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Tuning nonthermal to thermal distributions in time-dependent Paul traps.

Haggai Landa

Published Sep 27, 2018• 0 citations
OpenAlex

Abstract

We study the probability distribution of an atomic ion being laser-cooled in a radio-frequency Paul trap, in terms of Hamiltonian action-angle coordinates appropriate for the time-dependent potential. Close to the effective minimum in many Paul traps, the periodically-driven potential is approximately quadratic in the coordinates. We find that despite the microscopic nonequilibrium forces, a stationary thermal-like exponential distribution in the action is reached after coarse-graining the angles, with a mean action corresponding to the Doppler cooling limit. However, residual electric fields can push the ion from the origin of the quadrupole potential and set it into a large-amplitude oscillation. Above a threshold amplitude of such excess micromotion, the action distribution for motion expanded about the driven oscillation broadens and becomes distinctly nonthermal. We find that by a proper choice of the laser detuning the distribution can be made exponential again, with a mean action close to the Doppler cooling limit. This is important for quantum information processing and other applications, and in particular the derived approach can be immediately applied to crystals of trapped ions in planar configurations, where the driven motion of ions is unavoidable.

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The problem of ion motion and laser cooling in a radio frequency quadrupole trap is considered. It is shown by a simple numerical calculation that for ion motion in the absence of laser cooling the effect of the time varying potential v(R-bar)cos(Omega x t) can be approximated by a time independent effective potential whenever the frequency of oscillation of the electric field, Omega is sufficiently greater than a resonant frequency, (Omega)squared = (sq. root of (2) times eVo)/M were e is the electronic charge, Vo is the maximum potential applied to the trap electrodes, and M is the mass of the ion. Equations for the Hamiltonian matrix elements in the presence of laser cooling, in the Lambe-Dicke limit are derived and studied to determine the cooling transitions. The equations of motion for the density matrix in the Lambe-Dicke limit are derived using a simple representation of spontaneous emission. (Theses) (Author)

•Dec 1, 1984•0 citations
We study the probability distribution of an atomic ion being laser-cooled in a radio-frequency Paul trap, in terms of Hamiltonian action-angle coordinates appropriate for the time-dependent potential. Close to the effective minimum in many Paul traps, the periodically-driven potential is approximately quadratic in the coordinates. We find that despite the microscopic nonequilibrium forces, a stationary thermal-like exponential distribution in the action is reached after coarse-graining the angles, with a mean action corresponding to the Doppler cooling limit. However, residual electric fields can push the ion from the origin of the quadrupole potential and set it into a large-amplitude oscillation. Above a threshold amplitude of such excess micromotion, the action distribution for motion expanded about the driven oscillation broadens and becomes distinctly nonthermal. We find that by a proper choice of the laser detuning the distribution can be made exponential again, with a mean action close to the Doppler cooling limit. This is important for quantum information processing and other applications, and in particular the derived approach can be immediately applied to crystals of trapped ions in planar configurations, where the driven motion of ions is unavoidable.
We study the probability distribution of an atomic ion being laser cooled in a periodically driven Paul trap using a Floquet approach to the semiclassical photon scattering dynamics. We show that despite the microscopic nonequilibrium forces, a stationary thermal-like exponential distribution can be obtained in the Hamiltonian action, or equivalently in the number of quanta (phonons) of the motion linearized about the zero of the potential. At the presence of additional stray electric fields, the ion is pushed from the origin of the potential and set into a large-amplitude driven oscillation, and above a threshold amplitude of such ``excess micromotion,'' the action distribution of excitations about the driven oscillation broadens and becomes distinctly nonthermal. We find that by a proper choice of the laser detuning, the distribution can be made exponential again, with a mean phonon number close to that of the Doppler cooling limit. We derive a relation allowing to deduce just from the experimentally observable photon scattering rate both the required detuning for optimal cooling and the final mean phonon number. These results are important for quantum information processing and other applications, and in particular the derived approach can be applied to crystals of trapped ions in planar configurations, where the driven motion of ions is unavoidable.
We study the stochastic dynamics of a particle in a periodically driven potential. For atomic ions trapped in radio-frequency Paul traps, noise heating and laser cooling typically act slowly in comparison with the unperturbed motion. These stochastic processes can be accounted for in terms of a probability distribution defined over the action variables, which would otherwise be conserved within the regular regions of the Hamiltonian phase space. We present a semiclassical theory of low-saturation laser cooling applicable from the limit of low-amplitude motion to large-amplitude motion, accounting fully for the time-dependent and anharmonic trap. We employ our approach to a detailed study of the stochastic dynamics of a single ion, drawing general conclusions regarding the nonequilibrium dynamics of laser-cooled trapped ions. We predict a regime of anharmonic motion in which laser cooling becomes diffusive (i.e., it is equally likely to cool the ion as it is to heat it), and can also turn into effective heating. This implies that a high-energy ion could be easily lost from the trap despite being laser cooled; however, we find that this loss can be counteracted using a laser detuning much larger than Doppler detuning.
Laser cooling of a single trapped ion in a Paul trap is discussed theoretically in the Lamb-Dicke limit, with full consideration of the time dependence of the trapping potential. Resulting mean kinetic energies are defined as time averages over one period of the micromotion and are compared with final temperatures expected from the laser-cooling treatment with harmonic traps. For laser-atom detunings close to the micromotion frequency the results differ significantly from those expected for a harmonic trap potential. A physical interpretation is given and simple formulas are derived for the strong confinement case.
We report on observations of the thermal motion of a single, Doppler-cooled ion along the axis of a linear radio-frequency quadrupole trap. We show that for a harmonic potential the thermal occupation of energy levels leads to a Gaussian distribution of the ion's axial position. The dependence of the spatial thermal spread on the trap potential is used for precise calibration of our imaging system's point spread function and sub-millikelvin thermometry. We employ this technique to investigate the laser detuning dependence of the Doppler temperature.
We study the time-dependent fluorescence of an initially hot, multilevel, single atomic ion trapped in a radio-frequency Paul trap during Doppler cooling. We have developed an analytical model that describes the fluorescence dynamics during Doppler cooling which is used to extract the initial energy of the ion. While previous models of Doppler cooling thermometry were limited to atoms with a two-level energy structure and neglected the effect of the trap oscillating electric fields, our model applies to atoms with multilevel energy structure and takes into account the influence of micromotion on the cooling dynamics. This thermometry applies to any initial energy distribution. We experimentally test our model with an ion prepared in coherent, thermal, and Tsallis energy distributions.
The problem of ion motion and laser cooling in a radio frequency quadrupole trap is considered. It is shown by a simple numerical calculation that for ion motion in the absence of laser cooling the effect of the time varying potential v(R-bar)cos(Omega x t) can be approximated by a time independent effective potential whenever the frequency of oscillation of the electric field, Omega is sufficiently greater than a resonant frequency, (Omega)squared = (sq. root of (2) times eVo)/M were e is the electronic charge, Vo is the maximum potential applied to the trap electrodes, and M is the mass of the ion. Equations for the Hamiltonian matrix elements in the presence of laser cooling, in the Lambe-Dicke limit are derived and studied to determine the cooling transitions. The equations of motion for the density matrix in the Lambe-Dicke limit are derived using a simple representation of spontaneous emission. (Theses) (Author)