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Science

Photoelectrical imaging and coherent spin-state readout of single nitrogen-vacancy centers in diamond

Petr Siyushev, Miloš Nesládek, Emilie Bourgeois, Michal Gulka, Jaroslav Hrubý, T. Yamamoto, Michael Trupke, Tokuyuki Teraji, Junichi Isoya, Fedor Jelezko

Published Feb 14, 2019• 194 citations
Publisher

Abstract

Nitrogen-vacancy (NV) centers in diamond have become an important instrument for quantum sensing and quantum information science. However, the readout of NV spin state requires bulky optical setups, limiting fabrication of miniaturized compact devices for practical use. Here we realized photoelectrical detection of magnetic resonance as well as Rabi oscillations on a single-defect level. Furthermore, photoelectrical imaging of individual NV centers at room temperature was demonstrated, surpassing conventional optical readout methods by providing high imaging contrast and signal-to-noise ratio. These results pave the way toward fully integrated quantum diamond devices.

DOI
10.1126/science.aav2789

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Nitrogen-vacancy (NV) centers in diamond have become an important instrument for quantum sensing and quantum information science. However, the readout of NV spin state requires bulky optical setups, limiting fabrication of miniaturized compact devices for practical use. Here we realized photoelectrical detection of magnetic resonance as well as Rabi oscillations on a single-defect level. Furthermore, photoelectrical imaging of individual NV centers at room temperature was demonstrated, surpassing conventional optical readout methods by providing high imaging contrast and signal-to-noise ratio. These results pave the way toward fully integrated quantum diamond devices.
Among the possible defects that can occur in diamonds, one that draws attention is the nitrogen-vacancy (NV) center.Studied since the early 90s, in recent years, they became one of the most promising platforms for field applications of quantum technology at room temperature, especially for quantum sensing.They are sensitive to electric and magnetic fields, temperature, and strain, making these nanosensors a versatile platform for many applications.The NV center's spin state is easy to read and manipulate by optical means, and, most interestingly, it works well at room temperature, which facilitates its use.The great challenge to implement quantum protocols and quantum algorithms is the coherence time of the quantum states.The NV center stands out for having relatively high coherence times at room temperature.This dissertation presents measurements to characterize the electron spin coherence of NV centers in an ultrapure sample of diamond designed for quantum sensing applications.These measurements combine optical e magnetic resonance techniques.For that, a method was implemented using a conventional CCD camera and a clever imaging protocol, making it possible to perform various pulsed microwave experiments on the electron spin, such as Rabi oscillations and Hahn spin-echo, which were used for determining the characteristic relaxation times (T 1 and T 2 ).Results show that this system provides at least two readily accessible qubits that can be used in quantum protocols even at room temperature.
The nitrogen-vacancy (NV) center in diamond is one of the advanced candidates for solid-state quantum computing at room temperature and has proven to be competitive in terms of gate fidelity and the availability of quantum error correction codes. Ambient solid-state qubits may therefore provide quantum computing architectures as an alternative to current solutions. The NV center has an associated electronic spin that is conventionally read out via photoluminescence. As an alternative, the electrical readout is not limited by the confocal resolution of quantum microscopes, which is required in the development of NV-based quantum processors to establish a scalable individual single-spin readout on the order of a few nanometers (necessary for strong dipole-dipole coupling). In this work, the performance of photoelectric readout versus traditional optical readout is investigated to perform Quantum State Tomography measurements on a single NV center. A state fidelity of 0.995 ±\pm± 0.006 is achieved using photoelectrical spin-state readout for state reconstruction, comparable to simultaneous optical measurements. We report photocurrent signal delays, which significantly slow down the photocurrent tomography. We develop a model describing their origin, and propose strategies for their mitigation.
Photoelectrical readout of the electronic spin state of the nitrogen-vacancy (NV) center in diamond is attracting significant interest due to the numerous advantages it possesses compared with conventional fluorescence readout. The higher charge carrier rate compared to the photon rate and the integration of the detection scheme on a chip can significantly advance quantum sensing and computing with color centers in diamond. Until now, photoelectric readout has been performed on ensembles of NV centers or single NV centers deep in ultrapure diamond substrates. However, many applications require the artificial creation and precise placement of shallow NV centers, and photoelectric detection of such centers has been challenging. Here we demonstrate photoelectrical readout and coherent control of the electronic spin of implanted shallow ($\sim$10 nm) NV centers buried by diamond overgrowth. The photoelectrically measured Ramsey T2∗T_2^*T2∗​ agrees with conventional fluorescence readout and shows no measurable dependence on the readout photocurrent, for both shallow implanted and deep ingrown NV centers. We further find that overgrowth improves photoelectric readout by suppressing the background photocurrent. These results establish photoelectric readout as a viable route to chip-integrated, electrically detected nanoscale sensing and to spin registers based on engineered shallow NV centers.
Nitrogen-vacancy (NV) centers in diamond are of great interest for nano- and macro-scale magnetic field sensing. Most sensing protocols rely on conventional optical readout, which is limited by photon shot noise. The recently developed photoelectrical (PE) readout of the NV center electron spin state promises to overcome these limitations. However, the noise of the PE readout and its influence on readout efficiency have not been thoroughly studied. In this work, we perform magnetic field sensing and estimate the sensitivity using optical and PE readout with a single and an ensemble of NV centers in diamond. We investigate the electronic noise associated with the photoelectric detection and estimate the readout efficiency, using Gaussian statistics. Our quantitative analysis shows that the Johnson-Nyquist noise-limited photoelectric magnetic field sensitivity could outperform optical measurements by an order of magnitude. This work is an essential step towards the development of on-chip magnetometers using photoelectrical detection in diamond.
Nitrogen-vacancy centers in diamond continue to attract much attention as a basis for hybrid quantum information processing. The authors develop the coherent manipulation and readout of the spin states of a small ensemble of centers, using tailored microwave pulse sequences to reduce background photocurrent and dramatically improve the signal to noise ratio. This technique is a major step toward single-spin quantum hardware featuring compact designs, easy on-chip integration, and operation at room temperature.