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Physical Review A

Laser cooling of trapped ions: The influence of micromotion

J. I. Cirac, Luis J. Garay, R. Blatt, A. S. Parkins, P. Zoller

Published Jan 1, 1994• 77 citations
Publisher

Abstract

Laser cooling of a single trapped ion in a Paul trap is discussed theoretically in the Lamb-Dicke limit, with full consideration of the time dependence of the trapping potential. Resulting mean kinetic energies are defined as time averages over one period of the micromotion and are compared with final temperatures expected from the laser-cooling treatment with harmonic traps. For laser-atom detunings close to the micromotion frequency the results differ significantly from those expected for a harmonic trap potential. A physical interpretation is given and simple formulas are derived for the strong confinement case.

DOI
10.1103/physreva.49.421

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Laser cooling of a single trapped ion in a Paul trap is discussed theoretically in the Lamb-Dicke limit, with full consideration of the time dependence of the trapping potential. Resulting mean kinetic energies are defined as time averages over one period of the micromotion and are compared with final temperatures expected from the laser-cooling treatment with harmonic traps. For laser-atom detunings close to the micromotion frequency the results differ significantly from those expected for a harmonic trap potential. A physical interpretation is given and simple formulas are derived for the strong confinement case.
An experimental and theoretical study of laser sideband cooling of a trapped ion in a radiofrequency trap is presented. The influence of the micromotion in the time-dependent potential of a Paul trap can lead to a counterintuitive situation, where sideband cooling is possible for positive values of the laser detuning, i.e., for a laser frequency that is higher than the resonance frequency of the ion at rest. The cooling rate and the capture range are calculated in a semiclassical model. Experimental results of laser sideband cooling at positive detuning are demonstrated with a single trapped In+{\mathrm{In}}^{+}In+ ion stored in a miniature Paul trap.
The limitations to the achievement of low kinetic energies for laser cooling of single ions confined in electromagnetic traps are discussed. Sideband cooling of an ion in an rf (Paul) trap is reexamined including the effects of finite laser bandwidth and the energy of the rf micromotion. The micromotion is the oscillatory motion of the ion at the same frequency as the rf voltage applied to the trap electrodes. Sideband cooling of ions in a Penning trap is examined for the first time. In both cases, cooling to the zero-point energy of the ion in the trap should be possible and a method for verifying this condition is suggested. The implications for high-resolution, high-accuracy spectroscopy are investigated. Under certain conditions, the uncertainty in the second-order Doppler shift may be significantly less than 1 part in 1018{10}^{18}1018. .AE
Laser cooling of a single trapped ion with Zeeman substructure below the Doppler limit is considered theoretically. The laser field consists of two counterpropagating beams linearly polarized in different directions, and the internal atomic transition is Jg{\mathit{J}}_{\mathit{g}}Jg​=1/2\ensuremath{\rightarrow}Je{\mathit{J}}_{\mathit{e}}Je​=3/2. The ion is assumed to be localized to spatial dimensions smaller than the optical wavelength (Lamb-Dicke limit) and placed at a specific position with respect to the laser beams. Under the assumption that the rate for optical pumping between the atomic ground states defines the smallest time constant in the system, analytic expressions for the final energy and the cooling rates are derived, with both a semiclassical and a full quantum treatment. The results show that laser cooling of a trapped ion using polarization gradients leads to very low energies. These energies are insensitive to the precise localization of the ion with respect to the lasers, the angle between the direction of the polarizations of the laser beams, and the detuning of the cooling laser.
Laser cooling of trapped ions in a standing- and running-wave configuration is discussed theoretically. The ions are assumed to be spatially localized on the scale provided by the wavelength of the laser (Lamb-Dicke limit). A master equation for the center-of-mass distribution of the ion is derived for a multilevel system, and explicit results are presented for two- and three-level systems and harmonic trapping potentials. For the two-level system located at the node of the standing wave, we find final temperatures that are a factor of 2 lower than the limit for a running wave and cooling rates that do not saturate with the laser intensity. At the point of maximum gradient of the standing wave, blue detuned cooling is found that is analogous to the Sisyphus cooling of free atoms. For a three-level system we compare our results with those of Wineland, Dalibard, and Cohen-Tannoudji [J. Opt. Soc. Am. B 9, 32 (1992)].
We present a master equation that describes the dynamics of laser cooling of a trapped ion. It is valid in the Lamb–Dicke limit and rests on an adiabatic elimination combined with a degenerate perturbation treatment. It describes relaxation of probabilities and coherences in the harmonic-trap degrees of freedom. The eigenvalue spectrum the of the time-evolution operator is derived, and it follows that only one zero eigenvalue exists, giving the unique steady-state probability distribution. The coherences all decay to zero with time. The ultimate steady state is distribution, which can be characterized by a temperature. We also report a numerical calculation that a Planck supports our analytical work. The final energy of the cooling is given and discussed. Finally there is a comparison between the present results and our earlier, approximate, treatments.
We study laser cooling of two ions that are trapped in a harmonic potential and interact by Coulomb repulsion. Sideband cooling in the Lamb-Dicke regime is shown to work analogously to sideband cooling of a single ion. Outside the Lamb-Dicke regime, the incommensurable frequencies of the two vibrational modes result in a quasicontinuous energy spectrum that significantly alters the cooling dynamics. The cooling time decreases nonlinearly with the linewidth of the cooling transition, and the effect of dark states which may slow down the cooling is considerably reduced. We show that cooling to the ground state is also possible outside the Lamb-Dicke regime. We develop the model and use quantum Monte Carlo calculations for specific examples. We show that a rate equation treatment is a good approximation in all cases.