the first experiment, we managed to all-optically read out a superconducting qubit. We show that the assignment fidelity, the probability that a measurement of the qubit state matches the prepared state, is close to equal for all-optical, microwave-to-optics and conventional microwave readout. We show T1 and T2 measurements for all three readout types and give an analysis of the noise caused by the optics. Finally, we show that the infrared light does not affect the qubit performance in a negative way but that the heating it causes does. This is an important insight that we used in the next experiment. The second experiment is the upconversion of itinerant single microwave photons to the optical domain. We show that we can generate single microwave photons from a qubit-cavity system. We upconvert these single photons, measure them with a single photon detector and reconstruct their shape. By conducting a single photon Rabi measurement, we show correlations between the microwave and the optical domain. And by thorough signal-to-noise measurements and noise analysis, we find that we can generate single infrared photons with high signal-to-noise ratio 5.1 and low transducer added noise (<0.012 quanta). We show that this measurement creates a path towards entanglement of a superconducting qubit and an optical photon and what parameters need to be improved to achieve it. Additionally, this experiment is a proof of principle for an on-demand infrared single photon source. More generally, it allows to link microwave quantum technology in general to the optical domain.