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arXiv:1901.07267 · Science

Observation and stabilization of photonic Fock states in a hot radio-frequency resonator

Mario F. Gely, Marios Kounalakis, Christian Dickel, Jacob Dalle, Rémy Vatré, Brian Baker, M. Jenkins, Gary Alexander Steele

Published Mar 8, 2019• 47 citations
arXivHTMLPDF

Abstract

Detecting weak radio-frequency electromagnetic fields plays a crucial role in a wide range of fields, from radio astronomy to nuclear magnetic resonance imaging. In quantum optics, the ultimate limit of a weak field is a single photon. Detecting and manipulating single photons at megahertz frequencies presents a challenge because, even at cryogenic temperatures, thermal fluctuations are appreciable. Using a gigahertz superconducting qubit, we observed the quantization of a megahertz radio-frequency resonator, cooled it to the ground state, and stabilized Fock states. Releasing the resonator from our control, we observed its rethermalization with nanosecond resolution. Extending circuit quantum electrodynamics to the megahertz regime, we have enabled the exploration of thermodynamics at the quantum scale and allowed interfacing quantum circuits with megahertz systems such as spin systems or macroscopic mechanical oscillators.

DOI
10.1126/science.aaw3101

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Detecting weak radio-frequency electromagnetic fields plays a crucial role in a wide range of fields, from radio astronomy to nuclear magnetic resonance imaging. In quantum optics, the ultimate limit of a weak field is a single photon. Detecting and manipulating single photons at megahertz frequencies presents a challenge because, even at cryogenic temperatures, thermal fluctuations are appreciable. Using a gigahertz superconducting qubit, we observed the quantization of a megahertz radio-frequency resonator, cooled it to the ground state, and stabilized Fock states. Releasing the resonator from our control, we observed its rethermalization with nanosecond resolution. Extending circuit quantum electrodynamics to the megahertz regime, we have enabled the exploration of thermodynamics at the quantum scale and allowed interfacing quantum circuits with megahertz systems such as spin systems or macroscopic mechanical oscillators.
Quantum Optics It becomes increasingly difficult to detect long-wavelength single photons because of thermal fluctuations in the background. This can pose problems for single-photon detection for fields such as astronomy and nuclear magnetic resonance imaging. Gely et al. used a superconducting qubit, initially developed for circuit quantum electrodynamics (cQED) and quantum information processing for microwaves, to directly observe the quantization of radio-frequency electromagnetic fields stored in a photonic microresonator. They were then able to manipulate the quantum state of the radio-frequency field, forming one- and two-photon Fock states within the microresonator, and analyze how the system interacts dynamically with its environment. The cQED approach could be used for fundamental studies in quantum thermodynamics and also find practical application in imaging. Science , this issue p. [1072][1] [1]: /lookup/doi/10.1126/science.aaw3101
In this PhD thesis, we will present the theoretical and experimental work that led to the realization of a radio-frequency circuit quantum electrodynamics system (RFcQED). In chapter 2, we provide a detailed derivation of the Hamiltonian of circuit QED formulated in the context of the Rabi model, and extract expressions for the cross-Kerr interaction. The resulting requirements for the coupling rate in RFcQED are discussed, one of them being the need to dramatically increase the coupling rate compared to typical circuit QED device. In chapter 3 we cover two experimental approaches to increasing the coupling in a circuit QED system, one making use of a high impedance resonator, the second utilizing a large coupling capacitor. In chapter 4, we combine these two approaches to implement RFcQED. Through strong dispersive coupling, we could measure individual photons in a megahertz resonator, demonstrate quantum control by cooling the resonator to the ground state or preparing Fock states, and finally observe with nanosecond resolution the re-thermalization of these states. In chapter 5 we present QuCAT or Quantum Circuit Analyzer Tool in Python, a software package that can be used for the design of circuit QED systems such as the one presented in this thesis. In chapter 6 we discuss how certain interplays between general relativity and quantum mechanics cannot be described using our current laws of physics. In particular, we show how radio-frequency mechanical oscillators are perfect candidates to perform experiments in this regime. In chapter 7 we present the prospects for coupling such mechanical oscillator to weakly anharmonic superconducting circuits such as the transmon qubit or RFcQED systems.
We experimentally demonstrate a recently proposed single-junction quantum-circuit refrigerator (QCR) as an tunable low-temperature environment for a superconducting 4.7 GHz resonator. With the help of a transmon qubit, we measure the populations of the different resonator Fock states, thus providing reliable access to the temperature of the engineered electromagnetic environment and its effect on the resonator. We demonstrate coherent and thermal resonator states and that the on-demand dissipation provided by the QCR can drive these to a small fraction of a photon on average, even if starting above 1 K. We observe that the QCR can be operated either with a dc bias voltage or a gigahertz rf drive, or a combination of these. The bandwidth of the rf drive is not limited by the circuit itself and consequently, we show that 2.9 GHz continuous and 10 ns pulsed drives lead to identical desired refrigeration of the resonator. These observations answer to the shortcomings of previous works where the Fock states were not resolvable and the QCR exhibited slow charging dynamics. Thus, this work introduces a versatile tool to study open quantum systems, quantum thermodynamics, and to quickly reset superconducting qubits. Published by the American Physical Society 2024
Quantum control over a physical system requires thermal fluctuations and thermal decoherence to be negligible, which becomes more challenging with decreasing natural frequencies of the target system. For microwave circuits, the quantum regime can be reached simply by cooling them to mK temperatures. Radio-frequency (RF) systems in the MHz regime, however, require further cooling or have to be coupled to an auxiliary quantum system with a coupling rate exceeding their thermal decoherence rate. A powerful tool to cool below the thermodynamic bath temperature is sideband-cooling, a technique that originated from the field of trapped ions and cold atoms and that has been applied in cavity optomechanics for groundstate cooling of mechanical motion. Here, we engineer a system of two superconducting LC circuits coupled by a current-mediated photon-pressure interaction and demonstrate sideband-cooling of a hot RF circuit using a microwave cavity and the regime of quantum-coherent coupling between the circuits. Due to a dramatically increased coupling strength, we obtain a large single-photon quantum cooperativity Cq0∼1\mathcal{C}_{\mathrm{q}0} \sim 1Cq0​∼1 and reduce the residual thermal RF occupancy by 75% through sideband-cooling with less than a single pump photon. For larger pump powers, the photon-pressure coupling rate exceeds the RF thermal decoherence rate by a factor of three and the RF circuit is cooled into the quantum groundstate. Our results demonstrate photon-pressure coupling with a hot radio-frequency circuit in the quantum regime and lay the foundation for radio-frequency quantum photonics.
Circuit quantum electrodynamics (cQED), exemplified by a coupled system of a superconducting qubit and a microwave cavity, is a powerful framework for the quantum control and measurement of macroscopic quantum states in solid-state circuits. Quantum circuits based on superconducting qubits have emerged as one of the leading platforms in the pursuit of fault-tolerant quantum computing. Despite significant progress in extending qubit lifetimes, refining experimental protocols, and scaling up quantum processors, errors arising from the control and measurement of superconducting qubits continue to hinder the realization of a universal quantum computer. To investigate the error mechanisms for state-of-the-art qubits, we realize long-lived superconducting transmon qubits that exhibit fluctuating lifetimes, with an average of 0.2 ms and a maximum exceeding 0.4 ms. We then investigate their dominant error mechanism. By introducing novel time-resolved error measurements that are synchronized with the operation of the pulse tube cooler in a dilution refrigerator, we find that mechanical vibrations from the pulse tube induce nonequilibrium dynamics in highly coherent qubits, leading to their correlated bit-flip errors. Our findings not only deepen our understanding of qubit error mechanisms but also provide valuable insights into potential error-mitigation strategies for achieving fault tolerance by decoupling superconducting qubits from their mechanical environments. We also present a novel scheme for operating a cQED system in a regime where the cavity is largely displaced. We find that a qubit drive at the bare cavity frequency can effectively displace the cavity field while minimizing the cavity-drive-induced dephasing and the ac Stark shift. Furthermore, we demonstrate that standard cQED protocols, such as qubit control, readout, and cavity single-photon generation, remain compatible with largely displaced cavity fields, even beyond the critical photon number. These findings open new pathways for exploring cQED dynamics in large-photon-number regimes, including the study of nonlinear phenomena in microwave cavities, the saturation of two-level system baths for extending the coherence of microwave quantum states, and the acceleration of the dispersive readout. Finally, mechanical resonators have emerged as integral components in quantum computing for storing and transducing quantum information. Low-frequency mechanical resonators, with extremely low energy dissipation rates, are particularly interesting for extending the lifetimes of stored quantum information. However, integrating low-frequency mechanical resonators with qubits is challenging because their small energy gaps make coherent energy exchange and ground-state preparation difficult. In this thesis, we report the first steps towards the characterization of a hybrid quantum device, consisting of a Transmon qubit and a circuit optomechanical system, both coupled to a 3D microwave cavity.
Owing to their strong dipole moment and long coherence times, superconducting qubits have demonstrated remarkable success in hybrid quantum circuits. However, most qubit architectures are limited to the GHz frequency range, severely constraining the class of systems they can interact with. The fluxonium qubit, on the other hand, can be biased to very low frequency while being manipulated and read out with standard microwave techniques. Here, we design and operate a heavy fluxonium with an unprecedentedly low transition frequency of 1.8 MHz. We demonstrate resolved sideband cooling of the “hot” qubit transition with a final ground state population of 97.7%, corresponding to an effective temperature of 23 μ K . We further demonstrate coherent manipulation with coherence times T 1 = 34 μ s , T 2 * = 39 μ s , and single-shot readout of the qubit state. Importantly, by directly addressing the qubit transition with a capacitively coupled waveguide, we showcase its high sensitivity to a radio-frequency field. Through cyclic qubit preparation and interrogation, we transform this low-frequency fluxonium qubit into a frequency-resolved charge sensor. This method results in a charge sensitivity of 33 μ e / Hz , or an energy sensitivity (in joules per hertz) of 2.8 ℏ . This method rivals state-of-the-art transport-based devices, while maintaining inherent insensitivity to dc-charge noise. The high charge sensitivity combined with large capacitive shunt unlocks new avenues for exploring quantum phenomena in the 1–10 MHz range, such as the strong-coupling regime with a resonant macroscopic mechanical resonator. Published by the American Physical Society 2024